Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition

A range of coatings from a water based suspension of anatase has been prepared by suspension high velocity oxy-fuel spraying with the aim to study effects of heat power of the flame on phase composition, microstructure and surface topography. Three most commonly used approaches of quantitative phase...

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Main Authors: Pala, Z., Shaw, E., Murray, J.W., Senin, Nicola, Hussain, Tanvir
Format: Article
Published: Elsevier 2017
Subjects:
Online Access:https://eprints.nottingham.ac.uk/38916/
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author Pala, Z.
Shaw, E.
Murray, J.W.
Senin, Nicola
Hussain, Tanvir
author_facet Pala, Z.
Shaw, E.
Murray, J.W.
Senin, Nicola
Hussain, Tanvir
author_sort Pala, Z.
building Nottingham Research Data Repository
collection Online Access
description A range of coatings from a water based suspension of anatase has been prepared by suspension high velocity oxy-fuel spraying with the aim to study effects of heat power of the flame on phase composition, microstructure and surface topography. Three most commonly used approaches of quantitative phase analysis have been scrutinized with respect to their applicability and as some of the coatings showed presence of preferred orientation and it was argued that quantitative Rietveld refinement is the most accurate method for phase composition determination. Coatings had a layered duplex anatase/rutile microstructure with fraction of rutile increasing exponentially with heat power. Spraying at the lower heat power led to a lower surface roughness and higher power resulted in surfaces with pronounced humps, which were distributed homogeneously on the surface. The emergence of humps is related to an increase in macroscopic surface area of up to 30% with respect to the flat coating.
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spelling nottingham-389162020-05-04T19:58:45Z https://eprints.nottingham.ac.uk/38916/ Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition Pala, Z. Shaw, E. Murray, J.W. Senin, Nicola Hussain, Tanvir A range of coatings from a water based suspension of anatase has been prepared by suspension high velocity oxy-fuel spraying with the aim to study effects of heat power of the flame on phase composition, microstructure and surface topography. Three most commonly used approaches of quantitative phase analysis have been scrutinized with respect to their applicability and as some of the coatings showed presence of preferred orientation and it was argued that quantitative Rietveld refinement is the most accurate method for phase composition determination. Coatings had a layered duplex anatase/rutile microstructure with fraction of rutile increasing exponentially with heat power. Spraying at the lower heat power led to a lower surface roughness and higher power resulted in surfaces with pronounced humps, which were distributed homogeneously on the surface. The emergence of humps is related to an increase in macroscopic surface area of up to 30% with respect to the flat coating. Elsevier 2017-02 Article PeerReviewed Pala, Z., Shaw, E., Murray, J.W., Senin, Nicola and Hussain, Tanvir (2017) Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition. Journal of the European Ceramic Society, 37 (2). pp. 801-810. ISSN 1873-619X Suspension HVOF spraying; Rietveld refinement; Topography; Anatase; Rutile http://www.sciencedirect.com/science/article/pii/S0955221916304642 doi:10.1016/j.jeurceramsoc.2016.08.030 doi:10.1016/j.jeurceramsoc.2016.08.030
spellingShingle Suspension HVOF spraying; Rietveld refinement; Topography; Anatase; Rutile
Pala, Z.
Shaw, E.
Murray, J.W.
Senin, Nicola
Hussain, Tanvir
Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition
title Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition
title_full Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition
title_fullStr Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition
title_full_unstemmed Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition
title_short Suspension high velocity oxy-fuel spraying of TiO2: a quantitative approach to phase composition
title_sort suspension high velocity oxy-fuel spraying of tio2: a quantitative approach to phase composition
topic Suspension HVOF spraying; Rietveld refinement; Topography; Anatase; Rutile
url https://eprints.nottingham.ac.uk/38916/
https://eprints.nottingham.ac.uk/38916/
https://eprints.nottingham.ac.uk/38916/