Sub kGy photon irradiation alterations in graphite

Present work concerns polymer pencil-lead graphite (PPLG) and the potential use of these in elucidating irradiation-driven structural alterations. The study provides detailed analysis of radiation-induced structural interaction changes and the associated luminescence that originates from the energy...

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Main Authors: Bradley, D.A. *, Siti Nurasiah, M. N, Khandaker, Mayeen Uddin *, Almugren, K.S., Abdul Sani, S.F.
Format: Article
Language:English
Published: Elsevier 2020
Subjects:
Online Access:http://eprints.sunway.edu.my/1620/
http://eprints.sunway.edu.my/1620/1/Khandaker%20Sub%20KGy.pdf
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author Bradley, D.A. *
Siti Nurasiah, M. N
Khandaker, Mayeen Uddin *
Almugren, K.S.
Abdul Sani, S.F.
author_facet Bradley, D.A. *
Siti Nurasiah, M. N
Khandaker, Mayeen Uddin *
Almugren, K.S.
Abdul Sani, S.F.
author_sort Bradley, D.A. *
building SU Institutional Repository
collection Online Access
description Present work concerns polymer pencil-lead graphite (PPLG) and the potential use of these in elucidating irradiation-driven structural alterations. The study provides detailed analysis of radiation-induced structural interaction changes and the associated luminescence that originates from the energy absorption. Thermally stimulated emission from the different occupied defect energy levels reflects the received radiation dose, different for the different diameter PPLGs. The PPLG samples have been exposed to photon irradiation, specifically x-ray doses ranging from 1 to 10 Gy, extended to 30–200 Gy through use of a60Co gamma-ray source. Trapping parameters such as order of kinetics, activation energy and frequency factor are estimated using Chen's peak-shape method for a fixed-dose of 30 Gy. X-ray diffractometry was used to characterize the crystal structure of the PPLG, the aim being to identify the degree of structural order, atomic spacing and lattice constants of the various irradiated PPLG samples. The mean atomic spacing and degree of structural order for the different diameter PPLG are found to be 0.3332 nm and 26.6° respectively. Photoluminescence spectra from PPLG arising from diode laser excitation at 532 nm consist of two adjacent peaks, 602 nm (absorption) and 1074 nm (emission), with mean energy band gap values within the range 1.113–1.133 eV.
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spelling sunway-16202021-11-11T07:45:20Z http://eprints.sunway.edu.my/1620/ Sub kGy photon irradiation alterations in graphite Bradley, D.A. * Siti Nurasiah, M. N Khandaker, Mayeen Uddin * Almugren, K.S. Abdul Sani, S.F. R895-920 Medical Physics/Medical Radiology Present work concerns polymer pencil-lead graphite (PPLG) and the potential use of these in elucidating irradiation-driven structural alterations. The study provides detailed analysis of radiation-induced structural interaction changes and the associated luminescence that originates from the energy absorption. Thermally stimulated emission from the different occupied defect energy levels reflects the received radiation dose, different for the different diameter PPLGs. The PPLG samples have been exposed to photon irradiation, specifically x-ray doses ranging from 1 to 10 Gy, extended to 30–200 Gy through use of a60Co gamma-ray source. Trapping parameters such as order of kinetics, activation energy and frequency factor are estimated using Chen's peak-shape method for a fixed-dose of 30 Gy. X-ray diffractometry was used to characterize the crystal structure of the PPLG, the aim being to identify the degree of structural order, atomic spacing and lattice constants of the various irradiated PPLG samples. The mean atomic spacing and degree of structural order for the different diameter PPLG are found to be 0.3332 nm and 26.6° respectively. Photoluminescence spectra from PPLG arising from diode laser excitation at 532 nm consist of two adjacent peaks, 602 nm (absorption) and 1074 nm (emission), with mean energy band gap values within the range 1.113–1.133 eV. Elsevier 2020 Article PeerReviewed text en cc_by_nc_4 http://eprints.sunway.edu.my/1620/1/Khandaker%20Sub%20KGy.pdf Bradley, D.A. * and Siti Nurasiah, M. N and Khandaker, Mayeen Uddin * and Almugren, K.S. and Abdul Sani, S.F. (2020) Sub kGy photon irradiation alterations in graphite. Applied Radiation and Isotopes, 161. p. 109168. ISSN 0969-8043 http://doi.org/10.1016/j.apradiso.2020.109168 doi:10.1016/j.apradiso.2020.109168
spellingShingle R895-920 Medical Physics/Medical Radiology
Bradley, D.A. *
Siti Nurasiah, M. N
Khandaker, Mayeen Uddin *
Almugren, K.S.
Abdul Sani, S.F.
Sub kGy photon irradiation alterations in graphite
title Sub kGy photon irradiation alterations in graphite
title_full Sub kGy photon irradiation alterations in graphite
title_fullStr Sub kGy photon irradiation alterations in graphite
title_full_unstemmed Sub kGy photon irradiation alterations in graphite
title_short Sub kGy photon irradiation alterations in graphite
title_sort sub kgy photon irradiation alterations in graphite
topic R895-920 Medical Physics/Medical Radiology
url http://eprints.sunway.edu.my/1620/
http://eprints.sunway.edu.my/1620/
http://eprints.sunway.edu.my/1620/
http://eprints.sunway.edu.my/1620/1/Khandaker%20Sub%20KGy.pdf