Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation

This paper investigates the β-phase depletion behaviour during oxidation of free-standing CoNiCrA1Y (Co-31.7%Ni-20.8%Cr-8.1%A1-0.5%Y, all in wt%) bond coats prepared by high velocity oxy-fuel (HVOF) thermal spraying. The microstructure of the coatings was characterised using scanning electron micros...

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Main Authors: Chen, H., Jackson, G.A., Voisey, K.T., McCartney, D.G.
Format: Article
Published: Elsevier 2016
Subjects:
Online Access:https://eprints.nottingham.ac.uk/34384/
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author Chen, H.
Jackson, G.A.
Voisey, K.T.
McCartney, D.G.
author_facet Chen, H.
Jackson, G.A.
Voisey, K.T.
McCartney, D.G.
author_sort Chen, H.
building Nottingham Research Data Repository
collection Online Access
description This paper investigates the β-phase depletion behaviour during oxidation of free-standing CoNiCrA1Y (Co-31.7%Ni-20.8%Cr-8.1%A1-0.5%Y, all in wt%) bond coats prepared by high velocity oxy-fuel (HVOF) thermal spraying. The microstructure of the coatings was characterised using scanning electron microscopy with energy dispersive X-ray (EDX) analysis and electron backscatter diffraction (EBSD). It comprises a two phase structure of fcc γ-Ni and bcc β-NiA1, with grain sizes varying largely from 0.5 to 2 μm for both phases. Isothermal oxidation tests of the free-standing coatings were carried out at 1100 °C for times up to 250 h. The β phase depletion behaviour at the surface was measured and was also simulated using Thermo-Calc and DICTRA software. An A1 flux function derived from an oxide growth model was employed as the boundary condition in the diffusion model. The diffusion calculations were performed using the TTNi7 thermodynamic database together with the MOB2 mobility database. Reasonable agreement was achieved between the measured and the predicted element concentration and phase fraction profiles after various time periods. Grain boundary diffusion is likely to be important to element diffusion in this HVOF sprayed CoNiCrA1Y coating due to the sub-micron grains.
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spelling nottingham-343842020-05-04T17:46:25Z https://eprints.nottingham.ac.uk/34384/ Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation Chen, H. Jackson, G.A. Voisey, K.T. McCartney, D.G. This paper investigates the β-phase depletion behaviour during oxidation of free-standing CoNiCrA1Y (Co-31.7%Ni-20.8%Cr-8.1%A1-0.5%Y, all in wt%) bond coats prepared by high velocity oxy-fuel (HVOF) thermal spraying. The microstructure of the coatings was characterised using scanning electron microscopy with energy dispersive X-ray (EDX) analysis and electron backscatter diffraction (EBSD). It comprises a two phase structure of fcc γ-Ni and bcc β-NiA1, with grain sizes varying largely from 0.5 to 2 μm for both phases. Isothermal oxidation tests of the free-standing coatings were carried out at 1100 °C for times up to 250 h. The β phase depletion behaviour at the surface was measured and was also simulated using Thermo-Calc and DICTRA software. An A1 flux function derived from an oxide growth model was employed as the boundary condition in the diffusion model. The diffusion calculations were performed using the TTNi7 thermodynamic database together with the MOB2 mobility database. Reasonable agreement was achieved between the measured and the predicted element concentration and phase fraction profiles after various time periods. Grain boundary diffusion is likely to be important to element diffusion in this HVOF sprayed CoNiCrA1Y coating due to the sub-micron grains. Elsevier 2016-04-15 Article PeerReviewed Chen, H., Jackson, G.A., Voisey, K.T. and McCartney, D.G. (2016) Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation. Surface and Coatings Technology, 291 . pp. 34-42. ISSN 1879-3347 HVOF Spraying MCrA1Y Oxidation β Depletion Diffusion http://www.sciencedirect.com/science/article/pii/S0257897216300706 doi:10.1016/j.surfcoat.2016.02.008 doi:10.1016/j.surfcoat.2016.02.008
spellingShingle HVOF Spraying
MCrA1Y
Oxidation
β Depletion
Diffusion
Chen, H.
Jackson, G.A.
Voisey, K.T.
McCartney, D.G.
Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation
title Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation
title_full Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation
title_fullStr Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation
title_full_unstemmed Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation
title_short Modelling and experimental study on β-phase depletion behaviour of HVOF sprayed free-standing CoNiCrA1Y coatings during oxidation
title_sort modelling and experimental study on β-phase depletion behaviour of hvof sprayed free-standing conicra1y coatings during oxidation
topic HVOF Spraying
MCrA1Y
Oxidation
β Depletion
Diffusion
url https://eprints.nottingham.ac.uk/34384/
https://eprints.nottingham.ac.uk/34384/
https://eprints.nottingham.ac.uk/34384/