Metal-organic frameworks for gas storage applications
The work presented herein focuses on the continuous synthesis of metal-organic frameworks HKUST-1 and UTSA-16 using a nozzle reactor and Swirl reactor. Optimisations for both metal-organic frameworks were achieved at ambient conditions of 25 oC, 1 bar at lab-scale. Both optimisations were then succe...
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| Format: | Thesis (University of Nottingham only) |
| Language: | English |
| Published: |
2024
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| Online Access: | https://eprints.nottingham.ac.uk/76978/ |
| _version_ | 1848800952619892736 |
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| author | Priest, Scott |
| author_facet | Priest, Scott |
| author_sort | Priest, Scott |
| building | Nottingham Research Data Repository |
| collection | Online Access |
| description | The work presented herein focuses on the continuous synthesis of metal-organic frameworks HKUST-1 and UTSA-16 using a nozzle reactor and Swirl reactor. Optimisations for both metal-organic frameworks were achieved at ambient conditions of 25 oC, 1 bar at lab-scale. Both optimisations were then successfully scaled-up using an industrial continuous flow reactor, the Pilot+ nozzle reactor, followed by the Swirl reactor at Promethean Particles at 1 kg scale, each with high yields of 93.0 and 95.2 % and CO2 uptake performances of 20.1 wt. % and 12.8 wt. % for HKUST-1 and UTSA-16, respectively. |
| first_indexed | 2025-11-14T20:59:44Z |
| format | Thesis (University of Nottingham only) |
| id | nottingham-76978 |
| institution | University of Nottingham Malaysia Campus |
| institution_category | Local University |
| language | English |
| last_indexed | 2025-11-14T20:59:44Z |
| publishDate | 2024 |
| recordtype | eprints |
| repository_type | Digital Repository |
| spelling | nottingham-769782025-02-28T15:19:36Z https://eprints.nottingham.ac.uk/76978/ Metal-organic frameworks for gas storage applications Priest, Scott The work presented herein focuses on the continuous synthesis of metal-organic frameworks HKUST-1 and UTSA-16 using a nozzle reactor and Swirl reactor. Optimisations for both metal-organic frameworks were achieved at ambient conditions of 25 oC, 1 bar at lab-scale. Both optimisations were then successfully scaled-up using an industrial continuous flow reactor, the Pilot+ nozzle reactor, followed by the Swirl reactor at Promethean Particles at 1 kg scale, each with high yields of 93.0 and 95.2 % and CO2 uptake performances of 20.1 wt. % and 12.8 wt. % for HKUST-1 and UTSA-16, respectively. 2024-07-18 Thesis (University of Nottingham only) NonPeerReviewed application/pdf en cc_by https://eprints.nottingham.ac.uk/76978/1/Scott%20Priest%20-%2014341912%20-%20EngD%20Thesis%20Corrected%20Version%20Final.pdf Priest, Scott (2024) Metal-organic frameworks for gas storage applications. EngD thesis, University of Nottingham. MOFs CCS |
| spellingShingle | MOFs CCS Priest, Scott Metal-organic frameworks for gas storage applications |
| title | Metal-organic frameworks for gas storage applications |
| title_full | Metal-organic frameworks for gas storage applications |
| title_fullStr | Metal-organic frameworks for gas storage applications |
| title_full_unstemmed | Metal-organic frameworks for gas storage applications |
| title_short | Metal-organic frameworks for gas storage applications |
| title_sort | metal-organic frameworks for gas storage applications |
| topic | MOFs CCS |
| url | https://eprints.nottingham.ac.uk/76978/ |