Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF

Molecules of tris(2,2’-bipyridine-4-thiomethyl-BEDT-TTF)iron(II) (BEDT-TTF = bis(ethylenedithio)tetrathiafulvalene) assemble in pairs to form a novel supramolecular capsular structure in the solid state. Three BEDT-TTF residues from one complex lie in the three grooves between coordinated bipyridine...

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Main Authors: Wang, Qiang, Martin, Lee, Blake, Alexander J., Day, Peter, Akutsu, Hiroki, Wallis, John D.
Format: Article
Published: American Chemical Society 2016
Online Access:https://eprints.nottingham.ac.uk/37760/
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author Wang, Qiang
Martin, Lee
Blake, Alexander J.
Day, Peter
Akutsu, Hiroki
Wallis, John D.
author_facet Wang, Qiang
Martin, Lee
Blake, Alexander J.
Day, Peter
Akutsu, Hiroki
Wallis, John D.
author_sort Wang, Qiang
building Nottingham Research Data Repository
collection Online Access
description Molecules of tris(2,2’-bipyridine-4-thiomethyl-BEDT-TTF)iron(II) (BEDT-TTF = bis(ethylenedithio)tetrathiafulvalene) assemble in pairs to form a novel supramolecular capsular structure in the solid state. Three BEDT-TTF residues from one complex lie in the three grooves between coordinated bipyridines of the other complex, and vice versa, to form a capsule with three-fold rotational symmetry and an internal volume of ca. 160 Å3. Further aspects of the coordination chemistry of this ligand, its 6-substituted isomer and the 2,2’:6’2’’- terpyridyl-4’-thiomethyl-BEDT-TTF analogue are described.
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spelling nottingham-377602020-05-04T18:13:36Z https://eprints.nottingham.ac.uk/37760/ Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF Wang, Qiang Martin, Lee Blake, Alexander J. Day, Peter Akutsu, Hiroki Wallis, John D. Molecules of tris(2,2’-bipyridine-4-thiomethyl-BEDT-TTF)iron(II) (BEDT-TTF = bis(ethylenedithio)tetrathiafulvalene) assemble in pairs to form a novel supramolecular capsular structure in the solid state. Three BEDT-TTF residues from one complex lie in the three grooves between coordinated bipyridines of the other complex, and vice versa, to form a capsule with three-fold rotational symmetry and an internal volume of ca. 160 Å3. Further aspects of the coordination chemistry of this ligand, its 6-substituted isomer and the 2,2’:6’2’’- terpyridyl-4’-thiomethyl-BEDT-TTF analogue are described. American Chemical Society 2016-09-06 Article PeerReviewed Wang, Qiang, Martin, Lee, Blake, Alexander J., Day, Peter, Akutsu, Hiroki and Wallis, John D. (2016) Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF. Inorganic Chemistry, 55 (17). pp. 8543-8551. ISSN 1520-510X http://pubs.acs.org/doi/abs/10.1021/acs.inorgchem.6b01101 doi:10.1021/acs.inorgchem.6b01101 doi:10.1021/acs.inorgchem.6b01101
spellingShingle Wang, Qiang
Martin, Lee
Blake, Alexander J.
Day, Peter
Akutsu, Hiroki
Wallis, John D.
Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF
title Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF
title_full Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF
title_fullStr Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF
title_full_unstemmed Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF
title_short Coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted BEDT-TTFs: formation of a supramolecular capsule motif by the iron(II) tris complex of 2,2’-bipyridine-4-thiomethyl-BEDT-TTF
title_sort coordination chemistry of 2,2’-bipyridyl- and 2,2’:6’,2”-terpyridyl-substituted bedt-ttfs: formation of a supramolecular capsule motif by the iron(ii) tris complex of 2,2’-bipyridine-4-thiomethyl-bedt-ttf
url https://eprints.nottingham.ac.uk/37760/
https://eprints.nottingham.ac.uk/37760/
https://eprints.nottingham.ac.uk/37760/