Chitin nanowhisker aerogels

Chitin nanowhiskers are structured into mesoporous aerogels by using the same benign process used previously in our group to make cellulose nanowhisker aerogels. The nanowhiskers are sonicated in water to form a hydrogel before solvent-exchange with ethanol and drying under supercritical CO2 (scCO2)...

Full description

Bibliographic Details
Main Authors: Heath, Lindy, Zhu, Lifan, Thielemans, Wim
Format: Article
Published: Wiley-VCH Verlag 2013
Online Access:https://eprints.nottingham.ac.uk/2830/
_version_ 1848790886987595776
author Heath, Lindy
Zhu, Lifan
Thielemans, Wim
author_facet Heath, Lindy
Zhu, Lifan
Thielemans, Wim
author_sort Heath, Lindy
building Nottingham Research Data Repository
collection Online Access
description Chitin nanowhiskers are structured into mesoporous aerogels by using the same benign process used previously in our group to make cellulose nanowhisker aerogels. The nanowhiskers are sonicated in water to form a hydrogel before solvent-exchange with ethanol and drying under supercritical CO2 (scCO2). Aerogels are prepared with various densities and porosities, relating directly to the initial chitin nanowhisker content. scCO2 drying enables the mesoporous network structure to be retained as well as allowing the gel to retain its initial dimensions. The chitin aerogels have low densities (0.043–0.113 g cm−3), high porosities (up to 97 %), surface areas of up to 261 m2 g−1, and mechanical properties at the high end of other reported values (modulus between 7 and 9.3 MPa). The aerogels were further characterized by using X-ray diffraction, BET analysis, electron microscopy, FTIR, and thermogravimetric analysis. Characterization showed that the rod-like crystalline nature of the nanowhiskers was retained during the aerogel production process, making the aerogel truly an assembled structure of chitin nanocrystals. These aerogels also showed the lowest reported shrinkage during drying to date, with an average shrinkage of only 4 %.
first_indexed 2025-11-14T18:19:45Z
format Article
id nottingham-2830
institution University of Nottingham Malaysia Campus
institution_category Local University
last_indexed 2025-11-14T18:19:45Z
publishDate 2013
publisher Wiley-VCH Verlag
recordtype eprints
repository_type Digital Repository
spelling nottingham-28302020-05-04T16:35:23Z https://eprints.nottingham.ac.uk/2830/ Chitin nanowhisker aerogels Heath, Lindy Zhu, Lifan Thielemans, Wim Chitin nanowhiskers are structured into mesoporous aerogels by using the same benign process used previously in our group to make cellulose nanowhisker aerogels. The nanowhiskers are sonicated in water to form a hydrogel before solvent-exchange with ethanol and drying under supercritical CO2 (scCO2). Aerogels are prepared with various densities and porosities, relating directly to the initial chitin nanowhisker content. scCO2 drying enables the mesoporous network structure to be retained as well as allowing the gel to retain its initial dimensions. The chitin aerogels have low densities (0.043–0.113 g cm−3), high porosities (up to 97 %), surface areas of up to 261 m2 g−1, and mechanical properties at the high end of other reported values (modulus between 7 and 9.3 MPa). The aerogels were further characterized by using X-ray diffraction, BET analysis, electron microscopy, FTIR, and thermogravimetric analysis. Characterization showed that the rod-like crystalline nature of the nanowhiskers was retained during the aerogel production process, making the aerogel truly an assembled structure of chitin nanocrystals. These aerogels also showed the lowest reported shrinkage during drying to date, with an average shrinkage of only 4 %. Wiley-VCH Verlag 2013-01-18 Article PeerReviewed Heath, Lindy, Zhu, Lifan and Thielemans, Wim (2013) Chitin nanowhisker aerogels. ChemSusChem, 6 (3). pp. 537-544. ISSN 1864-5631 http://onlinelibrary.wiley.com/doi/10.1002/cssc.201200717/abstract;jsessionid=D216AEE4AA8DFA30C1B762116A997AD1.f03t02 doi:10.1002/cssc.201200717 doi:10.1002/cssc.201200717
spellingShingle Heath, Lindy
Zhu, Lifan
Thielemans, Wim
Chitin nanowhisker aerogels
title Chitin nanowhisker aerogels
title_full Chitin nanowhisker aerogels
title_fullStr Chitin nanowhisker aerogels
title_full_unstemmed Chitin nanowhisker aerogels
title_short Chitin nanowhisker aerogels
title_sort chitin nanowhisker aerogels
url https://eprints.nottingham.ac.uk/2830/
https://eprints.nottingham.ac.uk/2830/
https://eprints.nottingham.ac.uk/2830/