A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites

A versatile Rotary Chemical Vapour Deposition (RCVD) technique for the in-situ synthesis of large scale carbon-coated non-magnetic metal oxide nanoparticles (NPs) is presented, and a controllable coating thickness varying between 1–5 nm has been achieved. The technique has significantly up-scaled th...

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Main Authors: Wang, Nannan, Yang, Zhuxian, Xu, Fang, Thummavichai, Kunyapat, Chen, Hongmei, Xia, Yongde, Zhu, Yanqiu
Format: Article
Published: Nature Publishing Group 2017
Online Access:https://eprints.nottingham.ac.uk/52569/
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author Wang, Nannan
Yang, Zhuxian
Xu, Fang
Thummavichai, Kunyapat
Chen, Hongmei
Xia, Yongde
Zhu, Yanqiu
author_facet Wang, Nannan
Yang, Zhuxian
Xu, Fang
Thummavichai, Kunyapat
Chen, Hongmei
Xia, Yongde
Zhu, Yanqiu
author_sort Wang, Nannan
building Nottingham Research Data Repository
collection Online Access
description A versatile Rotary Chemical Vapour Deposition (RCVD) technique for the in-situ synthesis of large scale carbon-coated non-magnetic metal oxide nanoparticles (NPs) is presented, and a controllable coating thickness varying between 1–5 nm has been achieved. The technique has significantly up-scaled the traditional chemical vapour deposition (CVD) production for NPs from mg level to 10 s of grams per batch, with the potential for continuous manufacturing. The resulting smooth and uniform C-coatings sheathing the inner core metal oxide NPs are made of well-crystallised graphitic layers, as confirmed by electron microscopy imaging, electron dispersive spectrum elemental line scan, X-ray powder diffractions and Raman spectroscopy. Using nylon 12 as an example matrix, we further demonstrate that the inclusion of C-coated composite NPs into the matrix improves the thermal conductivity, from 0.205 W∙m−1∙K−1 for neat nylon 12 to 0.305 W∙m−1∙K−1 for a 4 wt% C-coated ZnO composite, in addition to a 27% improvement in tensile strength at 2 wt% addition.
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spelling nottingham-525692020-05-04T19:07:24Z https://eprints.nottingham.ac.uk/52569/ A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites Wang, Nannan Yang, Zhuxian Xu, Fang Thummavichai, Kunyapat Chen, Hongmei Xia, Yongde Zhu, Yanqiu A versatile Rotary Chemical Vapour Deposition (RCVD) technique for the in-situ synthesis of large scale carbon-coated non-magnetic metal oxide nanoparticles (NPs) is presented, and a controllable coating thickness varying between 1–5 nm has been achieved. The technique has significantly up-scaled the traditional chemical vapour deposition (CVD) production for NPs from mg level to 10 s of grams per batch, with the potential for continuous manufacturing. The resulting smooth and uniform C-coatings sheathing the inner core metal oxide NPs are made of well-crystallised graphitic layers, as confirmed by electron microscopy imaging, electron dispersive spectrum elemental line scan, X-ray powder diffractions and Raman spectroscopy. Using nylon 12 as an example matrix, we further demonstrate that the inclusion of C-coated composite NPs into the matrix improves the thermal conductivity, from 0.205 W∙m−1∙K−1 for neat nylon 12 to 0.305 W∙m−1∙K−1 for a 4 wt% C-coated ZnO composite, in addition to a 27% improvement in tensile strength at 2 wt% addition. Nature Publishing Group 2017-09-19 Article PeerReviewed Wang, Nannan, Yang, Zhuxian, Xu, Fang, Thummavichai, Kunyapat, Chen, Hongmei, Xia, Yongde and Zhu, Yanqiu (2017) A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites. Scientific Reports, 7 (1). 11829/1-11829/9. ISSN 2045-2322 https://www.nature.com/articles/s41598-017-12200-1 doi:10.1038/s41598-017-12200-1 doi:10.1038/s41598-017-12200-1
spellingShingle Wang, Nannan
Yang, Zhuxian
Xu, Fang
Thummavichai, Kunyapat
Chen, Hongmei
Xia, Yongde
Zhu, Yanqiu
A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites
title A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites
title_full A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites
title_fullStr A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites
title_full_unstemmed A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites
title_short A generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites
title_sort generic method to synthesise graphitic carbon coated nanoparticles in large scale and their derivative polymer nanocomposites
url https://eprints.nottingham.ac.uk/52569/
https://eprints.nottingham.ac.uk/52569/
https://eprints.nottingham.ac.uk/52569/