Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation

In this work, the separation of carbon dioxide (CO2) from the methane (CH4) using fixed bed Pressure Swing Adsorption (PSA) column was modeled and simulated. The adsorption kinetics on the 13X zeolite adsorbent was described by Linear Driving Force (LDF) model. Simulation of adsorption phenomena ins...

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Main Authors: Awah Nouh, Salma, Lau, Kok Keong, Mohd Shariff, Azmi
Format: Citation Index Journal
Language:English
Published: David Publishing Company 2010
Subjects:
Online Access:http://scholars.utp.edu.my/id/eprint/2605/
http://scholars.utp.edu.my/id/eprint/2605/1/Kinetic_Adsorption_of_CO2_ProofRead.pdf
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author Awah Nouh, Salma
Lau, Kok Keong
Mohd Shariff, Azmi
author_facet Awah Nouh, Salma
Lau, Kok Keong
Mohd Shariff, Azmi
author_sort Awah Nouh, Salma
building UTP Institutional Repository
collection Online Access
description In this work, the separation of carbon dioxide (CO2) from the methane (CH4) using fixed bed Pressure Swing Adsorption (PSA) column was modeled and simulated. The adsorption kinetics on the 13X zeolite adsorbent was described by Linear Driving Force (LDF) model. Simulation of adsorption phenomena inside the fixed bed was implemented using Computational Fluid Dynamic (CFD) method, based on porous media concept, and the mass transfer coefficients for gas components (CO2 and CH4) were developed using User Defined Scalars (UDS). The model was validated by comparing with the experimental data, which were collected based on a varied set of laboratory conditions. The prediction of the adsorption isotherm (uptake curve) and methane recovery using the simulation results exhibited a reasonable agreement with the experimental data. Moreover, the effects of feed flow rate and bed concentration evolution were investigated. The current results suggested that CFD approach is capable to predicate the hydrodynamics and adsorption phenomena in the fixed bed adsorption column.
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format Citation Index Journal
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institution Universiti Teknologi Petronas
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spelling oai:scholars.utp.edu.my:26052023-04-11T04:30:16Z http://scholars.utp.edu.my/id/eprint/2605/ Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation Awah Nouh, Salma Lau, Kok Keong Mohd Shariff, Azmi TP Chemical technology In this work, the separation of carbon dioxide (CO2) from the methane (CH4) using fixed bed Pressure Swing Adsorption (PSA) column was modeled and simulated. The adsorption kinetics on the 13X zeolite adsorbent was described by Linear Driving Force (LDF) model. Simulation of adsorption phenomena inside the fixed bed was implemented using Computational Fluid Dynamic (CFD) method, based on porous media concept, and the mass transfer coefficients for gas components (CO2 and CH4) were developed using User Defined Scalars (UDS). The model was validated by comparing with the experimental data, which were collected based on a varied set of laboratory conditions. The prediction of the adsorption isotherm (uptake curve) and methane recovery using the simulation results exhibited a reasonable agreement with the experimental data. Moreover, the effects of feed flow rate and bed concentration evolution were investigated. The current results suggested that CFD approach is capable to predicate the hydrodynamics and adsorption phenomena in the fixed bed adsorption column. David Publishing Company 2010-07 Citation Index Journal NonPeerReviewed application/pdf en http://scholars.utp.edu.my/id/eprint/2605/1/Kinetic_Adsorption_of_CO2_ProofRead.pdf Awah Nouh, Salma and Lau, Kok Keong and Mohd Shariff, Azmi (2010) Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation. [Citation Index Journal] http://www.davidpublishing.com
spellingShingle TP Chemical technology
Awah Nouh, Salma
Lau, Kok Keong
Mohd Shariff, Azmi
Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation
title Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation
title_full Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation
title_fullStr Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation
title_full_unstemmed Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation
title_short Kinetic Adsorption of CO2/CH4 Mixture using 13X Zeolite: Modeling and Simulation
title_sort kinetic adsorption of co2/ch4 mixture using 13x zeolite: modeling and simulation
topic TP Chemical technology
url http://scholars.utp.edu.my/id/eprint/2605/
http://scholars.utp.edu.my/id/eprint/2605/
http://scholars.utp.edu.my/id/eprint/2605/1/Kinetic_Adsorption_of_CO2_ProofRead.pdf