Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application

A simple concept is proposed to metallise polyamide 66 (PA66) spherulite structures with in situ synthesised gold nanoparticles (Au NPs) using a wet chemical method. This cost-effective approach, applied to produce a PA66/Au NP hybrid material, offers the advantages of controlling the nanoparticle s...

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Main Authors: Cheval, Nicolas, Gindy, Nabil, Flowkes, Clifford, Fahmi, Amir
Format: Article
Published: Springer 2012
Subjects:
Online Access:https://eprints.nottingham.ac.uk/48305/
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author Cheval, Nicolas
Gindy, Nabil
Flowkes, Clifford
Fahmi, Amir
author_facet Cheval, Nicolas
Gindy, Nabil
Flowkes, Clifford
Fahmi, Amir
author_sort Cheval, Nicolas
building Nottingham Research Data Repository
collection Online Access
description A simple concept is proposed to metallise polyamide 66 (PA66) spherulite structures with in situ synthesised gold nanoparticles (Au NPs) using a wet chemical method. This cost-effective approach, applied to produce a PA66/Au NP hybrid material, offers the advantages of controlling the nanoparticle size, the size distribution and the organic- inorganic interactions. These are the key factors that have to be controlled to construct consistent Au nanostructures which are essential for producing the catalytic activities of interest. The hybrid materials obtained are characterised by means of scanning electron microscopy, transmission electron microscopy, attenuated total reflection-Fourier transform infrared spectrometry and X-ray diffraction spectrometry. The results show that PA66 microspheres obtained via the crystallisation process are coated with Au NPs of 13 nm in size. It was found that controlling the metal coordination is the key parameter to template the Au NPs on the spherulite surfaces. The preparation processes and the key factors leading to the formation of PA66 spherulites coated with Au NPs are discussed. Moreover, the efficiency of the coated spherulites as a potential catalyst is proved by demonstrating the reduction of methylene blue via UV-visible spectrometry.
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spelling nottingham-483052020-05-04T16:34:53Z https://eprints.nottingham.ac.uk/48305/ Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application Cheval, Nicolas Gindy, Nabil Flowkes, Clifford Fahmi, Amir A simple concept is proposed to metallise polyamide 66 (PA66) spherulite structures with in situ synthesised gold nanoparticles (Au NPs) using a wet chemical method. This cost-effective approach, applied to produce a PA66/Au NP hybrid material, offers the advantages of controlling the nanoparticle size, the size distribution and the organic- inorganic interactions. These are the key factors that have to be controlled to construct consistent Au nanostructures which are essential for producing the catalytic activities of interest. The hybrid materials obtained are characterised by means of scanning electron microscopy, transmission electron microscopy, attenuated total reflection-Fourier transform infrared spectrometry and X-ray diffraction spectrometry. The results show that PA66 microspheres obtained via the crystallisation process are coated with Au NPs of 13 nm in size. It was found that controlling the metal coordination is the key parameter to template the Au NPs on the spherulite surfaces. The preparation processes and the key factors leading to the formation of PA66 spherulites coated with Au NPs are discussed. Moreover, the efficiency of the coated spherulites as a potential catalyst is proved by demonstrating the reduction of methylene blue via UV-visible spectrometry. Springer 2012-12-31 Article PeerReviewed Cheval, Nicolas, Gindy, Nabil, Flowkes, Clifford and Fahmi, Amir (2012) Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application. Nanoscale Research Letters, 7 (1). ISSN 1556-276X Polyamide 66; Nanoparticle; Catalyst; Microsphere; Gold; Spherulites https://doi.org/10.1186/1556-276X-7-182 doi:10.1186/1556-276X-7-182 doi:10.1186/1556-276X-7-182
spellingShingle Polyamide 66; Nanoparticle; Catalyst; Microsphere; Gold; Spherulites
Cheval, Nicolas
Gindy, Nabil
Flowkes, Clifford
Fahmi, Amir
Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application
title Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application
title_full Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application
title_fullStr Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application
title_full_unstemmed Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application
title_short Polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application
title_sort polyamide 66 microspheres metallised with in situ synthesised gold nanoparticles for a catalytic application
topic Polyamide 66; Nanoparticle; Catalyst; Microsphere; Gold; Spherulites
url https://eprints.nottingham.ac.uk/48305/
https://eprints.nottingham.ac.uk/48305/
https://eprints.nottingham.ac.uk/48305/