3D printed fluidics with embedded analytic functionality for automated reaction optimisation

Additive manufacturing or ‘3D printing’ is being developed as a novel manufacturing process for the production of bespoke micro- and milliscale fluidic devices. When coupled with online monitoring and optimisation software, this offers an advanced, customised method for performing automated chemical...

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Main Authors: Capel, Andrew J., Wright, Andrew, Harding, Matthew J., Weaver, George W., Li, Yuqi, Harris, Russell A., Edmondson, Steve, Goodridge, Ruth D., Christie, Steven D.R.
Format: Article
Published: Beilstein-Institut 2017
Subjects:
Online Access:https://eprints.nottingham.ac.uk/41469/
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author Capel, Andrew J.
Wright, Andrew
Harding, Matthew J.
Weaver, George W.
Li, Yuqi
Harris, Russell A.
Edmondson, Steve
Goodridge, Ruth D.
Christie, Steven D.R.
author_facet Capel, Andrew J.
Wright, Andrew
Harding, Matthew J.
Weaver, George W.
Li, Yuqi
Harris, Russell A.
Edmondson, Steve
Goodridge, Ruth D.
Christie, Steven D.R.
author_sort Capel, Andrew J.
building Nottingham Research Data Repository
collection Online Access
description Additive manufacturing or ‘3D printing’ is being developed as a novel manufacturing process for the production of bespoke micro- and milliscale fluidic devices. When coupled with online monitoring and optimisation software, this offers an advanced, customised method for performing automated chemical synthesis. This paper reports the use of two additive manufacturing processes, stereolithography and selective laser melting, to create multifunctional fluidic devices with embedded reaction monitoring capability. The selectively laser melted parts are the first published examples of multifunctional 3D printed metal fluidic devices. These devices allow high temperature and pressure chemistry to be performed in solvent systems destructive to the majority of devices manufactured via stereolithography, polymer jetting and fused deposition modelling processes previously utilised for this application. These devices were integrated with commercially available flow chemistry, chromatographic and spectroscopic analysis equipment, allowing automated online and inline optimisation of the reaction medium. This set-up allowed the optimisation of two reactions, a ketone functional group interconversion and a fused polycyclic heterocycle formation, via spectroscopic and chromatographic analysis.
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institution University of Nottingham Malaysia Campus
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publishDate 2017
publisher Beilstein-Institut
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spelling nottingham-414692020-05-04T18:30:13Z https://eprints.nottingham.ac.uk/41469/ 3D printed fluidics with embedded analytic functionality for automated reaction optimisation Capel, Andrew J. Wright, Andrew Harding, Matthew J. Weaver, George W. Li, Yuqi Harris, Russell A. Edmondson, Steve Goodridge, Ruth D. Christie, Steven D.R. Additive manufacturing or ‘3D printing’ is being developed as a novel manufacturing process for the production of bespoke micro- and milliscale fluidic devices. When coupled with online monitoring and optimisation software, this offers an advanced, customised method for performing automated chemical synthesis. This paper reports the use of two additive manufacturing processes, stereolithography and selective laser melting, to create multifunctional fluidic devices with embedded reaction monitoring capability. The selectively laser melted parts are the first published examples of multifunctional 3D printed metal fluidic devices. These devices allow high temperature and pressure chemistry to be performed in solvent systems destructive to the majority of devices manufactured via stereolithography, polymer jetting and fused deposition modelling processes previously utilised for this application. These devices were integrated with commercially available flow chemistry, chromatographic and spectroscopic analysis equipment, allowing automated online and inline optimisation of the reaction medium. This set-up allowed the optimisation of two reactions, a ketone functional group interconversion and a fused polycyclic heterocycle formation, via spectroscopic and chromatographic analysis. Beilstein-Institut 2017-01-18 Article PeerReviewed Capel, Andrew J., Wright, Andrew, Harding, Matthew J., Weaver, George W., Li, Yuqi, Harris, Russell A., Edmondson, Steve, Goodridge, Ruth D. and Christie, Steven D.R. (2017) 3D printed fluidics with embedded analytic functionality for automated reaction optimisation. Beilstein Journal of Organic Chemistry, 13 . pp. 111-119. ISSN 1860-5397 3D printing; Inline reaction analysis; Reaction optimisation; Selective laser melting; Stereolithography http://http://www.beilstein-journals.org/bjoc/single/articleFullText.htm?publicId=1860-5397-13-14 doi:10.3762/bjoc.13.14 doi:10.3762/bjoc.13.14
spellingShingle 3D printing; Inline reaction analysis; Reaction optimisation; Selective laser melting; Stereolithography
Capel, Andrew J.
Wright, Andrew
Harding, Matthew J.
Weaver, George W.
Li, Yuqi
Harris, Russell A.
Edmondson, Steve
Goodridge, Ruth D.
Christie, Steven D.R.
3D printed fluidics with embedded analytic functionality for automated reaction optimisation
title 3D printed fluidics with embedded analytic functionality for automated reaction optimisation
title_full 3D printed fluidics with embedded analytic functionality for automated reaction optimisation
title_fullStr 3D printed fluidics with embedded analytic functionality for automated reaction optimisation
title_full_unstemmed 3D printed fluidics with embedded analytic functionality for automated reaction optimisation
title_short 3D printed fluidics with embedded analytic functionality for automated reaction optimisation
title_sort 3d printed fluidics with embedded analytic functionality for automated reaction optimisation
topic 3D printing; Inline reaction analysis; Reaction optimisation; Selective laser melting; Stereolithography
url https://eprints.nottingham.ac.uk/41469/
https://eprints.nottingham.ac.uk/41469/
https://eprints.nottingham.ac.uk/41469/