[O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I)

The synthesis, spectroscopic characterization and X-ray crystal structure of the title compound, (4-tolyl)3PAu[SC(O-i-Pr)=NC6H4NO2-4] (1) are described. Spectroscopy exhibited the expected features confirming the formation of the compound. The molecular structure of 1 confirms the expected linear P–...

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Main Authors: Yeo, Chien Ing *, Tiekink, Edward R. T. *
Format: Article
Language:English
Published: MDPI 2018
Subjects:
Online Access:http://eprints.sunway.edu.my/933/
http://eprints.sunway.edu.my/933/1/Tiekink%20Molbank-2018.pdf
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author Yeo, Chien Ing *
Tiekink, Edward R. T. *
author_facet Yeo, Chien Ing *
Tiekink, Edward R. T. *
author_sort Yeo, Chien Ing *
building SU Institutional Repository
collection Online Access
description The synthesis, spectroscopic characterization and X-ray crystal structure of the title compound, (4-tolyl)3PAu[SC(O-i-Pr)=NC6H4NO2-4] (1) are described. Spectroscopy exhibited the expected features confirming the formation of the compound. The molecular structure of 1 confirms the expected linear P–Au–S coordination geometry defined by thiolate-S and phosphane-P atoms. The nearly 7◦ deviation from linearity is ascribed to the close approach of the imine-bound phenyl group, indicative of a semi-localized Au . . . π(arene) interaction. The three-dimensional molecular packing is consolidated by methyl- and tolyl-C–H . . . O(nitro) and tolyl-C–H . . . π(tolyl) interactions.
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spelling sunway-9332020-10-12T07:49:29Z http://eprints.sunway.edu.my/933/ [O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I) Yeo, Chien Ing * Tiekink, Edward R. T. * QD Chemistry The synthesis, spectroscopic characterization and X-ray crystal structure of the title compound, (4-tolyl)3PAu[SC(O-i-Pr)=NC6H4NO2-4] (1) are described. Spectroscopy exhibited the expected features confirming the formation of the compound. The molecular structure of 1 confirms the expected linear P–Au–S coordination geometry defined by thiolate-S and phosphane-P atoms. The nearly 7◦ deviation from linearity is ascribed to the close approach of the imine-bound phenyl group, indicative of a semi-localized Au . . . π(arene) interaction. The three-dimensional molecular packing is consolidated by methyl- and tolyl-C–H . . . O(nitro) and tolyl-C–H . . . π(tolyl) interactions. MDPI 2018 Article PeerReviewed text en http://eprints.sunway.edu.my/933/1/Tiekink%20Molbank-2018.pdf Yeo, Chien Ing * and Tiekink, Edward R. T. * (2018) [O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I). Molbank, 2018 (4). M1028. ISSN 1422-8599 http://doi.org/10.3390/M1028 doi:10.3390/M1028
spellingShingle QD Chemistry
Yeo, Chien Ing *
Tiekink, Edward R. T. *
[O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I)
title [O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I)
title_full [O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I)
title_fullStr [O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I)
title_full_unstemmed [O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I)
title_short [O-Isopropyl-N-(4-nitrophenyl)thiocarbamato-κS]-(tri-4-tolylphosphine-κP)gold(I)
title_sort [o-isopropyl-n-(4-nitrophenyl)thiocarbamato-κs]-(tri-4-tolylphosphine-κp)gold(i)
topic QD Chemistry
url http://eprints.sunway.edu.my/933/
http://eprints.sunway.edu.my/933/
http://eprints.sunway.edu.my/933/
http://eprints.sunway.edu.my/933/1/Tiekink%20Molbank-2018.pdf