Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy

We demonstrate direct epitaxial growth of high-quality hexagonal boron nitride (hBN) layers on graphite using high-temperature plasma-assisted molecular beam epitaxy. Atomic force microscopy reveals mono- and few-layer island growth, while conducting atomic force microscopy shows that the grown hBN...

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Main Authors: Cho, Yong-Jin, Summerfield, Alex, Davies, Andrew, Cheng, Tin S., Smith, Emily F., Mellor, Christopher J., Khlobystov, Andrei N., Foxon, C. Thomas, Eaves, Laurence, Beton, Peter H., Novikov, Sergei V.
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Published: Nature Publishing Group 2016
Online Access:https://eprints.nottingham.ac.uk/37309/
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author Cho, Yong-Jin
Summerfield, Alex
Davies, Andrew
Cheng, Tin S.
Smith, Emily F.
Mellor, Christopher J.
Khlobystov, Andrei N.
Foxon, C. Thomas
Eaves, Laurence
Beton, Peter H.
Novikov, Sergei V.
author_facet Cho, Yong-Jin
Summerfield, Alex
Davies, Andrew
Cheng, Tin S.
Smith, Emily F.
Mellor, Christopher J.
Khlobystov, Andrei N.
Foxon, C. Thomas
Eaves, Laurence
Beton, Peter H.
Novikov, Sergei V.
author_sort Cho, Yong-Jin
building Nottingham Research Data Repository
collection Online Access
description We demonstrate direct epitaxial growth of high-quality hexagonal boron nitride (hBN) layers on graphite using high-temperature plasma-assisted molecular beam epitaxy. Atomic force microscopy reveals mono- and few-layer island growth, while conducting atomic force microscopy shows that the grown hBN has a resistance which increases exponentially with the number of layers, and has electrical properties comparable to exfoliated hBN. X-ray photoelectron spectroscopy, Raman microscopy and spectroscopic ellipsometry measurements on hBN confirm the formation of sp2-bonded hBN and a band gap of 5.9 ± 0.1 eV with no chemical intermixing with graphite. We also observe hexagonal moiré patterns with a period of 15 nm, consistent with the alignment of the hBN lattice and the graphite substrate.
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institution University of Nottingham Malaysia Campus
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publishDate 2016
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spelling nottingham-373092020-05-04T18:09:09Z https://eprints.nottingham.ac.uk/37309/ Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy Cho, Yong-Jin Summerfield, Alex Davies, Andrew Cheng, Tin S. Smith, Emily F. Mellor, Christopher J. Khlobystov, Andrei N. Foxon, C. Thomas Eaves, Laurence Beton, Peter H. Novikov, Sergei V. We demonstrate direct epitaxial growth of high-quality hexagonal boron nitride (hBN) layers on graphite using high-temperature plasma-assisted molecular beam epitaxy. Atomic force microscopy reveals mono- and few-layer island growth, while conducting atomic force microscopy shows that the grown hBN has a resistance which increases exponentially with the number of layers, and has electrical properties comparable to exfoliated hBN. X-ray photoelectron spectroscopy, Raman microscopy and spectroscopic ellipsometry measurements on hBN confirm the formation of sp2-bonded hBN and a band gap of 5.9 ± 0.1 eV with no chemical intermixing with graphite. We also observe hexagonal moiré patterns with a period of 15 nm, consistent with the alignment of the hBN lattice and the graphite substrate. Nature Publishing Group 2016-09-29 Article PeerReviewed Cho, Yong-Jin, Summerfield, Alex, Davies, Andrew, Cheng, Tin S., Smith, Emily F., Mellor, Christopher J., Khlobystov, Andrei N., Foxon, C. Thomas, Eaves, Laurence, Beton, Peter H. and Novikov, Sergei V. (2016) Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy. Scientific Reports, 6 . 34474/1-34474/6. ISSN 2045-2322 http://www.nature.com/articles/srep34474 doi:10.1038/srep34474 doi:10.1038/srep34474
spellingShingle Cho, Yong-Jin
Summerfield, Alex
Davies, Andrew
Cheng, Tin S.
Smith, Emily F.
Mellor, Christopher J.
Khlobystov, Andrei N.
Foxon, C. Thomas
Eaves, Laurence
Beton, Peter H.
Novikov, Sergei V.
Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy
title Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy
title_full Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy
title_fullStr Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy
title_full_unstemmed Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy
title_short Hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy
title_sort hexagonal boron nitride tunnel barriers grown on graphite by high temperature molecular beam epitaxy
url https://eprints.nottingham.ac.uk/37309/
https://eprints.nottingham.ac.uk/37309/
https://eprints.nottingham.ac.uk/37309/