High-throughput miniaturized screening of nanoparticle formation via inkjet printing

The self‐assembly of specific polymers into well‐defined nanoparticles (NPs) is of great interest to the pharmaceutical industry as the resultant materials can act as drug delivery vehicles. In this work, a high‐throughput method to screen the ability of polymers to self‐assemble into NPs using a pi...

Full description

Bibliographic Details
Main Authors: Styliari, Ioanna D., Conte, Claudia, Pearce, Amanda K., Hüsler, Amanda, Cavanagh, Robert J., Limo, Marion J., Gordhan, Dipak, Nieto-Orellana, Alejandro, Suksiriworapong, Jiraphong, Couturaud, Benoit, Williams, Phil, Hook, Andrew L., Alexander, Morgan R., Garnett, Martin C., Alexander, Cameron, Burley, Jonathan C., Taresco, Vincenzo
Format: Article
Published: Wiley-VCH 2018
Subjects:
Online Access:https://eprints.nottingham.ac.uk/52245/
_version_ 1848798682174980096
author Styliari, Ioanna D.
Conte, Claudia
Pearce, Amanda K.
Hüsler, Amanda
Cavanagh, Robert J.
Limo, Marion J.
Gordhan, Dipak
Nieto-Orellana, Alejandro
Suksiriworapong, Jiraphong
Couturaud, Benoit
Williams, Phil
Hook, Andrew L.
Alexander, Morgan R.
Garnett, Martin C.
Alexander, Cameron
Burley, Jonathan C.
Taresco, Vincenzo
author_facet Styliari, Ioanna D.
Conte, Claudia
Pearce, Amanda K.
Hüsler, Amanda
Cavanagh, Robert J.
Limo, Marion J.
Gordhan, Dipak
Nieto-Orellana, Alejandro
Suksiriworapong, Jiraphong
Couturaud, Benoit
Williams, Phil
Hook, Andrew L.
Alexander, Morgan R.
Garnett, Martin C.
Alexander, Cameron
Burley, Jonathan C.
Taresco, Vincenzo
author_sort Styliari, Ioanna D.
building Nottingham Research Data Repository
collection Online Access
description The self‐assembly of specific polymers into well‐defined nanoparticles (NPs) is of great interest to the pharmaceutical industry as the resultant materials can act as drug delivery vehicles. In this work, a high‐throughput method to screen the ability of polymers to self‐assemble into NPs using a picoliter inkjet printer is presented. By dispensing polymer solutions in dimethyl sulfoxide (DMSO) from the printer into the wells of a 96‐well plate, containing water as an antisolvent, 50 suspensions are screened for nanoparticle formation rapidly using only nanoliters to microliters. A variety of polymer classes are used and in situ characterization of the submicroliter nanosuspensions shows that the particle size distributions match those of nanoparticles made from bulk suspensions. Dispensing organic polymer solutions into well plates via the printer is thus shown to be a reproducible and fast method for screening nanoparticle formation which uses two to three orders of magnitude less material than conventional techniques. Finally, a pilot study for a high‐throughput pipeline of nanoparticle production, physical property characterization, and cytocompatibility demonstrates the feasibility of the printing approach for screening of nanodrug delivery formulations. Nanoparticles are produced in the well plates, characterized for size and evaluated for effects on metabolic activity of lung cancer cells.
first_indexed 2025-11-14T20:23:39Z
format Article
id nottingham-52245
institution University of Nottingham Malaysia Campus
institution_category Local University
last_indexed 2025-11-14T20:23:39Z
publishDate 2018
publisher Wiley-VCH
recordtype eprints
repository_type Digital Repository
spelling nottingham-522452020-05-04T19:37:53Z https://eprints.nottingham.ac.uk/52245/ High-throughput miniaturized screening of nanoparticle formation via inkjet printing Styliari, Ioanna D. Conte, Claudia Pearce, Amanda K. Hüsler, Amanda Cavanagh, Robert J. Limo, Marion J. Gordhan, Dipak Nieto-Orellana, Alejandro Suksiriworapong, Jiraphong Couturaud, Benoit Williams, Phil Hook, Andrew L. Alexander, Morgan R. Garnett, Martin C. Alexander, Cameron Burley, Jonathan C. Taresco, Vincenzo The self‐assembly of specific polymers into well‐defined nanoparticles (NPs) is of great interest to the pharmaceutical industry as the resultant materials can act as drug delivery vehicles. In this work, a high‐throughput method to screen the ability of polymers to self‐assemble into NPs using a picoliter inkjet printer is presented. By dispensing polymer solutions in dimethyl sulfoxide (DMSO) from the printer into the wells of a 96‐well plate, containing water as an antisolvent, 50 suspensions are screened for nanoparticle formation rapidly using only nanoliters to microliters. A variety of polymer classes are used and in situ characterization of the submicroliter nanosuspensions shows that the particle size distributions match those of nanoparticles made from bulk suspensions. Dispensing organic polymer solutions into well plates via the printer is thus shown to be a reproducible and fast method for screening nanoparticle formation which uses two to three orders of magnitude less material than conventional techniques. Finally, a pilot study for a high‐throughput pipeline of nanoparticle production, physical property characterization, and cytocompatibility demonstrates the feasibility of the printing approach for screening of nanodrug delivery formulations. Nanoparticles are produced in the well plates, characterized for size and evaluated for effects on metabolic activity of lung cancer cells. Wiley-VCH 2018-08 Article PeerReviewed Styliari, Ioanna D., Conte, Claudia, Pearce, Amanda K., Hüsler, Amanda, Cavanagh, Robert J., Limo, Marion J., Gordhan, Dipak, Nieto-Orellana, Alejandro, Suksiriworapong, Jiraphong, Couturaud, Benoit, Williams, Phil, Hook, Andrew L., Alexander, Morgan R., Garnett, Martin C., Alexander, Cameron, Burley, Jonathan C. and Taresco, Vincenzo (2018) High-throughput miniaturized screening of nanoparticle formation via inkjet printing. Macromolecular Materials and Engineering, 303 (8). ISSN 1439-2054 High-throughput miniaturized screening; Inkjet printers; Nanoparticles; Self-assembling https://onlinelibrary.wiley.com/doi/full/10.1002/mame.201800146 doi:10.1002/mame.201800146 doi:10.1002/mame.201800146
spellingShingle High-throughput miniaturized screening; Inkjet printers; Nanoparticles; Self-assembling
Styliari, Ioanna D.
Conte, Claudia
Pearce, Amanda K.
Hüsler, Amanda
Cavanagh, Robert J.
Limo, Marion J.
Gordhan, Dipak
Nieto-Orellana, Alejandro
Suksiriworapong, Jiraphong
Couturaud, Benoit
Williams, Phil
Hook, Andrew L.
Alexander, Morgan R.
Garnett, Martin C.
Alexander, Cameron
Burley, Jonathan C.
Taresco, Vincenzo
High-throughput miniaturized screening of nanoparticle formation via inkjet printing
title High-throughput miniaturized screening of nanoparticle formation via inkjet printing
title_full High-throughput miniaturized screening of nanoparticle formation via inkjet printing
title_fullStr High-throughput miniaturized screening of nanoparticle formation via inkjet printing
title_full_unstemmed High-throughput miniaturized screening of nanoparticle formation via inkjet printing
title_short High-throughput miniaturized screening of nanoparticle formation via inkjet printing
title_sort high-throughput miniaturized screening of nanoparticle formation via inkjet printing
topic High-throughput miniaturized screening; Inkjet printers; Nanoparticles; Self-assembling
url https://eprints.nottingham.ac.uk/52245/
https://eprints.nottingham.ac.uk/52245/
https://eprints.nottingham.ac.uk/52245/