Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans

Polysaccharides, the most abundant biopolymers, are required for a host of activities in lower organisms, animals, and plants. Their solution characterization is challenging due to their complex shape, heterogeneity, and size. Here, recently developed data analysis approaches were applied for tradit...

Full description

Bibliographic Details
Main Authors: Gillis, Richard B., Adams, Gary G., Besong, David T.M., Machová, Eva, Ebringerová, Anna, Rowe, Arthur J., Harding, Stephen E., Patel, Trushar R.
Format: Article
Published: Springer 2017
Subjects:
Online Access:https://eprints.nottingham.ac.uk/41686/
_version_ 1848796330862837760
author Gillis, Richard B.
Adams, Gary G.
Besong, David T.M.
Machová, Eva
Ebringerová, Anna
Rowe, Arthur J.
Harding, Stephen E.
Patel, Trushar R.
author_facet Gillis, Richard B.
Adams, Gary G.
Besong, David T.M.
Machová, Eva
Ebringerová, Anna
Rowe, Arthur J.
Harding, Stephen E.
Patel, Trushar R.
author_sort Gillis, Richard B.
building Nottingham Research Data Repository
collection Online Access
description Polysaccharides, the most abundant biopolymers, are required for a host of activities in lower organisms, animals, and plants. Their solution characterization is challenging due to their complex shape, heterogeneity, and size. Here, recently developed data analysis approaches were applied for traditional sedimentation equilibrium and velocity methods in order to investigate the molar mass distribution(s) of a subtype of polysaccharide, namely, mannans from four Candida spp. The molecular weight distributions of these mannans were studied using two recently developed equilibrium approaches: SEDFIT-MSTAR and MULTISIG, resulting in corroboratory distribution profiles. Additionally, sedimentation velocity data for all four mannans, analyzed using ls-g*(s) and Extended Fujita approaches, suggest that two of the fungal mannans (FM-1 and FM-3) have a unimodal distribution of molecular species whereas two others (FM-2 and FM-4) displayed bi-modal and broad distributions, respectively: this demonstrates considerable molecular heterogeneity in these polysaccharides, consistent with previous observations of mannans and polysaccharides in general. These methods not only have applications for the characterization of mannans but for other biopolymers such as polysaccharides, DNA, and proteins (including intrinsically disordered proteins).
first_indexed 2025-11-14T19:46:16Z
format Article
id nottingham-41686
institution University of Nottingham Malaysia Campus
institution_category Local University
last_indexed 2025-11-14T19:46:16Z
publishDate 2017
publisher Springer
recordtype eprints
repository_type Digital Repository
spelling nottingham-416862020-05-04T19:57:57Z https://eprints.nottingham.ac.uk/41686/ Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans Gillis, Richard B. Adams, Gary G. Besong, David T.M. Machová, Eva Ebringerová, Anna Rowe, Arthur J. Harding, Stephen E. Patel, Trushar R. Polysaccharides, the most abundant biopolymers, are required for a host of activities in lower organisms, animals, and plants. Their solution characterization is challenging due to their complex shape, heterogeneity, and size. Here, recently developed data analysis approaches were applied for traditional sedimentation equilibrium and velocity methods in order to investigate the molar mass distribution(s) of a subtype of polysaccharide, namely, mannans from four Candida spp. The molecular weight distributions of these mannans were studied using two recently developed equilibrium approaches: SEDFIT-MSTAR and MULTISIG, resulting in corroboratory distribution profiles. Additionally, sedimentation velocity data for all four mannans, analyzed using ls-g*(s) and Extended Fujita approaches, suggest that two of the fungal mannans (FM-1 and FM-3) have a unimodal distribution of molecular species whereas two others (FM-2 and FM-4) displayed bi-modal and broad distributions, respectively: this demonstrates considerable molecular heterogeneity in these polysaccharides, consistent with previous observations of mannans and polysaccharides in general. These methods not only have applications for the characterization of mannans but for other biopolymers such as polysaccharides, DNA, and proteins (including intrinsically disordered proteins). Springer 2017-04 Article PeerReviewed Gillis, Richard B., Adams, Gary G., Besong, David T.M., Machová, Eva, Ebringerová, Anna, Rowe, Arthur J., Harding, Stephen E. and Patel, Trushar R. (2017) Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans. European Biophysics Journal, 46 (3). pp. 235-245. ISSN 0175-7571 AUC; Extended Fujita approach; MULTISIG; SEDFIT-MSTAR; Sedimentation http://link.springer.com/article/10.1007%2Fs00249-016-1159-5 doi:10.1007/s00249-016-1159-5 doi:10.1007/s00249-016-1159-5
spellingShingle AUC; Extended Fujita approach; MULTISIG; SEDFIT-MSTAR; Sedimentation
Gillis, Richard B.
Adams, Gary G.
Besong, David T.M.
Machová, Eva
Ebringerová, Anna
Rowe, Arthur J.
Harding, Stephen E.
Patel, Trushar R.
Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans
title Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans
title_full Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans
title_fullStr Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans
title_full_unstemmed Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans
title_short Application of novel analytical ultracentrifuge analysis to solutions of fungal mannans
title_sort application of novel analytical ultracentrifuge analysis to solutions of fungal mannans
topic AUC; Extended Fujita approach; MULTISIG; SEDFIT-MSTAR; Sedimentation
url https://eprints.nottingham.ac.uk/41686/
https://eprints.nottingham.ac.uk/41686/
https://eprints.nottingham.ac.uk/41686/