Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution

The study was undertaken to compare from technical and economic point of view the treatment of antibiotic aqueous solution containing amoxicillin, ampicillin, and cloxacillin by Fenton, photo-Fenton, TiO2 photocatalytic and UV/ZnO processes. The best operating conditions for treatment of antibioti...

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Main Authors: Elmolla, E. S., Chaudhuri, M.
Format: Article
Language:English
Published: Elsevier 2010
Subjects:
Online Access:http://scholars.utp.edu.my/id/eprint/2286/
http://scholars.utp.edu.my/id/eprint/2286/1/Comparison_of_Different_Advancved_Oxidation_Procesees_for_Treatment_of_Antibiotic_Aqueous_Solution.pdf
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author Elmolla, E. S.
Chaudhuri, M.
author_facet Elmolla, E. S.
Chaudhuri, M.
author_sort Elmolla, E. S.
building UTP Institutional Repository
collection Online Access
description The study was undertaken to compare from technical and economic point of view the treatment of antibiotic aqueous solution containing amoxicillin, ampicillin, and cloxacillin by Fenton, photo-Fenton, TiO2 photocatalytic and UV/ZnO processes. The best operating conditions for treatment of antibiotic aqueous solution containing 104, 105 and 103 mg/L of amoxicillin, ampicillin, and cloxacillin, respectively were: Fenton process—COD/H2O2/Fe2+ molar ratio 1:3:0.30 and pH 3; photo-Fenton process — COD/H2O2/Fe2+ molar ratio 1:1.5:0.075 and pH 3; UV/ TiO2/H2O2 process — TiO2 1 g/L, ambient pH∼5 andH2O2 100 g/L; UV/ZnO process — ZnO 0.5 g/L and pH 11. All studied processeswere able to degrade the antibiotics and improve biodegradability (BOD5/CODratio), except for UV/ZnO process which did not improve biodegradability. Photo-Fenton process exhibited higher rate constant (0.029 min−1) than that of Fenton process (0.0144 min−1) and this may be ascribed to photochemical regeneration of Fe2+ ions by photoreduction of Fe3+ ions and hence increasing hydroxyl radical production rate. Rate constants of UV/ZnO process (0.00056 min−1) and UV/TiO2/H2O2 process (0.0005 min−1)were lower than that of Fenton and photo-Fenton processes. Photo-Fenton process appeared to be the most cost-effective compared to the other studied processes.
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spelling oai:scholars.utp.edu.my:22862017-01-19T08:24:40Z http://scholars.utp.edu.my/id/eprint/2286/ Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution Elmolla, E. S. Chaudhuri, M. TD Environmental technology. Sanitary engineering The study was undertaken to compare from technical and economic point of view the treatment of antibiotic aqueous solution containing amoxicillin, ampicillin, and cloxacillin by Fenton, photo-Fenton, TiO2 photocatalytic and UV/ZnO processes. The best operating conditions for treatment of antibiotic aqueous solution containing 104, 105 and 103 mg/L of amoxicillin, ampicillin, and cloxacillin, respectively were: Fenton process—COD/H2O2/Fe2+ molar ratio 1:3:0.30 and pH 3; photo-Fenton process — COD/H2O2/Fe2+ molar ratio 1:1.5:0.075 and pH 3; UV/ TiO2/H2O2 process — TiO2 1 g/L, ambient pH∼5 andH2O2 100 g/L; UV/ZnO process — ZnO 0.5 g/L and pH 11. All studied processeswere able to degrade the antibiotics and improve biodegradability (BOD5/CODratio), except for UV/ZnO process which did not improve biodegradability. Photo-Fenton process exhibited higher rate constant (0.029 min−1) than that of Fenton process (0.0144 min−1) and this may be ascribed to photochemical regeneration of Fe2+ ions by photoreduction of Fe3+ ions and hence increasing hydroxyl radical production rate. Rate constants of UV/ZnO process (0.00056 min−1) and UV/TiO2/H2O2 process (0.0005 min−1)were lower than that of Fenton and photo-Fenton processes. Photo-Fenton process appeared to be the most cost-effective compared to the other studied processes. Elsevier 2010 Article PeerReviewed application/pdf en http://scholars.utp.edu.my/id/eprint/2286/1/Comparison_of_Different_Advancved_Oxidation_Procesees_for_Treatment_of_Antibiotic_Aqueous_Solution.pdf Elmolla, E. S. and Chaudhuri, M. (2010) Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution. Desalination, 256 (1-3). pp. 43-47. ISSN 0011-9164
spellingShingle TD Environmental technology. Sanitary engineering
Elmolla, E. S.
Chaudhuri, M.
Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution
title Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution
title_full Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution
title_fullStr Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution
title_full_unstemmed Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution
title_short Comparison of Different Advanced Oxidation Processes for Treatment of Antibiotic Aqueous Solution
title_sort comparison of different advanced oxidation processes for treatment of antibiotic aqueous solution
topic TD Environmental technology. Sanitary engineering
url http://scholars.utp.edu.my/id/eprint/2286/
http://scholars.utp.edu.my/id/eprint/2286/1/Comparison_of_Different_Advancved_Oxidation_Procesees_for_Treatment_of_Antibiotic_Aqueous_Solution.pdf