Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations

The “smart” amine donors o‐xylylenediamine and cadaverine were employed for the rapid screening of a large ketone library and subsequent preparative‐scale synthesis of selected compounds using a commercially available amine transaminase, ATA256. The methodology enables both screening and preparative...

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Main Authors: Gomm, Andrew, Grigoriou, Stylianos, Peel, Christopher, Ryan, James, Mujtaba, Nafees, Clarke, Thomas, Kulcinskaja, Evelina, O'Reilly, Elaine
Format: Article
Language:English
Published: Wiley 2018
Online Access:https://eprints.nottingham.ac.uk/53766/
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author Gomm, Andrew
Grigoriou, Stylianos
Peel, Christopher
Ryan, James
Mujtaba, Nafees
Clarke, Thomas
Kulcinskaja, Evelina
O'Reilly, Elaine
author_facet Gomm, Andrew
Grigoriou, Stylianos
Peel, Christopher
Ryan, James
Mujtaba, Nafees
Clarke, Thomas
Kulcinskaja, Evelina
O'Reilly, Elaine
author_sort Gomm, Andrew
building Nottingham Research Data Repository
collection Online Access
description The “smart” amine donors o‐xylylenediamine and cadaverine were employed for the rapid screening of a large ketone library and subsequent preparative‐scale synthesis of selected compounds using a commercially available amine transaminase, ATA256. The methodology enables both screening and preparative‐scale biotransformations to be performed with a single enzyme and simplifies the generation of sp3‐rich small‐molecule libraries.
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spelling nottingham-537662019-07-06T04:30:18Z https://eprints.nottingham.ac.uk/53766/ Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations Gomm, Andrew Grigoriou, Stylianos Peel, Christopher Ryan, James Mujtaba, Nafees Clarke, Thomas Kulcinskaja, Evelina O'Reilly, Elaine The “smart” amine donors o‐xylylenediamine and cadaverine were employed for the rapid screening of a large ketone library and subsequent preparative‐scale synthesis of selected compounds using a commercially available amine transaminase, ATA256. The methodology enables both screening and preparative‐scale biotransformations to be performed with a single enzyme and simplifies the generation of sp3‐rich small‐molecule libraries. Wiley 2018-07-06 Article PeerReviewed application/pdf en https://eprints.nottingham.ac.uk/53766/1/Smart%20anime%20donors.pdf Gomm, Andrew, Grigoriou, Stylianos, Peel, Christopher, Ryan, James, Mujtaba, Nafees, Clarke, Thomas, Kulcinskaja, Evelina and O'Reilly, Elaine (2018) Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations. European Journal of Organic Chemistry . ISSN 1099-0690 https://onlinelibrary.wiley.com/doi/abs/10.1002/ejoc.201800799 doi:10.1002/ejoc.201800799 doi:10.1002/ejoc.201800799
spellingShingle Gomm, Andrew
Grigoriou, Stylianos
Peel, Christopher
Ryan, James
Mujtaba, Nafees
Clarke, Thomas
Kulcinskaja, Evelina
O'Reilly, Elaine
Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations
title Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations
title_full Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations
title_fullStr Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations
title_full_unstemmed Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations
title_short Application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations
title_sort application of “smart” amine donors for rapid screening and scale-up of transaminase-mediated biotransformations
url https://eprints.nottingham.ac.uk/53766/
https://eprints.nottingham.ac.uk/53766/
https://eprints.nottingham.ac.uk/53766/