The impact of oxidation on spore and pollen chemistry

Sporomorphs (pollen and spores) have an outer wall composed of sporopollenin. Sporopollenin chemistry contains both a signature of ambient ultraviolet-B flux and taxonomic information, but it is currently unknown how sensitive this is to standard palynological processing techniques. Oxidation in par...

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Main Authors: Jardine, Phillip E., Fraser, Wesley T., Lomax, Barry H., Gosling, William D.
Format: Article
Published: Geological Society 2015
Subjects:
Online Access:https://eprints.nottingham.ac.uk/37162/
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author Jardine, Phillip E.
Fraser, Wesley T.
Lomax, Barry H.
Gosling, William D.
author_facet Jardine, Phillip E.
Fraser, Wesley T.
Lomax, Barry H.
Gosling, William D.
author_sort Jardine, Phillip E.
building Nottingham Research Data Repository
collection Online Access
description Sporomorphs (pollen and spores) have an outer wall composed of sporopollenin. Sporopollenin chemistry contains both a signature of ambient ultraviolet-B flux and taxonomic information, but it is currently unknown how sensitive this is to standard palynological processing techniques. Oxidation in particular is known to cause physical degradation to sporomorphs, and it is expected that this should have a concordant impact on sporopollenin chemistry. Here, we test this by experimentally oxidizing Lycopodium (clubmoss) spores using two common oxidation techniques: acetolysis and nitric acid. We also carry out acetolysis on eight angiosperm (flowering plant) taxa to test the generality of our results. Using Fourier Transform infrared (FTIR) spectroscopy, we find that acetolysis removes labile, non-fossilizable components of sporomorphs, but has a limited impact upon the chemistry of sporopollenin under normal processing durations. Nitric acid is more aggressive and does break down sporopollenin and reorganize its chemical structure, but when limited to short treatments (i.e. ≤10 min) at room temperature sporomorphs still contain most of the original chemical signal. These findings suggest that when used carefully oxidation does not adversely affect sporopollenin chemistry, and that palaeoclimatic and taxonomic signatures contained within the sporomorph wall are recoverable from standard palynological preparations.
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spelling nottingham-371622020-05-04T17:05:21Z https://eprints.nottingham.ac.uk/37162/ The impact of oxidation on spore and pollen chemistry Jardine, Phillip E. Fraser, Wesley T. Lomax, Barry H. Gosling, William D. Sporomorphs (pollen and spores) have an outer wall composed of sporopollenin. Sporopollenin chemistry contains both a signature of ambient ultraviolet-B flux and taxonomic information, but it is currently unknown how sensitive this is to standard palynological processing techniques. Oxidation in particular is known to cause physical degradation to sporomorphs, and it is expected that this should have a concordant impact on sporopollenin chemistry. Here, we test this by experimentally oxidizing Lycopodium (clubmoss) spores using two common oxidation techniques: acetolysis and nitric acid. We also carry out acetolysis on eight angiosperm (flowering plant) taxa to test the generality of our results. Using Fourier Transform infrared (FTIR) spectroscopy, we find that acetolysis removes labile, non-fossilizable components of sporomorphs, but has a limited impact upon the chemistry of sporopollenin under normal processing durations. Nitric acid is more aggressive and does break down sporopollenin and reorganize its chemical structure, but when limited to short treatments (i.e. ≤10 min) at room temperature sporomorphs still contain most of the original chemical signal. These findings suggest that when used carefully oxidation does not adversely affect sporopollenin chemistry, and that palaeoclimatic and taxonomic signatures contained within the sporomorph wall are recoverable from standard palynological preparations. Geological Society 2015-05-01 Article PeerReviewed Jardine, Phillip E., Fraser, Wesley T., Lomax, Barry H. and Gosling, William D. (2015) The impact of oxidation on spore and pollen chemistry. Journal of Micropalaeontology, 34 (2). pp. 139-149. ISSN 2041-4978 oxidation palynology ultraviolet-B FTIR sporopollenin http://jm.lyellcollection.org/content/early/2015/04/28/jmpaleo2014-022 doi:10.1144/jmpaleo2014-022 doi:10.1144/jmpaleo2014-022
spellingShingle oxidation
palynology
ultraviolet-B
FTIR
sporopollenin
Jardine, Phillip E.
Fraser, Wesley T.
Lomax, Barry H.
Gosling, William D.
The impact of oxidation on spore and pollen chemistry
title The impact of oxidation on spore and pollen chemistry
title_full The impact of oxidation on spore and pollen chemistry
title_fullStr The impact of oxidation on spore and pollen chemistry
title_full_unstemmed The impact of oxidation on spore and pollen chemistry
title_short The impact of oxidation on spore and pollen chemistry
title_sort impact of oxidation on spore and pollen chemistry
topic oxidation
palynology
ultraviolet-B
FTIR
sporopollenin
url https://eprints.nottingham.ac.uk/37162/
https://eprints.nottingham.ac.uk/37162/
https://eprints.nottingham.ac.uk/37162/