Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources

The use of different vanadium sources in the synthesis of multi-metal MoVTeNb oxide catalysts has been investigated for their effect on the physicochemical properties of catalysts. Metal oxides were synthesized by slurry method assisted with a microwave irradiation. Vanadium pentoxide (V2O5), vanady...

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Main Authors: Haslinda Mohd Sidek, Irmawati Ramli, Norhazlin Zainuddin, Ahangar, Hossein Abbastabar, Taufiq-Yap Yun Hin
Format: Article
Language:English
Published: Penerbit Universiti Kebangsaan Malaysia 2021
Online Access:http://journalarticle.ukm.my/17594/
http://journalarticle.ukm.my/17594/1/21.pdf
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author Haslinda Mohd Sidek,
Irmawati Ramli,
Norhazlin Zainuddin,
Ahangar, Hossein Abbastabar
Taufiq-Yap Yun Hin,
author_facet Haslinda Mohd Sidek,
Irmawati Ramli,
Norhazlin Zainuddin,
Ahangar, Hossein Abbastabar
Taufiq-Yap Yun Hin,
author_sort Haslinda Mohd Sidek,
building UKM Institutional Repository
collection Online Access
description The use of different vanadium sources in the synthesis of multi-metal MoVTeNb oxide catalysts has been investigated for their effect on the physicochemical properties of catalysts. Metal oxides were synthesized by slurry method assisted with a microwave irradiation. Vanadium pentoxide (V2O5), vanadyl sulphate (VOSO4) and ammonium metavanadate (NH4VO3) were used as the vanadium sources, respectively. X-ray diffraction (XRD) pattern showed the existence of orthorhombic (M1) phases in all catalysts. The catalyst prepared using V2O5 produced the highest formation of the phase. This was further supported by Inductive Couple Plasma-Atomic Emission Spectroscopy (ICP-AES), which showed that the V2O5 catalyst has the highest V: Mo ratio, mainly responsible for the high catalytic activity. Temperature Programmed Reduction in Hydrogen (H2-TPR) showed better reducibility for the catalyst when compared to the others. Temperature Programmed Reaction (TPRn) confirmed that the oxidants active for propane conversion into acrylic acid were originated from the lattice of the catalyst.
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spelling oai:generic.eprints.org:175942021-11-19T02:10:50Z http://journalarticle.ukm.my/17594/ Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources Haslinda Mohd Sidek, Irmawati Ramli, Norhazlin Zainuddin, Ahangar, Hossein Abbastabar Taufiq-Yap Yun Hin, The use of different vanadium sources in the synthesis of multi-metal MoVTeNb oxide catalysts has been investigated for their effect on the physicochemical properties of catalysts. Metal oxides were synthesized by slurry method assisted with a microwave irradiation. Vanadium pentoxide (V2O5), vanadyl sulphate (VOSO4) and ammonium metavanadate (NH4VO3) were used as the vanadium sources, respectively. X-ray diffraction (XRD) pattern showed the existence of orthorhombic (M1) phases in all catalysts. The catalyst prepared using V2O5 produced the highest formation of the phase. This was further supported by Inductive Couple Plasma-Atomic Emission Spectroscopy (ICP-AES), which showed that the V2O5 catalyst has the highest V: Mo ratio, mainly responsible for the high catalytic activity. Temperature Programmed Reduction in Hydrogen (H2-TPR) showed better reducibility for the catalyst when compared to the others. Temperature Programmed Reaction (TPRn) confirmed that the oxidants active for propane conversion into acrylic acid were originated from the lattice of the catalyst. Penerbit Universiti Kebangsaan Malaysia 2021-08 Article PeerReviewed application/pdf en http://journalarticle.ukm.my/17594/1/21.pdf Haslinda Mohd Sidek, and Irmawati Ramli, and Norhazlin Zainuddin, and Ahangar, Hossein Abbastabar and Taufiq-Yap Yun Hin, (2021) Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources. Sains Malaysiana, 50 (8). pp. 2395-2405. ISSN 0126-6039 https://www.ukm.my/jsm/malay_journals/jilid50bil8_2021/KandunganJilid50Bil8_2021.html
spellingShingle Haslinda Mohd Sidek,
Irmawati Ramli,
Norhazlin Zainuddin,
Ahangar, Hossein Abbastabar
Taufiq-Yap Yun Hin,
Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources
title Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources
title_full Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources
title_fullStr Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources
title_full_unstemmed Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources
title_short Physicochemical properties of MoVTeNb mixed oxide catalysts synthesized using different vanadium sources
title_sort physicochemical properties of movtenb mixed oxide catalysts synthesized using different vanadium sources
url http://journalarticle.ukm.my/17594/
http://journalarticle.ukm.my/17594/
http://journalarticle.ukm.my/17594/1/21.pdf