Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase

This thesis is comprised of two sections; The first is a semi synthesis of the cytotoxic natural product jerantinine A. Starting from the natural product tabersonine, isolated from Voacanga africana, which contains the 3 stereocenters present in jerantinine alkaloids set in the correct conformation....

Full description

Bibliographic Details
Main Author: Eastman, H
Format: Thesis (University of Nottingham only)
Language:English
Published: 2020
Subjects:
Online Access:https://eprints.nottingham.ac.uk/63797/
_version_ 1848800058048249856
author Eastman, H
author_facet Eastman, H
author_sort Eastman, H
building Nottingham Research Data Repository
collection Online Access
description This thesis is comprised of two sections; The first is a semi synthesis of the cytotoxic natural product jerantinine A. Starting from the natural product tabersonine, isolated from Voacanga africana, which contains the 3 stereocenters present in jerantinine alkaloids set in the correct conformation. The reaction conditions were optimised and produced jerantinine A from tabersonine in a 16% yield over 7 steps. Following this, the biological activity was evaluated using MCF-7 Cancer cell lines, a clonogenic assay, cell cycle analysis and a tubulin polymerisation assay. These results concluded that jerantinine A was a tubulin destabilising agent and were visualised using confocal microscopy. The second section is using alcohol dehydrogenases in the formation of disubstituted tetrahydropyrans. The biocatalytic strategy of the synthesis of 2-6, disubstituted tetrahydropyrans was achieved using an alcohol dehydrogenase triggered intramolecular oxa-Michael reaction from prochiral ketoenone starting materials. These were produced in good yields with up to >99% e.e. and 12:1 d.r.. This methodology was then used in the synthesis of an analogue of the natural product brocaketone A in a 26% yield over the synthesis. 2,5-Disubstituted tetrahydrofurans were also produced using this methodology but were produced in poor d.r
first_indexed 2025-11-14T20:45:31Z
format Thesis (University of Nottingham only)
id nottingham-63797
institution University of Nottingham Malaysia Campus
institution_category Local University
language English
last_indexed 2025-11-14T20:45:31Z
publishDate 2020
recordtype eprints
repository_type Digital Repository
spelling nottingham-637972025-02-28T15:07:06Z https://eprints.nottingham.ac.uk/63797/ Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase Eastman, H This thesis is comprised of two sections; The first is a semi synthesis of the cytotoxic natural product jerantinine A. Starting from the natural product tabersonine, isolated from Voacanga africana, which contains the 3 stereocenters present in jerantinine alkaloids set in the correct conformation. The reaction conditions were optimised and produced jerantinine A from tabersonine in a 16% yield over 7 steps. Following this, the biological activity was evaluated using MCF-7 Cancer cell lines, a clonogenic assay, cell cycle analysis and a tubulin polymerisation assay. These results concluded that jerantinine A was a tubulin destabilising agent and were visualised using confocal microscopy. The second section is using alcohol dehydrogenases in the formation of disubstituted tetrahydropyrans. The biocatalytic strategy of the synthesis of 2-6, disubstituted tetrahydropyrans was achieved using an alcohol dehydrogenase triggered intramolecular oxa-Michael reaction from prochiral ketoenone starting materials. These were produced in good yields with up to >99% e.e. and 12:1 d.r.. This methodology was then used in the synthesis of an analogue of the natural product brocaketone A in a 26% yield over the synthesis. 2,5-Disubstituted tetrahydrofurans were also produced using this methodology but were produced in poor d.r 2020-12-31 Thesis (University of Nottingham only) NonPeerReviewed application/pdf en arr https://eprints.nottingham.ac.uk/63797/1/Final%20Thesis%20Harry%20Eastman%283%29.pdf Eastman, H (2020) Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase. PhD thesis, University of Nottingham. Chemistry Jerantinine alkaloids Synthesis Biocatalytic
spellingShingle Chemistry
Jerantinine alkaloids
Synthesis
Biocatalytic
Eastman, H
Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase
title Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase
title_full Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase
title_fullStr Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase
title_full_unstemmed Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase
title_short Total Synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - Disubstituted tetrahydropyrans using an alcohol dehydrogenase
title_sort total synthesis of jerantinine alkaloids and a biocatalytic synthesis of 2,6 - disubstituted tetrahydropyrans using an alcohol dehydrogenase
topic Chemistry
Jerantinine alkaloids
Synthesis
Biocatalytic
url https://eprints.nottingham.ac.uk/63797/