Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies

In the present study, 2-bromo-4-chlorophenyl-2-bromobutanoate (3) was synthesized via the reaction of 2-bromo-4-chlorophenol with 2-bromobutanoyl bromide in the presence of pyridine. A variety of 2-bromo-4-chlorophenyl-2-bromobutanoate derivatives (5a–f) were synthesized with moderate to good yields...

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Main Authors: Nazeer, Usman, Rasool, Nasir, Aqsa, Mujahid, Mansha, Asim, Muhammad Zubair, Abdul Wahab Saaroni, Kosar, Naveen, Mahmood, Tariq, Ali Raza, Shah, Syed Adnan, Ali Shah, Zainul Amiruddin, Zakaria, Muhammad Nadeem, Akhtar
Format: Article
Language:English
Published: MDPI - Open Access Publishing 2020
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Online Access:https://umpir.ump.edu.my/id/eprint/29288/
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author Nazeer, Usman
Rasool, Nasir
Aqsa, Mujahid
Mansha, Asim
Muhammad Zubair, Abdul Wahab Saaroni
Kosar, Naveen
Mahmood, Tariq
Ali Raza, Shah
Syed Adnan, Ali Shah
Zainul Amiruddin, Zakaria
Muhammad Nadeem, Akhtar
author_facet Nazeer, Usman
Rasool, Nasir
Aqsa, Mujahid
Mansha, Asim
Muhammad Zubair, Abdul Wahab Saaroni
Kosar, Naveen
Mahmood, Tariq
Ali Raza, Shah
Syed Adnan, Ali Shah
Zainul Amiruddin, Zakaria
Muhammad Nadeem, Akhtar
author_sort Nazeer, Usman
building UMP Institutional Repository
collection Online Access
description In the present study, 2-bromo-4-chlorophenyl-2-bromobutanoate (3) was synthesized via the reaction of 2-bromo-4-chlorophenol with 2-bromobutanoyl bromide in the presence of pyridine. A variety of 2-bromo-4-chlorophenyl-2-bromobutanoate derivatives (5a–f) were synthesized with moderate to good yields via a Pd-catalyzed Suzuki cross-coupling reaction. To find out the reactivity and electronic properties of the compounds, Frontier molecular orbital analysis, non-linear optical properties, and molecular electrostatic potential studies were performed.
first_indexed 2025-11-15T03:58:06Z
format Article
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institution Universiti Malaysia Pahang
institution_category Local University
language English
last_indexed 2025-11-15T03:58:06Z
publishDate 2020
publisher MDPI - Open Access Publishing
recordtype eprints
repository_type Digital Repository
spelling ump-292882025-09-29T02:07:45Z https://umpir.ump.edu.my/id/eprint/29288/ Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies Nazeer, Usman Rasool, Nasir Aqsa, Mujahid Mansha, Asim Muhammad Zubair, Abdul Wahab Saaroni Kosar, Naveen Mahmood, Tariq Ali Raza, Shah Syed Adnan, Ali Shah Zainul Amiruddin, Zakaria Muhammad Nadeem, Akhtar Q Science (General) QC Physics QD Chemistry In the present study, 2-bromo-4-chlorophenyl-2-bromobutanoate (3) was synthesized via the reaction of 2-bromo-4-chlorophenol with 2-bromobutanoyl bromide in the presence of pyridine. A variety of 2-bromo-4-chlorophenyl-2-bromobutanoate derivatives (5a–f) were synthesized with moderate to good yields via a Pd-catalyzed Suzuki cross-coupling reaction. To find out the reactivity and electronic properties of the compounds, Frontier molecular orbital analysis, non-linear optical properties, and molecular electrostatic potential studies were performed. MDPI - Open Access Publishing 2020 Article PeerReviewed pdf en cc_by_4 https://umpir.ump.edu.my/id/eprint/29288/1/10.%20Selective%20Arylation%20of%202-Bromo-4-chlorophenyl-2-bromobutanoate%20via%20a%20Pd.pdf Nazeer, Usman and Rasool, Nasir and Aqsa, Mujahid and Mansha, Asim and Muhammad Zubair, Abdul Wahab Saaroni and Kosar, Naveen and Mahmood, Tariq and Ali Raza, Shah and Syed Adnan, Ali Shah and Zainul Amiruddin, Zakaria and Muhammad Nadeem, Akhtar (2020) Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies. Molecules, 25 (15). pp. 1-14. ISSN 1420-3049 (print); 1420-3049 (online). (Published) https://doi.org/10.3390/molecules25153521 https://doi.org/10.3390/molecules25153521 https://doi.org/10.3390/molecules25153521
spellingShingle Q Science (General)
QC Physics
QD Chemistry
Nazeer, Usman
Rasool, Nasir
Aqsa, Mujahid
Mansha, Asim
Muhammad Zubair, Abdul Wahab Saaroni
Kosar, Naveen
Mahmood, Tariq
Ali Raza, Shah
Syed Adnan, Ali Shah
Zainul Amiruddin, Zakaria
Muhammad Nadeem, Akhtar
Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies
title Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies
title_full Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies
title_fullStr Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies
title_full_unstemmed Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies
title_short Selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (NLO) properties via dft studies
title_sort selective arylation of 2-bromo-4-chlorophenyl-2-bromobutanoate via a pd-catalyzed suzuki cross-coupling reaction and its electronic and non-linear optical (nlo) properties via dft studies
topic Q Science (General)
QC Physics
QD Chemistry
url https://umpir.ump.edu.my/id/eprint/29288/
https://umpir.ump.edu.my/id/eprint/29288/
https://umpir.ump.edu.my/id/eprint/29288/