Persistent localized states for a chaotically mixed bistable reaction

We describe the evolution of a bistable chemical reaction in a closed two-dimensional chaotic laminar flow, from a localized initial disturbance. When the fluid mixing is sufficiently slow, the disturbance may spread and eventually occupy the entire fluid domain. By contrast, rapid mixing tends to d...

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Main Author: Cox, Stephen M.
Format: Article
Published: 2006
Subjects:
Online Access:https://eprints.nottingham.ac.uk/499/
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author Cox, Stephen M.
author_facet Cox, Stephen M.
author_sort Cox, Stephen M.
building Nottingham Research Data Repository
collection Online Access
description We describe the evolution of a bistable chemical reaction in a closed two-dimensional chaotic laminar flow, from a localized initial disturbance. When the fluid mixing is sufficiently slow, the disturbance may spread and eventually occupy the entire fluid domain. By contrast, rapid mixing tends to dilute the initial state and so extinguish the disturbance. Such a dichotomy is well known. However, we report here a hitherto apparently unremarked intermediate case, a persistent highly localized disturbance. Such a localized state arises when the Damkoehler number is great enough to sustain a "hot spot," but not so great as to lead to global spread. We show that such a disturbance is located in the neighborhood of an unstable periodic orbit of the flow, and we describe some limited aspects of its behavior using a reduced, lamellar model. Copyright American Physical Society (APS) 2006.
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spelling nottingham-4992020-05-04T20:29:20Z https://eprints.nottingham.ac.uk/499/ Persistent localized states for a chaotically mixed bistable reaction Cox, Stephen M. We describe the evolution of a bistable chemical reaction in a closed two-dimensional chaotic laminar flow, from a localized initial disturbance. When the fluid mixing is sufficiently slow, the disturbance may spread and eventually occupy the entire fluid domain. By contrast, rapid mixing tends to dilute the initial state and so extinguish the disturbance. Such a dichotomy is well known. However, we report here a hitherto apparently unremarked intermediate case, a persistent highly localized disturbance. Such a localized state arises when the Damkoehler number is great enough to sustain a "hot spot," but not so great as to lead to global spread. We show that such a disturbance is located in the neighborhood of an unstable periodic orbit of the flow, and we describe some limited aspects of its behavior using a reduced, lamellar model. Copyright American Physical Society (APS) 2006. 2006-11 Article PeerReviewed Cox, Stephen M. (2006) Persistent localized states for a chaotically mixed bistable reaction. Physical Review E, 74 (5). 056206-1. chaotic advection sine flow localized hotspot
spellingShingle chaotic advection
sine flow
localized hotspot
Cox, Stephen M.
Persistent localized states for a chaotically mixed bistable reaction
title Persistent localized states for a chaotically mixed bistable reaction
title_full Persistent localized states for a chaotically mixed bistable reaction
title_fullStr Persistent localized states for a chaotically mixed bistable reaction
title_full_unstemmed Persistent localized states for a chaotically mixed bistable reaction
title_short Persistent localized states for a chaotically mixed bistable reaction
title_sort persistent localized states for a chaotically mixed bistable reaction
topic chaotic advection
sine flow
localized hotspot
url https://eprints.nottingham.ac.uk/499/