Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane
Nickel-supported Fibrous zeolite-Y (Ni/FHY) was successfully synthesized via the microemulsion method using HY as seed, followed by catalytic evaluation in dry reforming of methane (DRM) for hydrogen production. Ni/FHY possessed good NiO distribution, improved metal-support interface, and strong bas...
| Main Authors: | , , , , , , , |
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| Format: | Article |
| Language: | English English |
| Published: |
Elsevier Ltd
2023
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| Subjects: | |
| Online Access: | http://umpir.ump.edu.my/id/eprint/39200/ http://umpir.ump.edu.my/id/eprint/39200/1/Properties-activity%20correlation%20of%20Nickel%20supported.pdf http://umpir.ump.edu.my/id/eprint/39200/2/Properties-activity%20correlation%20of%20Nickel%20supported%20on%20fibrous%20zeolite-y%20for%20dry%20reforming%20of%20methane.pdf |
| _version_ | 1848825709078773760 |
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| author | S.N., Miskan H.D., Setiabudi M.B., Bahari Vo, Dai-Viet N. B., Abdullah A.A., Jalil S.A.F., Syed Muhammad S.B., Ismail |
| author_facet | S.N., Miskan H.D., Setiabudi M.B., Bahari Vo, Dai-Viet N. B., Abdullah A.A., Jalil S.A.F., Syed Muhammad S.B., Ismail |
| author_sort | S.N., Miskan |
| building | UMP Institutional Repository |
| collection | Online Access |
| description | Nickel-supported Fibrous zeolite-Y (Ni/FHY) was successfully synthesized via the microemulsion method using HY as seed, followed by catalytic evaluation in dry reforming of methane (DRM) for hydrogen production. Ni/FHY possessed good NiO distribution, improved metal-support interface, and strong basicity, accredited to the fibrous structure of FHY. This unique morphology led to the enrichment in the amount of accessible Ni active sites, thus resulting in the superior activity of Ni/FHY (XCH=95.1%,XCO=91.1%,H2/CO=0.89) compared to Ni/HY (XCH=92.7%,XCO=89.8%,H2/CO=0.78). Meanwhile, the inferior performance of Ni/HY could be caused by the poor distribution of Ni with large particles, thus contributing to high carbon deposition and Ni sintering. The unique physicochemical properties and superior catalytic activity confirmed its viability in the DRM. |
| first_indexed | 2025-11-15T03:33:14Z |
| format | Article |
| id | ump-39200 |
| institution | Universiti Malaysia Pahang |
| institution_category | Local University |
| language | English English |
| last_indexed | 2025-11-15T03:33:14Z |
| publishDate | 2023 |
| publisher | Elsevier Ltd |
| recordtype | eprints |
| repository_type | Digital Repository |
| spelling | ump-392002023-11-08T00:54:14Z http://umpir.ump.edu.my/id/eprint/39200/ Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane S.N., Miskan H.D., Setiabudi M.B., Bahari Vo, Dai-Viet N. B., Abdullah A.A., Jalil S.A.F., Syed Muhammad S.B., Ismail T Technology (General) TP Chemical technology Nickel-supported Fibrous zeolite-Y (Ni/FHY) was successfully synthesized via the microemulsion method using HY as seed, followed by catalytic evaluation in dry reforming of methane (DRM) for hydrogen production. Ni/FHY possessed good NiO distribution, improved metal-support interface, and strong basicity, accredited to the fibrous structure of FHY. This unique morphology led to the enrichment in the amount of accessible Ni active sites, thus resulting in the superior activity of Ni/FHY (XCH=95.1%,XCO=91.1%,H2/CO=0.89) compared to Ni/HY (XCH=92.7%,XCO=89.8%,H2/CO=0.78). Meanwhile, the inferior performance of Ni/HY could be caused by the poor distribution of Ni with large particles, thus contributing to high carbon deposition and Ni sintering. The unique physicochemical properties and superior catalytic activity confirmed its viability in the DRM. Elsevier Ltd 2023 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/39200/1/Properties-activity%20correlation%20of%20Nickel%20supported.pdf pdf en http://umpir.ump.edu.my/id/eprint/39200/2/Properties-activity%20correlation%20of%20Nickel%20supported%20on%20fibrous%20zeolite-y%20for%20dry%20reforming%20of%20methane.pdf S.N., Miskan and H.D., Setiabudi and M.B., Bahari and Vo, Dai-Viet N. and B., Abdullah and A.A., Jalil and S.A.F., Syed Muhammad and S.B., Ismail (2023) Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane. International Journal of Hydrogen Energy. ISSN 0360-3199. (In Press / Online First) (In Press / Online First) https://doi.org/10.1016/j.ijhydene.2022.12.201 10.1016/j.ijhydene.2022.12.201 |
| spellingShingle | T Technology (General) TP Chemical technology S.N., Miskan H.D., Setiabudi M.B., Bahari Vo, Dai-Viet N. B., Abdullah A.A., Jalil S.A.F., Syed Muhammad S.B., Ismail Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane |
| title | Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane |
| title_full | Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane |
| title_fullStr | Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane |
| title_full_unstemmed | Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane |
| title_short | Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane |
| title_sort | properties-activity correlation of nickel supported on fibrous zeolite-y for dry reforming of methane |
| topic | T Technology (General) TP Chemical technology |
| url | http://umpir.ump.edu.my/id/eprint/39200/ http://umpir.ump.edu.my/id/eprint/39200/ http://umpir.ump.edu.my/id/eprint/39200/ http://umpir.ump.edu.my/id/eprint/39200/1/Properties-activity%20correlation%20of%20Nickel%20supported.pdf http://umpir.ump.edu.my/id/eprint/39200/2/Properties-activity%20correlation%20of%20Nickel%20supported%20on%20fibrous%20zeolite-y%20for%20dry%20reforming%20of%20methane.pdf |