Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire

Van der Waals (vdW) layered crystals and heterostructures have attracted substantial interest for potential applications in a wide range of emerging technologies. An important, but often overlooked, consideration in the development of implementable devices is phonon transport through the structure i...

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Main Authors: Beardsley, R.P., Akimov, Andrey V., Greener, Jake D.G., Mudd, Gary W., Sandeep, Sathyan, Kudrynskyi, Zakhar R., Kovalyuk, Zakhar D., Patanè, Amalia, Kent, Anthony J.
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Published: Nature Publishing Group 2016
Online Access:https://eprints.nottingham.ac.uk/33530/
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author Beardsley, R.P.
Akimov, Andrey V.
Greener, Jake D.G.
Mudd, Gary W.
Sandeep, Sathyan
Kudrynskyi, Zakhar R.
Kovalyuk, Zakhar D.
Patanè, Amalia
Kent, Anthony J.
author_facet Beardsley, R.P.
Akimov, Andrey V.
Greener, Jake D.G.
Mudd, Gary W.
Sandeep, Sathyan
Kudrynskyi, Zakhar R.
Kovalyuk, Zakhar D.
Patanè, Amalia
Kent, Anthony J.
author_sort Beardsley, R.P.
building Nottingham Research Data Repository
collection Online Access
description Van der Waals (vdW) layered crystals and heterostructures have attracted substantial interest for potential applications in a wide range of emerging technologies. An important, but often overlooked, consideration in the development of implementable devices is phonon transport through the structure interfaces. Here we report on the interface properties of exfoliated InSe on a sapphire substrate. We use a picosecond acoustic technique to probe the phonon resonances in the InSe vdW layered crystal. Analysis of the nanomechanics indicates that the InSe is mechanically decoupled from the substrate and thus presents an elastically imperfect interface. A high degree of phonon isolation at the interface points toward applications in thermoelectric devices, or the inclusion of an acoustic transition layer in device design. These findings demonstrate basic properties of layered structures and so illustrate the usefulness of nanomechanical probing in nanolayer/nanolayer or nanolayer/substrate interface tuning in vdW heterostructures.
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spelling nottingham-335302020-05-04T17:57:49Z https://eprints.nottingham.ac.uk/33530/ Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire Beardsley, R.P. Akimov, Andrey V. Greener, Jake D.G. Mudd, Gary W. Sandeep, Sathyan Kudrynskyi, Zakhar R. Kovalyuk, Zakhar D. Patanè, Amalia Kent, Anthony J. Van der Waals (vdW) layered crystals and heterostructures have attracted substantial interest for potential applications in a wide range of emerging technologies. An important, but often overlooked, consideration in the development of implementable devices is phonon transport through the structure interfaces. Here we report on the interface properties of exfoliated InSe on a sapphire substrate. We use a picosecond acoustic technique to probe the phonon resonances in the InSe vdW layered crystal. Analysis of the nanomechanics indicates that the InSe is mechanically decoupled from the substrate and thus presents an elastically imperfect interface. A high degree of phonon isolation at the interface points toward applications in thermoelectric devices, or the inclusion of an acoustic transition layer in device design. These findings demonstrate basic properties of layered structures and so illustrate the usefulness of nanomechanical probing in nanolayer/nanolayer or nanolayer/substrate interface tuning in vdW heterostructures. Nature Publishing Group 2016-06-03 Article PeerReviewed Beardsley, R.P., Akimov, Andrey V., Greener, Jake D.G., Mudd, Gary W., Sandeep, Sathyan, Kudrynskyi, Zakhar R., Kovalyuk, Zakhar D., Patanè, Amalia and Kent, Anthony J. (2016) Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire. Scientific Reports, 6 . p. 26970. ISSN 2045-2322 http://www.nature.com/articles/srep26970 doi:10.1038/srep26970 doi:10.1038/srep26970
spellingShingle Beardsley, R.P.
Akimov, Andrey V.
Greener, Jake D.G.
Mudd, Gary W.
Sandeep, Sathyan
Kudrynskyi, Zakhar R.
Kovalyuk, Zakhar D.
Patanè, Amalia
Kent, Anthony J.
Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire
title Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire
title_full Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire
title_fullStr Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire
title_full_unstemmed Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire
title_short Nanomechanical probing of the layer/substrate interface of an exfoliated InSe sheet on sapphire
title_sort nanomechanical probing of the layer/substrate interface of an exfoliated inse sheet on sapphire
url https://eprints.nottingham.ac.uk/33530/
https://eprints.nottingham.ac.uk/33530/
https://eprints.nottingham.ac.uk/33530/