Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis

The title ZnII complex, [Zn(C19H20N3OS)2] {systematic name: bis[(N-ethyl-N0-{(Z)-[(2E)-3-(4-methoxyphenyl)-1-phenylprop-2-en-1-ylidene]amino}carbamimidoyl)sulfanido]zinc(II)}, features a tetrahedrally coordinated ZnII ion within an N2S2 donor set provided by two N,S-chelating thiosemicarbazone anio...

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Main Authors: Tan, Ming Yueh, Crouse, Karen A., Ravoof, Thahira Begum S. A., Jotani, Mukesh M., Tiekink, Edward R. T. *
Format: Article
Language:English
Published: 2018
Subjects:
Online Access:http://eprints.sunway.edu.my/736/
http://eprints.sunway.edu.my/736/1/Tiekink%20Bis%20%284-methoxychalcone%20....%29Acta%20Cryst%202018%20E74%20151.pdf
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author Tan, Ming Yueh
Crouse, Karen A.
Ravoof, Thahira Begum S. A.
Jotani, Mukesh M.
Tiekink, Edward R. T. *
author_facet Tan, Ming Yueh
Crouse, Karen A.
Ravoof, Thahira Begum S. A.
Jotani, Mukesh M.
Tiekink, Edward R. T. *
author_sort Tan, Ming Yueh
building SU Institutional Repository
collection Online Access
description The title ZnII complex, [Zn(C19H20N3OS)2] {systematic name: bis[(N-ethyl-N0-{(Z)-[(2E)-3-(4-methoxyphenyl)-1-phenylprop-2-en-1-ylidene]amino}carbamimidoyl)sulfanido]zinc(II)}, features a tetrahedrally coordinated ZnII ion within an N2S2 donor set provided by two N,S-chelating thiosemicarbazone anions. The resulting five-membered Zn,C,N2,S chelate rings adopt different conformations, i.e. almost planar and an envelope with the Zn atom being the flap atom. The configuration about the imine bond within the chelate ring is Z but those about the exocyclic imine and ethylene bonds are E. In the crystal, supramolecular [100] chains mediated by thioamide-N—H...S(thione) hydrogen bonds and eight-membered thioamide {.....HNCS}2 synthons are observed. A range of interactions, including C—H...O, C—H...., C—H....(chelate ring) and .(methoxybenzene)—.(chelate ring) consolidate the packing. The Hirshfeld surface analysis performed on the title complex also indicates the influence of the interactions involving the chelate rings upon the packing along with the more conventional contacts.
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spelling sunway-7362020-10-07T09:18:46Z http://eprints.sunway.edu.my/736/ Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis Tan, Ming Yueh Crouse, Karen A. Ravoof, Thahira Begum S. A. Jotani, Mukesh M. Tiekink, Edward R. T. * QD Chemistry The title ZnII complex, [Zn(C19H20N3OS)2] {systematic name: bis[(N-ethyl-N0-{(Z)-[(2E)-3-(4-methoxyphenyl)-1-phenylprop-2-en-1-ylidene]amino}carbamimidoyl)sulfanido]zinc(II)}, features a tetrahedrally coordinated ZnII ion within an N2S2 donor set provided by two N,S-chelating thiosemicarbazone anions. The resulting five-membered Zn,C,N2,S chelate rings adopt different conformations, i.e. almost planar and an envelope with the Zn atom being the flap atom. The configuration about the imine bond within the chelate ring is Z but those about the exocyclic imine and ethylene bonds are E. In the crystal, supramolecular [100] chains mediated by thioamide-N—H...S(thione) hydrogen bonds and eight-membered thioamide {.....HNCS}2 synthons are observed. A range of interactions, including C—H...O, C—H...., C—H....(chelate ring) and .(methoxybenzene)—.(chelate ring) consolidate the packing. The Hirshfeld surface analysis performed on the title complex also indicates the influence of the interactions involving the chelate rings upon the packing along with the more conventional contacts. 2018 Article PeerReviewed text en http://eprints.sunway.edu.my/736/1/Tiekink%20Bis%20%284-methoxychalcone%20....%29Acta%20Cryst%202018%20E74%20151.pdf Tan, Ming Yueh and Crouse, Karen A. and Ravoof, Thahira Begum S. A. and Jotani, Mukesh M. and Tiekink, Edward R. T. * (2018) Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis. Acta Crystallographica Section E Crystallographic Communications, 74 (2). pp. 151-157. ISSN 2056-9890 http://dx.doi.org/10.1107/s2056989018000282 doi:10.1107/s2056989018000282
spellingShingle QD Chemistry
Tan, Ming Yueh
Crouse, Karen A.
Ravoof, Thahira Begum S. A.
Jotani, Mukesh M.
Tiekink, Edward R. T. *
Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis
title Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis
title_full Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis
title_fullStr Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis
title_full_unstemmed Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis
title_short Bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 N 1,S)zinc(II): Crystal structure and Hirshfeld surface analysis
title_sort bis(4-methoxychalcone 4-ethylthiosemicarbazonato-κ2 n 1,s)zinc(ii): crystal structure and hirshfeld surface analysis
topic QD Chemistry
url http://eprints.sunway.edu.my/736/
http://eprints.sunway.edu.my/736/
http://eprints.sunway.edu.my/736/
http://eprints.sunway.edu.my/736/1/Tiekink%20Bis%20%284-methoxychalcone%20....%29Acta%20Cryst%202018%20E74%20151.pdf