Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite

Currently, biodegradable materials like polyhydroxyalkanoates (PHA) and polylactic acid (PLA) are receiving huge attention from the both scientific and industrial sectors. However, since PHA has poor thermal properties, there is a shortfall in the exploration of PHA ability with filler. Therefore, t...

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Main Authors: Nazaruddin, N. S., Saidatul Shima, Jamari
Format: Article
Language:English
Published: Universiti Malaysia Pahang 2021
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/33048/
http://umpir.ump.edu.my/id/eprint/33048/1/Effect%20on%20thermal%20properties%20of%20nanocellulose%20fibre.pdf
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author Nazaruddin, N. S.
Saidatul Shima, Jamari
author_facet Nazaruddin, N. S.
Saidatul Shima, Jamari
author_sort Nazaruddin, N. S.
building UMP Institutional Repository
collection Online Access
description Currently, biodegradable materials like polyhydroxyalkanoates (PHA) and polylactic acid (PLA) are receiving huge attention from the both scientific and industrial sectors. However, since PHA has poor thermal properties, there is a shortfall in the exploration of PHA ability with filler. Therefore, this research aim is to investigate the thermal effect of nanocellulose fiber (NCF) fillers with PHA polymer. The first solution of PHA composite is prepared by dissolving 1g of PHA in 40mL of dichloromethane at 30°C for 10 minutes. The PHA-NCF composite solution is prepared by adding 1wt%, 2wt%, 3wt%, and 4wt% of NCF dissolved in 40 mL of dichloromethane into the PHA solution. The mixture solution is agitated at 45°C with a magnetic stirrer for 10 minutes. The mixture is poured into a petri dish. The prepared films were characterized by Differential Scanning Calorimeter (DSC), Fourier Transforms Infrared Spectroscopy, (FTIR), and Thermogravimetric Analysis (TGA). The FTIR analysis shows that all PHA/NCF composite samples contain similar functional groups when compared with the pure PHA. No significant changes on the thermal properties of the PHA composite was observed with the addition of NCF fillers. However, comparison within the PHA/NCF samples shows that the PHA with 2% of NCF has a higher melting temperature and requires the highest enthalpy of melting. Hence, the addition of 2% of NCF is selected to be the optimum amount of NCF filler addition to the PHA composite.
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spelling ump-330482022-01-04T03:13:19Z http://umpir.ump.edu.my/id/eprint/33048/ Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite Nazaruddin, N. S. Saidatul Shima, Jamari TP Chemical technology Currently, biodegradable materials like polyhydroxyalkanoates (PHA) and polylactic acid (PLA) are receiving huge attention from the both scientific and industrial sectors. However, since PHA has poor thermal properties, there is a shortfall in the exploration of PHA ability with filler. Therefore, this research aim is to investigate the thermal effect of nanocellulose fiber (NCF) fillers with PHA polymer. The first solution of PHA composite is prepared by dissolving 1g of PHA in 40mL of dichloromethane at 30°C for 10 minutes. The PHA-NCF composite solution is prepared by adding 1wt%, 2wt%, 3wt%, and 4wt% of NCF dissolved in 40 mL of dichloromethane into the PHA solution. The mixture solution is agitated at 45°C with a magnetic stirrer for 10 minutes. The mixture is poured into a petri dish. The prepared films were characterized by Differential Scanning Calorimeter (DSC), Fourier Transforms Infrared Spectroscopy, (FTIR), and Thermogravimetric Analysis (TGA). The FTIR analysis shows that all PHA/NCF composite samples contain similar functional groups when compared with the pure PHA. No significant changes on the thermal properties of the PHA composite was observed with the addition of NCF fillers. However, comparison within the PHA/NCF samples shows that the PHA with 2% of NCF has a higher melting temperature and requires the highest enthalpy of melting. Hence, the addition of 2% of NCF is selected to be the optimum amount of NCF filler addition to the PHA composite. Universiti Malaysia Pahang 2021-04-29 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/33048/1/Effect%20on%20thermal%20properties%20of%20nanocellulose%20fibre.pdf Nazaruddin, N. S. and Saidatul Shima, Jamari (2021) Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite. Journal of Chemical Engineering and Industrial Biotechnology (JCEIB), 7 (1). pp. 10-13. ISSN 0126-8139. (Published) https://doi.org/10.15282/jceib.v7i1.6111 https://doi.org/10.15282/jceib.v7i1.6111
spellingShingle TP Chemical technology
Nazaruddin, N. S.
Saidatul Shima, Jamari
Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite
title Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite
title_full Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite
title_fullStr Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite
title_full_unstemmed Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite
title_short Effect on thermal properties of nanocellulose fibre (NCF) reinforced biodegradable polyhydroxylalkanoates (PHA) composite
title_sort effect on thermal properties of nanocellulose fibre (ncf) reinforced biodegradable polyhydroxylalkanoates (pha) composite
topic TP Chemical technology
url http://umpir.ump.edu.my/id/eprint/33048/
http://umpir.ump.edu.my/id/eprint/33048/
http://umpir.ump.edu.my/id/eprint/33048/
http://umpir.ump.edu.my/id/eprint/33048/1/Effect%20on%20thermal%20properties%20of%20nanocellulose%20fibre.pdf