Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic

Enhancing the optical performance of rare earth doped binary inorganic glasses is an everdemanding quest. Samarium (Sm3+) doped zinc tellurite glasses containing Manganese (Mn) nanoparticles (NPs) with composition (59-x)TeO2-20ZnCl2-10ZnO-10Li2O-1Sm2O3-(x)Mn3O4, where x = 0 to 0.06 mol% are prepared...

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Main Authors: Nurul Ainaa Najihah, Busra, Ramli, Arifin, Goshal, Sib Krishna, Rodziah, Nazlan
Format: Article
Language:English
Published: Trans Tech Publications 2020
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/28578/
http://umpir.ump.edu.my/id/eprint/28578/7/Role%20of%20Sm3%20on%20Mn%20Nanoparticles%20Embedded%20Zinc%20Tellurite%20Glasses.pdf
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author Nurul Ainaa Najihah, Busra
Ramli, Arifin
Goshal, Sib Krishna
Rodziah, Nazlan
author_facet Nurul Ainaa Najihah, Busra
Ramli, Arifin
Goshal, Sib Krishna
Rodziah, Nazlan
author_sort Nurul Ainaa Najihah, Busra
building UMP Institutional Repository
collection Online Access
description Enhancing the optical performance of rare earth doped binary inorganic glasses is an everdemanding quest. Samarium (Sm3+) doped zinc tellurite glasses containing Manganese (Mn) nanoparticles (NPs) with composition (59-x)TeO2-20ZnCl2-10ZnO-10Li2O-1Sm2O3-(x)Mn3O4, where x = 0 to 0.06 mol% are prepared by melt quenching technique. The role played by Mn NPs in enhancing the optical behaviors are analyzed and discussed. The XRD patterns confirm the amorphous nature of the glass. The UV-Vis-NIR spectra reveal seven prominent absorption bands of Sm3+ ions. The photoluminescence spectra display four peaks corresponding to 4G5/2→6H5/2, 4G5/2 →6H7/2, 4G5/2→6H9/2 and 4G5/2 →6H11/2 transitions. An enhancement in the luminescence intensity is observed up to 0.05 mol% concentration of NPs and the intensity quenches beyond it. The enhancement is attributed to local electric field effect of NPs in the proximity of Sm3+ ion. Our results on improved optical response via precise control of NPs contents may be useful for the development of solid state lasers and amplifiers.
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spelling ump-285782021-02-08T08:21:12Z http://umpir.ump.edu.my/id/eprint/28578/ Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic Nurul Ainaa Najihah, Busra Ramli, Arifin Goshal, Sib Krishna Rodziah, Nazlan QC Physics Enhancing the optical performance of rare earth doped binary inorganic glasses is an everdemanding quest. Samarium (Sm3+) doped zinc tellurite glasses containing Manganese (Mn) nanoparticles (NPs) with composition (59-x)TeO2-20ZnCl2-10ZnO-10Li2O-1Sm2O3-(x)Mn3O4, where x = 0 to 0.06 mol% are prepared by melt quenching technique. The role played by Mn NPs in enhancing the optical behaviors are analyzed and discussed. The XRD patterns confirm the amorphous nature of the glass. The UV-Vis-NIR spectra reveal seven prominent absorption bands of Sm3+ ions. The photoluminescence spectra display four peaks corresponding to 4G5/2→6H5/2, 4G5/2 →6H7/2, 4G5/2→6H9/2 and 4G5/2 →6H11/2 transitions. An enhancement in the luminescence intensity is observed up to 0.05 mol% concentration of NPs and the intensity quenches beyond it. The enhancement is attributed to local electric field effect of NPs in the proximity of Sm3+ ion. Our results on improved optical response via precise control of NPs contents may be useful for the development of solid state lasers and amplifiers. Trans Tech Publications 2020 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/28578/7/Role%20of%20Sm3%20on%20Mn%20Nanoparticles%20Embedded%20Zinc%20Tellurite%20Glasses.pdf Nurul Ainaa Najihah, Busra and Ramli, Arifin and Goshal, Sib Krishna and Rodziah, Nazlan (2020) Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic. Materials Science Forum, 981. pp. 73-77. ISSN 0255-5476. (Published) https://doi.org/10.4028/www.scientific.net/MSF.981.73 https://doi.org/10.4028/www.scientific.net/MSF.981.73
spellingShingle QC Physics
Nurul Ainaa Najihah, Busra
Ramli, Arifin
Goshal, Sib Krishna
Rodziah, Nazlan
Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic
title Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic
title_full Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic
title_fullStr Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic
title_full_unstemmed Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic
title_short Role of Sm3+ on Mn Nanoparticles Embedded Zinc Tellurite Glasses: Absorption and Luminescence Characteristic
title_sort role of sm3+ on mn nanoparticles embedded zinc tellurite glasses: absorption and luminescence characteristic
topic QC Physics
url http://umpir.ump.edu.my/id/eprint/28578/
http://umpir.ump.edu.my/id/eprint/28578/
http://umpir.ump.edu.my/id/eprint/28578/
http://umpir.ump.edu.my/id/eprint/28578/7/Role%20of%20Sm3%20on%20Mn%20Nanoparticles%20Embedded%20Zinc%20Tellurite%20Glasses.pdf