Catalytic reductions and synthesis applications of organic azides

Known for over a century, organic azides are compounds of significant interest. Organic azides are potentially very useful compounds – they can be considered to function as ‘protected’ amines. In spite of certain hazards associated with these compounds, research into the chemistry of azides remains...

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Main Author: Scrafield, Benjamin Luke
Format: Thesis (University of Nottingham only)
Language:English
Published: 2022
Subjects:
Online Access:https://eprints.nottingham.ac.uk/69823/
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author Scrafield, Benjamin Luke
author_facet Scrafield, Benjamin Luke
author_sort Scrafield, Benjamin Luke
building Nottingham Research Data Repository
collection Online Access
description Known for over a century, organic azides are compounds of significant interest. Organic azides are potentially very useful compounds – they can be considered to function as ‘protected’ amines. In spite of certain hazards associated with these compounds, research into the chemistry of azides remains active. Chapter 1 of this thesis provides an overview of this considerable body of research in terms of the properties of organic azides, methods for their preparation, and aspects of their reactivity. The primary aim of this project was to examine the scope and utility of a catalytic azide reduction. Previous catalytic methods display certain practical limitations, which are overcome by the new system. As discussed in Chapter 2, this work included preparing a variety of azides and examining their reactivity in the catalytic azide reduction. This chemistry was then extended to include post-reduction transformations. Chapter 3 details our attempts to apply this method in the preparation of small molecule targets of interest.
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spelling nottingham-698232023-11-15T15:51:06Z https://eprints.nottingham.ac.uk/69823/ Catalytic reductions and synthesis applications of organic azides Scrafield, Benjamin Luke Known for over a century, organic azides are compounds of significant interest. Organic azides are potentially very useful compounds – they can be considered to function as ‘protected’ amines. In spite of certain hazards associated with these compounds, research into the chemistry of azides remains active. Chapter 1 of this thesis provides an overview of this considerable body of research in terms of the properties of organic azides, methods for their preparation, and aspects of their reactivity. The primary aim of this project was to examine the scope and utility of a catalytic azide reduction. Previous catalytic methods display certain practical limitations, which are overcome by the new system. As discussed in Chapter 2, this work included preparing a variety of azides and examining their reactivity in the catalytic azide reduction. This chemistry was then extended to include post-reduction transformations. Chapter 3 details our attempts to apply this method in the preparation of small molecule targets of interest. 2022-12-31 Thesis (University of Nottingham only) NonPeerReviewed application/pdf en cc_by https://eprints.nottingham.ac.uk/69823/1/Thesis%20-%20BLS%20%28corrected%29.pdf Scrafield, Benjamin Luke (2022) Catalytic reductions and synthesis applications of organic azides. PhD thesis, University of Nottingham. Catalytic reductions Organic azides
spellingShingle Catalytic reductions
Organic azides
Scrafield, Benjamin Luke
Catalytic reductions and synthesis applications of organic azides
title Catalytic reductions and synthesis applications of organic azides
title_full Catalytic reductions and synthesis applications of organic azides
title_fullStr Catalytic reductions and synthesis applications of organic azides
title_full_unstemmed Catalytic reductions and synthesis applications of organic azides
title_short Catalytic reductions and synthesis applications of organic azides
title_sort catalytic reductions and synthesis applications of organic azides
topic Catalytic reductions
Organic azides
url https://eprints.nottingham.ac.uk/69823/