N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis

In the title carbohydrazide, C10H7N3O4S, the dihedral angle between the terminal five-membered rings is 27.4 (2)°, with these lying to the same side of the plane through the central CN2C(=O) atoms (r.m.s. deviation = 0.0403 Å), leading to a curved mol­ecule. The conformation about the C=N imine bond...

Full description

Bibliographic Details
Main Authors: Cardoso, Laura N. F., Nogueira, Thais C. M., Wardell, James L., Wardell, Solange M. S. V., Souza, Marcus V. N. de, Jotani, Mukesh M., Tiekink, Edward R. T. *
Format: Article
Language:English
Published: International Union of Crystallography 2016
Subjects:
Online Access:http://eprints.sunway.edu.my/644/
http://eprints.sunway.edu.my/644/1/Acta%20E_RC%202016%2072%201025.pdf
_version_ 1848801867739430912
author Cardoso, Laura N. F.
Nogueira, Thais C. M.
Wardell, James L.
Wardell, Solange M. S. V.
Souza, Marcus V. N. de
Jotani, Mukesh M.
Tiekink, Edward R. T. *
author_facet Cardoso, Laura N. F.
Nogueira, Thais C. M.
Wardell, James L.
Wardell, Solange M. S. V.
Souza, Marcus V. N. de
Jotani, Mukesh M.
Tiekink, Edward R. T. *
author_sort Cardoso, Laura N. F.
building SU Institutional Repository
collection Online Access
description In the title carbohydrazide, C10H7N3O4S, the dihedral angle between the terminal five-membered rings is 27.4 (2)°, with these lying to the same side of the plane through the central CN2C(=O) atoms (r.m.s. deviation = 0.0403 Å), leading to a curved mol­ecule. The conformation about the C=N imine bond [1.281 (5) Å] is E, and the carbonyl O and amide H atoms are anti. In the crystal, N-H...O hydrogen bonds lead to supra­molecular chains, generated by a 41 screw-axis along the c direction. A three-dimensional architecture is consolidated by thienyl-C-H...O(nitro) and furanyl-C-H...O(nitro) inter­actions, as well as [pi]-[pi] inter­actions between the thienyl and furanyl rings [inter-centroid distance = 3.515 (2) Å]. These, and other, weak inter­molecular inter­actions, e.g. nitro-N-O...[pi](thien­yl), have been investigated by Hirshfeld surface analysis, which confirms the dominance of the conventional N-H...O hydrogen bonding to the overall mol­ecular packing.
first_indexed 2025-11-14T21:14:17Z
format Article
id sunway-644
institution Sunway University
institution_category Local University
language English
last_indexed 2025-11-14T21:14:17Z
publishDate 2016
publisher International Union of Crystallography
recordtype eprints
repository_type Digital Repository
spelling sunway-6442020-10-07T10:01:23Z http://eprints.sunway.edu.my/644/ N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis Cardoso, Laura N. F. Nogueira, Thais C. M. Wardell, James L. Wardell, Solange M. S. V. Souza, Marcus V. N. de Jotani, Mukesh M. Tiekink, Edward R. T. * QD Chemistry In the title carbohydrazide, C10H7N3O4S, the dihedral angle between the terminal five-membered rings is 27.4 (2)°, with these lying to the same side of the plane through the central CN2C(=O) atoms (r.m.s. deviation = 0.0403 Å), leading to a curved mol­ecule. The conformation about the C=N imine bond [1.281 (5) Å] is E, and the carbonyl O and amide H atoms are anti. In the crystal, N-H...O hydrogen bonds lead to supra­molecular chains, generated by a 41 screw-axis along the c direction. A three-dimensional architecture is consolidated by thienyl-C-H...O(nitro) and furanyl-C-H...O(nitro) inter­actions, as well as [pi]-[pi] inter­actions between the thienyl and furanyl rings [inter-centroid distance = 3.515 (2) Å]. These, and other, weak inter­molecular inter­actions, e.g. nitro-N-O...[pi](thien­yl), have been investigated by Hirshfeld surface analysis, which confirms the dominance of the conventional N-H...O hydrogen bonding to the overall mol­ecular packing. International Union of Crystallography 2016 Article PeerReviewed text en http://eprints.sunway.edu.my/644/1/Acta%20E_RC%202016%2072%201025.pdf Cardoso, Laura N. F. and Nogueira, Thais C. M. and Wardell, James L. and Wardell, Solange M. S. V. and Souza, Marcus V. N. de and Jotani, Mukesh M. and Tiekink, Edward R. T. * (2016) N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis. Acta Crystallographica Section E Crystallographic Communications, 72 (7). pp. 1025-1031. ISSN 2056-9890 http://dx.doi.org/10.1107/S2056989016009968 doi:10.1107/S2056989016009968
spellingShingle QD Chemistry
Cardoso, Laura N. F.
Nogueira, Thais C. M.
Wardell, James L.
Wardell, Solange M. S. V.
Souza, Marcus V. N. de
Jotani, Mukesh M.
Tiekink, Edward R. T. *
N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis
title N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis
title_full N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis
title_fullStr N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis
title_full_unstemmed N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis
title_short N′-[(1E)-(5-Nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and Hirshfeld surface analysis
title_sort n′-[(1e)-(5-nitrofuran-2-yl)methylidene]thiophene-2-carbohydrazide: crystal structure and hirshfeld surface analysis
topic QD Chemistry
url http://eprints.sunway.edu.my/644/
http://eprints.sunway.edu.my/644/
http://eprints.sunway.edu.my/644/
http://eprints.sunway.edu.my/644/1/Acta%20E_RC%202016%2072%201025.pdf