Expedient synthesis of an atypical oxazolidinone compound library

In order to address the current downturn in the drug discovery pipeline, initiatives are being undertaken to synthesise screening libraries of sp3-rich, low molecular weight compounds. As part of the European Lead Factory initiative, the synthesis and derivatisation of a simple hexahydrooxazolo[5,4-...

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Main Authors: Cully, Sarah J., Storr, Thomas E., Rawling, Michael J., Abeysena, Induka R., Hamza, Daniel, Jones, Geraint, Pearce, Christopher A., Quddus, Abdul, Lewis, William, Stockman, Robert A.
Format: Article
Published: Elsevier 2016
Online Access:https://eprints.nottingham.ac.uk/36176/
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author Cully, Sarah J.
Storr, Thomas E.
Rawling, Michael J.
Abeysena, Induka R.
Hamza, Daniel
Jones, Geraint
Pearce, Christopher A.
Quddus, Abdul
Lewis, William
Stockman, Robert A.
author_facet Cully, Sarah J.
Storr, Thomas E.
Rawling, Michael J.
Abeysena, Induka R.
Hamza, Daniel
Jones, Geraint
Pearce, Christopher A.
Quddus, Abdul
Lewis, William
Stockman, Robert A.
author_sort Cully, Sarah J.
building Nottingham Research Data Repository
collection Online Access
description In order to address the current downturn in the drug discovery pipeline, initiatives are being undertaken to synthesise screening libraries of sp3-rich, low molecular weight compounds. As part of the European Lead Factory initiative, the synthesis and derivatisation of a simple hexahydrooxazolo[5,4-c]pyridin-2(1H)-one bicyclic carbamate has been achieved. The synthetic route employed involved a telescoped hetero-Diels-Alder/[2,3]-sigmatropic rearrangement/cyclisation sequence to deliver the desired core scaffold containing two points for further diversification. When applied, this synthesis was found to be robust and scalable which allowed the production of a 155 compound library.
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publishDate 2016
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spelling nottingham-361762020-05-04T18:05:35Z https://eprints.nottingham.ac.uk/36176/ Expedient synthesis of an atypical oxazolidinone compound library Cully, Sarah J. Storr, Thomas E. Rawling, Michael J. Abeysena, Induka R. Hamza, Daniel Jones, Geraint Pearce, Christopher A. Quddus, Abdul Lewis, William Stockman, Robert A. In order to address the current downturn in the drug discovery pipeline, initiatives are being undertaken to synthesise screening libraries of sp3-rich, low molecular weight compounds. As part of the European Lead Factory initiative, the synthesis and derivatisation of a simple hexahydrooxazolo[5,4-c]pyridin-2(1H)-one bicyclic carbamate has been achieved. The synthetic route employed involved a telescoped hetero-Diels-Alder/[2,3]-sigmatropic rearrangement/cyclisation sequence to deliver the desired core scaffold containing two points for further diversification. When applied, this synthesis was found to be robust and scalable which allowed the production of a 155 compound library. Elsevier 2016-08-27 Article PeerReviewed Cully, Sarah J., Storr, Thomas E., Rawling, Michael J., Abeysena, Induka R., Hamza, Daniel, Jones, Geraint, Pearce, Christopher A., Quddus, Abdul, Lewis, William and Stockman, Robert A. (2016) Expedient synthesis of an atypical oxazolidinone compound library. Bioorganic and Medicinal Chemistry . ISSN 1464-3391 http://www.sciencedirect.com/science/article/pii/S096808961630654X doi:10.1016/j.bmc.2016.08.046 doi:10.1016/j.bmc.2016.08.046
spellingShingle Cully, Sarah J.
Storr, Thomas E.
Rawling, Michael J.
Abeysena, Induka R.
Hamza, Daniel
Jones, Geraint
Pearce, Christopher A.
Quddus, Abdul
Lewis, William
Stockman, Robert A.
Expedient synthesis of an atypical oxazolidinone compound library
title Expedient synthesis of an atypical oxazolidinone compound library
title_full Expedient synthesis of an atypical oxazolidinone compound library
title_fullStr Expedient synthesis of an atypical oxazolidinone compound library
title_full_unstemmed Expedient synthesis of an atypical oxazolidinone compound library
title_short Expedient synthesis of an atypical oxazolidinone compound library
title_sort expedient synthesis of an atypical oxazolidinone compound library
url https://eprints.nottingham.ac.uk/36176/
https://eprints.nottingham.ac.uk/36176/
https://eprints.nottingham.ac.uk/36176/