Ferrocene functionalized multi-walled carbon nanotubes as supercapacitor electrodes

Modified multi-walled carbon nanotubes (MWCNTs) functionalized by a redox-active ferrocene (Fc-MWCNTs) were successfully synthesized to enhance the electrochemical performance of MWCNTs for supercapacitor application. The ferrocene moieties were attached to the surface of MWCNTs via a thiourea linke...

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Bibliographic Details
Main Authors: Ali, Gomaa A. M., Megiel, Elzbieta, Cieciórski, Piotr, Thalji, Mohammad R., Romański, Jan, Algarni, H., K. F., Chong
Format: Article
Language:English
Published: Elsevier 2020
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/29155/
http://umpir.ump.edu.my/id/eprint/29155/1/Ferrocene%20functionalized%20multi1.pdf
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Summary:Modified multi-walled carbon nanotubes (MWCNTs) functionalized by a redox-active ferrocene (Fc-MWCNTs) were successfully synthesized to enhance the electrochemical performance of MWCNTs for supercapacitor application. The ferrocene moieties were attached to the surface of MWCNTs via a thiourea linker with anions-interacting capability. The Fc-MWCNTs were characterized using XPS, FTIR, SEM, TGA, DTG, and XRF methods. The electrochemical performance details were investigated using cyclic voltammetry, galvanostatic charge-discharge, and electrochemical impedance spectroscopy. The Fc-MWCNTs electrode showed excellent capacity retention (90.8% over 5000 cycles) and a specific capacitance of 50 F g−1 at 0.25 A g−1 that is several times higher as compared to the pristine MWCNTs. The fabricated Fc-MWCNTs is proposed to be a suitable and promising candidate for energy storage material. dec