Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication

In this article, we report the synthesis of a series of multi-branched benzylidene (BI) ketone-based photo-initiators for two-photon polymerisation based 3D printing/additive manufacturing. Resins prepared by the addition of 1 wt.% of these initiators were processed in a commercial 2 photon polymeri...

Full description

Bibliographic Details
Main Authors: Zhang, Fan, Hu, Q., Castanon, A., He, Y., Liu, Y., Paul, B.T., Tuck, C.J., Hague, Richard J.M., Wildman, Ricky D.
Format: Article
Published: Elsevier 2017
Subjects:
Online Access:https://eprints.nottingham.ac.uk/48496/
_version_ 1848797777545396224
author Zhang, Fan
Hu, Q.
Castanon, A.
He, Y.
Liu, Y.
Paul, B.T.
Tuck, C.J.
Hague, Richard J.M.
Wildman, Ricky D.
author_facet Zhang, Fan
Hu, Q.
Castanon, A.
He, Y.
Liu, Y.
Paul, B.T.
Tuck, C.J.
Hague, Richard J.M.
Wildman, Ricky D.
author_sort Zhang, Fan
building Nottingham Research Data Repository
collection Online Access
description In this article, we report the synthesis of a series of multi-branched benzylidene (BI) ketone-based photo-initiators for two-photon polymerisation based 3D printing/additive manufacturing. Resins prepared by the addition of 1 wt.% of these initiators were processed in a commercial 2 photon polymerisation system to fabricate 3D woodpile structures, the qualities of which were examined to determine the efficiencies of the initiators. The results showed that compared to commercial initiator Irgacure 369, the four-branched initiator 4-BI exhibited excellent performance with higher writing speeds and broader ideal processing windows. The successful fabrication of complex 3D structures at high writing speeds (up to 100 mm/s) indicated that the four-branched initiator 4-BI could potentially increase the fabrication efficiency and hence become a promising initiator for two-photon polymerisation.
first_indexed 2025-11-14T20:09:16Z
format Article
id nottingham-48496
institution University of Nottingham Malaysia Campus
institution_category Local University
last_indexed 2025-11-14T20:09:16Z
publishDate 2017
publisher Elsevier
recordtype eprints
repository_type Digital Repository
spelling nottingham-484962020-05-04T19:04:22Z https://eprints.nottingham.ac.uk/48496/ Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication Zhang, Fan Hu, Q. Castanon, A. He, Y. Liu, Y. Paul, B.T. Tuck, C.J. Hague, Richard J.M. Wildman, Ricky D. In this article, we report the synthesis of a series of multi-branched benzylidene (BI) ketone-based photo-initiators for two-photon polymerisation based 3D printing/additive manufacturing. Resins prepared by the addition of 1 wt.% of these initiators were processed in a commercial 2 photon polymerisation system to fabricate 3D woodpile structures, the qualities of which were examined to determine the efficiencies of the initiators. The results showed that compared to commercial initiator Irgacure 369, the four-branched initiator 4-BI exhibited excellent performance with higher writing speeds and broader ideal processing windows. The successful fabrication of complex 3D structures at high writing speeds (up to 100 mm/s) indicated that the four-branched initiator 4-BI could potentially increase the fabrication efficiency and hence become a promising initiator for two-photon polymerisation. Elsevier 2017-08-31 Article PeerReviewed Zhang, Fan, Hu, Q., Castanon, A., He, Y., Liu, Y., Paul, B.T., Tuck, C.J., Hague, Richard J.M. and Wildman, Ricky D. (2017) Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication. Additive Manufacturing, 16 . pp. 206-212. ISSN 2214-8604 two photon polymerization; photo-initiator; TPIP; micro-fabrication http://www.sciencedirect.com/science/article/pii/S2214860416301774?via%3Dihub doi:10.1016/j.addma.2017.06.008 doi:10.1016/j.addma.2017.06.008
spellingShingle two photon polymerization; photo-initiator; TPIP; micro-fabrication
Zhang, Fan
Hu, Q.
Castanon, A.
He, Y.
Liu, Y.
Paul, B.T.
Tuck, C.J.
Hague, Richard J.M.
Wildman, Ricky D.
Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication
title Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication
title_full Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication
title_fullStr Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication
title_full_unstemmed Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication
title_short Multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication
title_sort multi-branched benzylidene ketone based photoinitiators for multiphoton fabrication
topic two photon polymerization; photo-initiator; TPIP; micro-fabrication
url https://eprints.nottingham.ac.uk/48496/
https://eprints.nottingham.ac.uk/48496/
https://eprints.nottingham.ac.uk/48496/