Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension

New microstructures with interesting, unique and stable textures, particularly relevant to food systems were created by redispersing Microfibrillar cellulose (MFC). This paper reports the interactions between microfibrillar cellulose and carboxymethyl cellulose (CMC) in redispersed aqueous suspensio...

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Main Authors: Agarwal, Deepa, Macnaughtan, William, Foster, Tim
Format: Article
Language:English
Published: Elsevier 2018
Subjects:
Online Access:https://eprints.nottingham.ac.uk/50015/
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author Agarwal, Deepa
Macnaughtan, William
Foster, Tim
author_facet Agarwal, Deepa
Macnaughtan, William
Foster, Tim
author_sort Agarwal, Deepa
building Nottingham Research Data Repository
collection Online Access
description New microstructures with interesting, unique and stable textures, particularly relevant to food systems were created by redispersing Microfibrillar cellulose (MFC). This paper reports the interactions between microfibrillar cellulose and carboxymethyl cellulose (CMC) in redispersed aqueous suspensions, by using rheological measurements on variable ratios of MFC/CMC and correlating these with apparent water mobility as determined by time domain NMR. MFC is a network of cellulose fibrils produced by subjecting pure cellulose pulp to high-pressure mechanical homogenisation. A charged polymer such as CMC reduces the aggregation of microfibrillar/fibre bundles upon drying. Small amplitude oscillatory rheological analysis showed the viscoelastic gel-like behaviour of suspensions which was independent of the CMC content in the MFC suspension. A viscous synergistic effect was observed when CMC was added to MFC before drying, leading to improved redispersibility of the suspension. Novel measurements of NMR relaxation suggested that the aggregated microfibrillar/fibre bundles normally dominate the relaxation times (T2). The dense microfibrillar network plays an important role in generating stable rheological properties and controlling the mobility of the polymer and hence the apparent mobility of the water in the suspensions.
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spelling nottingham-500152019-01-02T04:30:31Z https://eprints.nottingham.ac.uk/50015/ Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension Agarwal, Deepa Macnaughtan, William Foster, Tim New microstructures with interesting, unique and stable textures, particularly relevant to food systems were created by redispersing Microfibrillar cellulose (MFC). This paper reports the interactions between microfibrillar cellulose and carboxymethyl cellulose (CMC) in redispersed aqueous suspensions, by using rheological measurements on variable ratios of MFC/CMC and correlating these with apparent water mobility as determined by time domain NMR. MFC is a network of cellulose fibrils produced by subjecting pure cellulose pulp to high-pressure mechanical homogenisation. A charged polymer such as CMC reduces the aggregation of microfibrillar/fibre bundles upon drying. Small amplitude oscillatory rheological analysis showed the viscoelastic gel-like behaviour of suspensions which was independent of the CMC content in the MFC suspension. A viscous synergistic effect was observed when CMC was added to MFC before drying, leading to improved redispersibility of the suspension. Novel measurements of NMR relaxation suggested that the aggregated microfibrillar/fibre bundles normally dominate the relaxation times (T2). The dense microfibrillar network plays an important role in generating stable rheological properties and controlling the mobility of the polymer and hence the apparent mobility of the water in the suspensions. Elsevier 2018-04-01 Article PeerReviewed application/pdf en https://eprints.nottingham.ac.uk/50015/1/DA_Manuscript_Authors%20Accepted_081217.pdf Agarwal, Deepa, Macnaughtan, William and Foster, Tim (2018) Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension. Carbohydrate Polymers, 185 . pp. 112-119. ISSN 1879-1344 Microfibrillar cellulose ; Carboxymethyl cellulose ; Low-field NMR ; Relaxation time ; Rheology https://www.sciencedirect.com/science/article/pii/S0144861717315035 doi:10.1016/j.carbpol.2017.12.086 doi:10.1016/j.carbpol.2017.12.086
spellingShingle Microfibrillar cellulose ; Carboxymethyl cellulose ; Low-field NMR ; Relaxation time ; Rheology
Agarwal, Deepa
Macnaughtan, William
Foster, Tim
Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension
title Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension
title_full Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension
title_fullStr Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension
title_full_unstemmed Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension
title_short Interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension
title_sort interactions between microfibrillar cellulose and carboxymethyl cellulose in an aqueous suspension
topic Microfibrillar cellulose ; Carboxymethyl cellulose ; Low-field NMR ; Relaxation time ; Rheology
url https://eprints.nottingham.ac.uk/50015/
https://eprints.nottingham.ac.uk/50015/
https://eprints.nottingham.ac.uk/50015/