N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis

This thesis details aims at forming low-coordinate metal complexes, stabilised by N-based ligands, with significant focus on carbazole based systems. The sysnthesis of ligands containing these moieties is first targeted, giving a detailed explanation of how differing synthetic pathways that allow mo...

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Main Author: Nolla Saltiel, Roberto
Format: Thesis (University of Nottingham only)
Language:English
Published: 2019
Subjects:
Online Access:https://eprints.nottingham.ac.uk/56541/
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author Nolla Saltiel, Roberto
author_facet Nolla Saltiel, Roberto
author_sort Nolla Saltiel, Roberto
building Nottingham Research Data Repository
collection Online Access
description This thesis details aims at forming low-coordinate metal complexes, stabilised by N-based ligands, with significant focus on carbazole based systems. The sysnthesis of ligands containing these moieties is first targeted, giving a detailed explanation of how differing synthetic pathways that allow modifications to the central carbazole core, in turn allow the formation of stable low-coordinate metal centres. Stabilised metal centres derived from these studies, have been found useful in the dehydrogenation of dimethylamine-borane adducts. While also suitable in the selective anti-Markovnikov hydrophosphination of activated alkenes.
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format Thesis (University of Nottingham only)
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institution University of Nottingham Malaysia Campus
institution_category Local University
language English
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publishDate 2019
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spelling nottingham-565412025-02-28T14:29:28Z https://eprints.nottingham.ac.uk/56541/ N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis Nolla Saltiel, Roberto This thesis details aims at forming low-coordinate metal complexes, stabilised by N-based ligands, with significant focus on carbazole based systems. The sysnthesis of ligands containing these moieties is first targeted, giving a detailed explanation of how differing synthetic pathways that allow modifications to the central carbazole core, in turn allow the formation of stable low-coordinate metal centres. Stabilised metal centres derived from these studies, have been found useful in the dehydrogenation of dimethylamine-borane adducts. While also suitable in the selective anti-Markovnikov hydrophosphination of activated alkenes. 2019-07-17 Thesis (University of Nottingham only) NonPeerReviewed application/pdf en arr https://eprints.nottingham.ac.uk/56541/1/PhD%20Thesis%20Roberto%20Nolla%20Saltiel.pdf Nolla Saltiel, Roberto (2019) N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis. PhD thesis, University of Nottingham. ligands carbazoles alkali metal complexes
spellingShingle ligands
carbazoles
alkali metal complexes
Nolla Saltiel, Roberto
N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis
title N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis
title_full N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis
title_fullStr N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis
title_full_unstemmed N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis
title_short N/P-based Sterically Demanding Ligands: Synthesis, Reactivity and Catalysis
title_sort n/p-based sterically demanding ligands: synthesis, reactivity and catalysis
topic ligands
carbazoles
alkali metal complexes
url https://eprints.nottingham.ac.uk/56541/