Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms

We present photoelectron energy and angular distributions for resonant two-photon ionization via several low-lying Rydberg states of atomic Kr. The experiments were performed by using synchrotron radiation to pump the Rydberg states and a continuous wave laser to probe them. Photoelectron images, re...

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Main Authors: Saquet, N., Holland, D.M.P., Pratt, S.T., Cubaynes, D., Tang, X., Garcia, G.A., Nahon, Laurent, Reid, Katharine L.
Format: Article
Published: American Physical Society 2016
Online Access:https://eprints.nottingham.ac.uk/32006/
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author Saquet, N.
Holland, D.M.P.
Pratt, S.T.
Cubaynes, D.
Tang, X.
Garcia, G.A.
Nahon, Laurent
Reid, Katharine L.
author_facet Saquet, N.
Holland, D.M.P.
Pratt, S.T.
Cubaynes, D.
Tang, X.
Garcia, G.A.
Nahon, Laurent
Reid, Katharine L.
author_sort Saquet, N.
building Nottingham Research Data Repository
collection Online Access
description We present photoelectron energy and angular distributions for resonant two-photon ionization via several low-lying Rydberg states of atomic Kr. The experiments were performed by using synchrotron radiation to pump the Rydberg states and a continuous wave laser to probe them. Photoelectron images, recorded with both linear and circular polarized pump and probe light, were obtained in coincidence with mass-analyzed Kr ions. The photoelectron angular distributions and branching ratios for direct ionization into the Kr+ 2P3/2 and 2P1/2 spin-orbit continua show considerable dependence on the intermediate level, as well as on the polarizations of the pump and probe light. Photoelectron angular distributions were also recorded with several polarization combinations following two-colour excitation of the (2P1/2)5f[5/2]2 autoionizing resonance. These results are compared with the results of recent work on the corresponding autoionizing resonance in atomic Xe.
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spelling nottingham-320062020-05-04T17:40:04Z https://eprints.nottingham.ac.uk/32006/ Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms Saquet, N. Holland, D.M.P. Pratt, S.T. Cubaynes, D. Tang, X. Garcia, G.A. Nahon, Laurent Reid, Katharine L. We present photoelectron energy and angular distributions for resonant two-photon ionization via several low-lying Rydberg states of atomic Kr. The experiments were performed by using synchrotron radiation to pump the Rydberg states and a continuous wave laser to probe them. Photoelectron images, recorded with both linear and circular polarized pump and probe light, were obtained in coincidence with mass-analyzed Kr ions. The photoelectron angular distributions and branching ratios for direct ionization into the Kr+ 2P3/2 and 2P1/2 spin-orbit continua show considerable dependence on the intermediate level, as well as on the polarizations of the pump and probe light. Photoelectron angular distributions were also recorded with several polarization combinations following two-colour excitation of the (2P1/2)5f[5/2]2 autoionizing resonance. These results are compared with the results of recent work on the corresponding autoionizing resonance in atomic Xe. American Physical Society 2016-03-28 Article PeerReviewed Saquet, N., Holland, D.M.P., Pratt, S.T., Cubaynes, D., Tang, X., Garcia, G.A., Nahon, Laurent and Reid, Katharine L. (2016) Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms. Physical Review A, 93 (3). 033419/1-033419/11. ISSN 1094-1622 http://journals.aps.org/pra/abstract/10.1103/PhysRevA.93.033419 doi:10.1103/PhysRevA.93.033419 doi:10.1103/PhysRevA.93.033419
spellingShingle Saquet, N.
Holland, D.M.P.
Pratt, S.T.
Cubaynes, D.
Tang, X.
Garcia, G.A.
Nahon, Laurent
Reid, Katharine L.
Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms
title Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms
title_full Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms
title_fullStr Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms
title_full_unstemmed Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms
title_short Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms
title_sort effect of electronic angular momentum exchange on photoelectron anisotropy following the two-colour ionization of krypton atoms
url https://eprints.nottingham.ac.uk/32006/
https://eprints.nottingham.ac.uk/32006/
https://eprints.nottingham.ac.uk/32006/