Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions

Waste corn-cob cellulose supported poly(amidoxime) palladium nanoparticles (PdNs@PA) were prepared by the surface modification of waste corn-cob cellulose through graft co-polymerization and subsequent amidoximation. The supported nanoperticles showed high catalytic activity (45-400 mol ppm) toward...

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Main Authors: Sultana, Tahnim, Mandal, Bablu Hira, Lutfor, M. R., Sarkar, Shaheen M.
Format: Article
Published: Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim 2016
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/16925/
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author Sultana, Tahnim
Mandal, Bablu Hira
Lutfor, M. R.
Sarkar, Shaheen M.
author_facet Sultana, Tahnim
Mandal, Bablu Hira
Lutfor, M. R.
Sarkar, Shaheen M.
author_sort Sultana, Tahnim
building UMP Institutional Repository
collection Online Access
description Waste corn-cob cellulose supported poly(amidoxime) palladium nanoparticles (PdNs@PA) were prepared by the surface modification of waste corn-cob cellulose through graft co-polymerization and subsequent amidoximation. The supported nanoperticles showed high catalytic activity (45-400 mol ppm) towards Suzuki-Miyaura cross-coupling of aryl bromides/chlorides with organoboronic acids to give the corresponding biaryl products up to 99% yield with high turnover number (TON) 19777 and turnover frequency (TOF) 4944 h-1. The PdNs@PA was easily recovered from the reaction mixture and reused several times without significant loss of its catalytic activity
first_indexed 2025-11-15T02:07:19Z
format Article
id ump-16925
institution Universiti Malaysia Pahang
institution_category Local University
last_indexed 2025-11-15T02:07:19Z
publishDate 2016
publisher Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim
recordtype eprints
repository_type Digital Repository
spelling ump-169252019-09-10T02:29:00Z http://umpir.ump.edu.my/id/eprint/16925/ Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions Sultana, Tahnim Mandal, Bablu Hira Lutfor, M. R. Sarkar, Shaheen M. QD Chemistry Waste corn-cob cellulose supported poly(amidoxime) palladium nanoparticles (PdNs@PA) were prepared by the surface modification of waste corn-cob cellulose through graft co-polymerization and subsequent amidoximation. The supported nanoperticles showed high catalytic activity (45-400 mol ppm) towards Suzuki-Miyaura cross-coupling of aryl bromides/chlorides with organoboronic acids to give the corresponding biaryl products up to 99% yield with high turnover number (TON) 19777 and turnover frequency (TOF) 4944 h-1. The PdNs@PA was easily recovered from the reaction mixture and reused several times without significant loss of its catalytic activity Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim 2016 Article PeerReviewed Sultana, Tahnim and Mandal, Bablu Hira and Lutfor, M. R. and Sarkar, Shaheen M. (2016) Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions. ChemistrySelect, 1 (13). pp. 4108-4112. ISSN 2365-6549. (Published) http://dx.doi.org/10.1002/slct.201600537 DOI: 10.1002/slct.201600537
spellingShingle QD Chemistry
Sultana, Tahnim
Mandal, Bablu Hira
Lutfor, M. R.
Sarkar, Shaheen M.
Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions
title Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions
title_full Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions
title_fullStr Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions
title_full_unstemmed Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions
title_short Bio-Waste Corn–cob Cellulose Supported Poly(amidoxime) Palladium Nanoparticles for Suzuki-Miyaura Cross-Coupling Reactions
title_sort bio-waste corn–cob cellulose supported poly(amidoxime) palladium nanoparticles for suzuki-miyaura cross-coupling reactions
topic QD Chemistry
url http://umpir.ump.edu.my/id/eprint/16925/
http://umpir.ump.edu.my/id/eprint/16925/
http://umpir.ump.edu.my/id/eprint/16925/