Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane

The prime cause for catalyst deactivation during dry reforming of methane (DRM) has been attributed to the deposition of carbon. Nanofibrous (NF) catalysts are attractive candidates that offer high catalytic activity and stability in DRM. A comparative study between electrospun and impregnated Co/Ce...

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Main Authors: Siti Nor Amira, Rosli, Nur Hidayati, Othman, Nguyen, Van Cuong, Sumaiya, Zainal Abidin
Format: Article
Language:English
English
Published: Wiley 2023
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/37965/
http://umpir.ump.edu.my/id/eprint/37965/1/Synergistic%20syngas%20production_%20Needleless%20electrospinning%20synthesis.pdf
http://umpir.ump.edu.my/id/eprint/37965/2/Synergistic%20syngas%20production_Needleless%20electrospinning%20synthesis_FULL.pdf
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author Siti Nor Amira, Rosli
Nur Hidayati, Othman
Nguyen, Van Cuong
Sumaiya, Zainal Abidin
author_facet Siti Nor Amira, Rosli
Nur Hidayati, Othman
Nguyen, Van Cuong
Sumaiya, Zainal Abidin
author_sort Siti Nor Amira, Rosli
building UMP Institutional Repository
collection Online Access
description The prime cause for catalyst deactivation during dry reforming of methane (DRM) has been attributed to the deposition of carbon. Nanofibrous (NF) catalysts are attractive candidates that offer high catalytic activity and stability in DRM. A comparative study between electrospun and impregnated Co/CeO2–La2O3 catalysts in the DRM reaction was carried out to evaluate the merits of the NF catalyst. Application of the electrospun catalyst yielded the highest activity in DRM and showed a substantial improvement in resistance to carbon formation. The unique structure of the NF electrospun catalyst, the robust metal-support interaction, and the increased surface area could more effectively suppress deactivation of the catalyst during an 8-h DRM reaction than the impregnated catalyst.
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institution Universiti Malaysia Pahang
institution_category Local University
language English
English
last_indexed 2025-11-15T03:28:11Z
publishDate 2023
publisher Wiley
recordtype eprints
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spelling ump-379652023-07-07T03:03:13Z http://umpir.ump.edu.my/id/eprint/37965/ Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane Siti Nor Amira, Rosli Nur Hidayati, Othman Nguyen, Van Cuong Sumaiya, Zainal Abidin TP Chemical technology The prime cause for catalyst deactivation during dry reforming of methane (DRM) has been attributed to the deposition of carbon. Nanofibrous (NF) catalysts are attractive candidates that offer high catalytic activity and stability in DRM. A comparative study between electrospun and impregnated Co/CeO2–La2O3 catalysts in the DRM reaction was carried out to evaluate the merits of the NF catalyst. Application of the electrospun catalyst yielded the highest activity in DRM and showed a substantial improvement in resistance to carbon formation. The unique structure of the NF electrospun catalyst, the robust metal-support interaction, and the increased surface area could more effectively suppress deactivation of the catalyst during an 8-h DRM reaction than the impregnated catalyst. Wiley 2023-06 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/37965/1/Synergistic%20syngas%20production_%20Needleless%20electrospinning%20synthesis.pdf pdf en http://umpir.ump.edu.my/id/eprint/37965/2/Synergistic%20syngas%20production_Needleless%20electrospinning%20synthesis_FULL.pdf Siti Nor Amira, Rosli and Nur Hidayati, Othman and Nguyen, Van Cuong and Sumaiya, Zainal Abidin (2023) Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane. Chemical Engineering and Technology, 40. pp. 1-10. ISSN 1521-4125. (Published) https://doi.org/10.1002/ceat.202300151 https://doi.org/10.1002/ceat.202300151
spellingShingle TP Chemical technology
Siti Nor Amira, Rosli
Nur Hidayati, Othman
Nguyen, Van Cuong
Sumaiya, Zainal Abidin
Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane
title Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane
title_full Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane
title_fullStr Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane
title_full_unstemmed Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane
title_short Synergistic syngas production: Needleless electrospinning synthesis of Co/CeO2–La2O3 catalyst for efficient dry reforming of methane
title_sort synergistic syngas production: needleless electrospinning synthesis of co/ceo2–la2o3 catalyst for efficient dry reforming of methane
topic TP Chemical technology
url http://umpir.ump.edu.my/id/eprint/37965/
http://umpir.ump.edu.my/id/eprint/37965/
http://umpir.ump.edu.my/id/eprint/37965/
http://umpir.ump.edu.my/id/eprint/37965/1/Synergistic%20syngas%20production_%20Needleless%20electrospinning%20synthesis.pdf
http://umpir.ump.edu.my/id/eprint/37965/2/Synergistic%20syngas%20production_Needleless%20electrospinning%20synthesis_FULL.pdf