Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process

The indirect steam gasification of biomass to olefins (IDBTO) coupled with CO2 utilization was proposed and simulated. Energy and exergy efficiencies, net CO2 emissions, and economic evaluation were performed against IDBTO as well as the direct oxygen-steam gasification of biomass to olifins (DBTO)....

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Main Authors: Jiang, Peng, Parvez, Ashak Mahmud, Meng, Yang, Xu, Meng-xia, Shui, Tian-chi, Sun, Cheng-gong, Wu, Tao
Format: Article
Language:English
Published: 2019
Subjects:
Online Access:https://eprints.nottingham.ac.uk/59003/
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author Jiang, Peng
Parvez, Ashak Mahmud
Meng, Yang
Xu, Meng-xia
Shui, Tian-chi
Sun, Cheng-gong
Wu, Tao
author_facet Jiang, Peng
Parvez, Ashak Mahmud
Meng, Yang
Xu, Meng-xia
Shui, Tian-chi
Sun, Cheng-gong
Wu, Tao
author_sort Jiang, Peng
building Nottingham Research Data Repository
collection Online Access
description The indirect steam gasification of biomass to olefins (IDBTO) coupled with CO2 utilization was proposed and simulated. Energy and exergy efficiencies, net CO2 emissions, and economic evaluation were performed against IDBTO as well as the direct oxygen-steam gasification of biomass to olifins (DBTO). The influences of unreacted gas recycling fraction (RU) and CO2 to dry biomass mass ratio (CO2/B) on the thermodynamic performance of the processes were also studied. The results showed that the yields of olefins of DBTO and IDBTO were 17 wt% and 19 wt%, respectively, the overall energy and exergy efficiencies of the IDBTO were around 49% and 44%, which were 8% and 7% higher than those of the DBTO process, respectively. A higher RU was found favor higher energy and exergy efficiencies for both routes. Besides, for the IDBTO process, it is found that the addition of CO2 to gasification system led to an improvement in both energy efficiency and exergy efficiency by around 1.6%. Moreover, life-cycle net CO2 emission was predicted to be -4.4 kg CO2 eq./ kg olefins for IDBTO, while for DBTO, it was -8.7 kg CO2 eq./ kg. However, the quantitative economic performance of IDBTO was superior to that of the DBTO process.
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spelling nottingham-590032019-09-18T00:57:49Z https://eprints.nottingham.ac.uk/59003/ Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process Jiang, Peng Parvez, Ashak Mahmud Meng, Yang Xu, Meng-xia Shui, Tian-chi Sun, Cheng-gong Wu, Tao The indirect steam gasification of biomass to olefins (IDBTO) coupled with CO2 utilization was proposed and simulated. Energy and exergy efficiencies, net CO2 emissions, and economic evaluation were performed against IDBTO as well as the direct oxygen-steam gasification of biomass to olifins (DBTO). The influences of unreacted gas recycling fraction (RU) and CO2 to dry biomass mass ratio (CO2/B) on the thermodynamic performance of the processes were also studied. The results showed that the yields of olefins of DBTO and IDBTO were 17 wt% and 19 wt%, respectively, the overall energy and exergy efficiencies of the IDBTO were around 49% and 44%, which were 8% and 7% higher than those of the DBTO process, respectively. A higher RU was found favor higher energy and exergy efficiencies for both routes. Besides, for the IDBTO process, it is found that the addition of CO2 to gasification system led to an improvement in both energy efficiency and exergy efficiency by around 1.6%. Moreover, life-cycle net CO2 emission was predicted to be -4.4 kg CO2 eq./ kg olefins for IDBTO, while for DBTO, it was -8.7 kg CO2 eq./ kg. However, the quantitative economic performance of IDBTO was superior to that of the DBTO process. 2019-11-15 Article PeerReviewed application/pdf en cc_by https://eprints.nottingham.ac.uk/59003/1/combinepdf.pdf Jiang, Peng, Parvez, Ashak Mahmud, Meng, Yang, Xu, Meng-xia, Shui, Tian-chi, Sun, Cheng-gong and Wu, Tao (2019) Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process. Energy, 187 . p. 115933. ISSN 03605442 Bio-olefin; Thermodynamic analysis; Environmental assessment; CO2 utilization; Negative net CO2 emission; Techno-economic analysis http://dx.doi.org/10.1016/j.energy.2019.115933 doi:10.1016/j.energy.2019.115933 doi:10.1016/j.energy.2019.115933
spellingShingle Bio-olefin; Thermodynamic analysis; Environmental assessment; CO2 utilization; Negative net CO2 emission; Techno-economic analysis
Jiang, Peng
Parvez, Ashak Mahmud
Meng, Yang
Xu, Meng-xia
Shui, Tian-chi
Sun, Cheng-gong
Wu, Tao
Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process
title Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process
title_full Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process
title_fullStr Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process
title_full_unstemmed Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process
title_short Exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process
title_sort exergetic, economic and carbon emission studies of bio-olefin production via indirect steam gasification process
topic Bio-olefin; Thermodynamic analysis; Environmental assessment; CO2 utilization; Negative net CO2 emission; Techno-economic analysis
url https://eprints.nottingham.ac.uk/59003/
https://eprints.nottingham.ac.uk/59003/
https://eprints.nottingham.ac.uk/59003/