Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions

In an effort to reduce the overall energy penalty and capital expenditure associated with carbon capture technologies, a variety of porous solid adsorbents have been developed. The limitations of solid sorbent in large-scale process are related to its CO2 uptake, physicochemical stability, lifecycle...

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Main Authors: Meng, Yang, Yan, Yuxin, Jiang, Peng, Wu, Xinyun, Sun, Cheng-gong, Wu, Tao, Pang, Cheng Heng
Format: Article
Language:English
Published: EDP Sciences 2020
Online Access:https://eprints.nottingham.ac.uk/60579/
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author Meng, Yang
Yan, Yuxin
Jiang, Peng
Wu, Xinyun
Sun, Cheng-gong
Wu, Tao
Pang, Cheng Heng
author_facet Meng, Yang
Yan, Yuxin
Jiang, Peng
Wu, Xinyun
Sun, Cheng-gong
Wu, Tao
Pang, Cheng Heng
author_sort Meng, Yang
building Nottingham Research Data Repository
collection Online Access
description In an effort to reduce the overall energy penalty and capital expenditure associated with carbon capture technologies, a variety of porous solid adsorbents have been developed. The limitations of solid sorbent in large-scale process are related to its CO2 uptake, physicochemical stability, lifecycle, regenerability and operation condition. In this paper, siliceous foam materials were synthesized via a modified microemulsion templating method and functionalized with branched polyethylenimine (PEI). The physical characteristics of synthesized silica adsorbents under different aging conditions were analysed via N2 sorption analysis and Scanned Electron Microscopy (SEM) morphological analysis. CO2 uptake was evaluated by thermogravimetric analyser (TGA). The results show that CO2 uptake is desirable even under low CO2 partial pressure and is predictable with multiple linear regression (MLR) model in the range of examined materials.
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spelling nottingham-605792020-05-12T00:51:52Z https://eprints.nottingham.ac.uk/60579/ Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions Meng, Yang Yan, Yuxin Jiang, Peng Wu, Xinyun Sun, Cheng-gong Wu, Tao Pang, Cheng Heng In an effort to reduce the overall energy penalty and capital expenditure associated with carbon capture technologies, a variety of porous solid adsorbents have been developed. The limitations of solid sorbent in large-scale process are related to its CO2 uptake, physicochemical stability, lifecycle, regenerability and operation condition. In this paper, siliceous foam materials were synthesized via a modified microemulsion templating method and functionalized with branched polyethylenimine (PEI). The physical characteristics of synthesized silica adsorbents under different aging conditions were analysed via N2 sorption analysis and Scanned Electron Microscopy (SEM) morphological analysis. CO2 uptake was evaluated by thermogravimetric analyser (TGA). The results show that CO2 uptake is desirable even under low CO2 partial pressure and is predictable with multiple linear regression (MLR) model in the range of examined materials. EDP Sciences 2020-03-23 Article PeerReviewed application/pdf en cc_by https://eprints.nottingham.ac.uk/60579/1/Siliceous%20foam%20material%20and%20its%20application%20in%20post-combustion%20carbon%20capture%20for%20NGCC%20plants%20Effects%20of%20aging%20conditions.pdf Meng, Yang, Yan, Yuxin, Jiang, Peng, Wu, Xinyun, Sun, Cheng-gong, Wu, Tao and Pang, Cheng Heng (2020) Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions. E3S Web of Conferences, 158 . 03004. ISSN 2267-1242 http://dx.doi.org/10.1051/e3sconf/202015803004 doi:10.1051/e3sconf/202015803004 doi:10.1051/e3sconf/202015803004
spellingShingle Meng, Yang
Yan, Yuxin
Jiang, Peng
Wu, Xinyun
Sun, Cheng-gong
Wu, Tao
Pang, Cheng Heng
Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions
title Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions
title_full Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions
title_fullStr Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions
title_full_unstemmed Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions
title_short Siliceous foam material and its application in post-combustion carbon capture for NGCC plants: effects of aging conditions
title_sort siliceous foam material and its application in post-combustion carbon capture for ngcc plants: effects of aging conditions
url https://eprints.nottingham.ac.uk/60579/
https://eprints.nottingham.ac.uk/60579/
https://eprints.nottingham.ac.uk/60579/