Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea

Context: There is an unmet need to discover new treatments for Alzheimer’s disease. This study determined the anti-acetylcholinesterase (AChE) activity, DPPH free radical scavenging and antioxidant properties of Carpolobia lutea G. Don (Polygalaceae). Objective: To quantify C. lutea anti-AChE, DPPH...

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Main Authors: Nwidu, Lucky Legbosi, Elmorsy, Ekramy, Thornton, Jack, Wijamunige, Buddhika, Wijesekara, Anusha, Tarbox, Rebecca, Warren, Averil, Carter, Wayne
Format: Article
Published: Taylor & Francis 2017
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Online Access:https://eprints.nottingham.ac.uk/43529/
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author Nwidu, Lucky Legbosi
Elmorsy, Ekramy
Thornton, Jack
Wijamunige, Buddhika
Wijesekara, Anusha
Tarbox, Rebecca
Warren, Averil
Carter, Wayne
author_facet Nwidu, Lucky Legbosi
Elmorsy, Ekramy
Thornton, Jack
Wijamunige, Buddhika
Wijesekara, Anusha
Tarbox, Rebecca
Warren, Averil
Carter, Wayne
author_sort Nwidu, Lucky Legbosi
building Nottingham Research Data Repository
collection Online Access
description Context: There is an unmet need to discover new treatments for Alzheimer’s disease. This study determined the anti-acetylcholinesterase (AChE) activity, DPPH free radical scavenging and antioxidant properties of Carpolobia lutea G. Don (Polygalaceae). Objective: To quantify C. lutea anti-AChE, DPPH free radical scavenging, and antioxidant activities, and cell cytotoxicity. Materials and methods: Plant stem, leaves, and roots were subjected to sequential solvent extractions, and screened for anti-AChE activity across a concentration range of 0.02-200 μg//mL. Plant DPPH radical scavenging activity, reducing power, and total phenolic and flavonoid content were determined, and cytotoxicity evaluated using human hepatocytes. Results: C. lutea exhibited concentration dependent anti-AChE activity. The most potent inhibitory activity for the stem was the crude ethanol extract and hexane stem fraction oil (IC₅₀ = 140 μg/mL); for the leaves the chloroform leaf fraction (IC₅₀ = 60 μg/mL/mL); and for roots, the methanol, ethyl acetate, and aqueous root fractions (IC₅₀ = 0.3-3 μg/mL). Dose-dependent free radical scavenging activity and reducing power were observed with increasing stem, leaf, or root concentration. Total phenolics were highest in the stem: ~632 mg gallic acid equivalents/g for a hexane stem fraction oil. Total flavonoid content was highest in the leaves: ~297 mg quercetin equivalents/g for a chloroform leaf fraction. At 1 μg/mL, only the crude ethanol extract oil was significantly cytotoxic to hepatocytes. Discussion and conclusion: C. lutea possesses anti-AChE activity and beneficial antioxidant capacity indicative of its potential development as a treatment of Alzheimer’s and other diseases characterized by a cholinergic deficit.
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spelling nottingham-435292020-05-04T18:50:47Z https://eprints.nottingham.ac.uk/43529/ Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea Nwidu, Lucky Legbosi Elmorsy, Ekramy Thornton, Jack Wijamunige, Buddhika Wijesekara, Anusha Tarbox, Rebecca Warren, Averil Carter, Wayne Context: There is an unmet need to discover new treatments for Alzheimer’s disease. This study determined the anti-acetylcholinesterase (AChE) activity, DPPH free radical scavenging and antioxidant properties of Carpolobia lutea G. Don (Polygalaceae). Objective: To quantify C. lutea anti-AChE, DPPH free radical scavenging, and antioxidant activities, and cell cytotoxicity. Materials and methods: Plant stem, leaves, and roots were subjected to sequential solvent extractions, and screened for anti-AChE activity across a concentration range of 0.02-200 μg//mL. Plant DPPH radical scavenging activity, reducing power, and total phenolic and flavonoid content were determined, and cytotoxicity evaluated using human hepatocytes. Results: C. lutea exhibited concentration dependent anti-AChE activity. The most potent inhibitory activity for the stem was the crude ethanol extract and hexane stem fraction oil (IC₅₀ = 140 μg/mL); for the leaves the chloroform leaf fraction (IC₅₀ = 60 μg/mL/mL); and for roots, the methanol, ethyl acetate, and aqueous root fractions (IC₅₀ = 0.3-3 μg/mL). Dose-dependent free radical scavenging activity and reducing power were observed with increasing stem, leaf, or root concentration. Total phenolics were highest in the stem: ~632 mg gallic acid equivalents/g for a hexane stem fraction oil. Total flavonoid content was highest in the leaves: ~297 mg quercetin equivalents/g for a chloroform leaf fraction. At 1 μg/mL, only the crude ethanol extract oil was significantly cytotoxic to hepatocytes. Discussion and conclusion: C. lutea possesses anti-AChE activity and beneficial antioxidant capacity indicative of its potential development as a treatment of Alzheimer’s and other diseases characterized by a cholinergic deficit. Taylor & Francis 2017-06-19 Article PeerReviewed Nwidu, Lucky Legbosi, Elmorsy, Ekramy, Thornton, Jack, Wijamunige, Buddhika, Wijesekara, Anusha, Tarbox, Rebecca, Warren, Averil and Carter, Wayne (2017) Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea. Pharmaceutical Biology, 55 (1). pp. 1875-1883. ISSN 1744-5116 Anti-acetylcholinesterase; Carpolobia lutea; Antioxidant; Alzheimer's disease https://www.tandfonline.com/doi/full/10.1080/13880209.2017.1339283 doi:10.1080/13880209.2017.1339283 doi:10.1080/13880209.2017.1339283
spellingShingle Anti-acetylcholinesterase; Carpolobia lutea; Antioxidant; Alzheimer's disease
Nwidu, Lucky Legbosi
Elmorsy, Ekramy
Thornton, Jack
Wijamunige, Buddhika
Wijesekara, Anusha
Tarbox, Rebecca
Warren, Averil
Carter, Wayne
Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea
title Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea
title_full Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea
title_fullStr Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea
title_full_unstemmed Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea
title_short Anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of Carpolobia lutea
title_sort anti-acetylcholinesterase activity and antioxidant properties of extracts and fractions of carpolobia lutea
topic Anti-acetylcholinesterase; Carpolobia lutea; Antioxidant; Alzheimer's disease
url https://eprints.nottingham.ac.uk/43529/
https://eprints.nottingham.ac.uk/43529/
https://eprints.nottingham.ac.uk/43529/