A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides

We report here a new catalytic reaction in which, p-nitro azides are acylated by aldehydes to produce amides and molecular nitrogen in a single step. The transformation is believed to proceed via an electron transfer process mediated by the tert-butoxide ion, and catalysed by a thiazolium salt deriv...

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Main Authors: Carbone, Giorgio, Burnley, James, Moses, John E.
Format: Article
Published: Royal Society of Chemistry 2013
Online Access:https://eprints.nottingham.ac.uk/2050/
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author Carbone, Giorgio
Burnley, James
Moses, John E.
author_facet Carbone, Giorgio
Burnley, James
Moses, John E.
author_sort Carbone, Giorgio
building Nottingham Research Data Repository
collection Online Access
description We report here a new catalytic reaction in which, p-nitro azides are acylated by aldehydes to produce amides and molecular nitrogen in a single step. The transformation is believed to proceed via an electron transfer process mediated by the tert-butoxide ion, and catalysed by a thiazolium salt derived species.
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publishDate 2013
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spelling nottingham-20502020-05-04T16:35:48Z https://eprints.nottingham.ac.uk/2050/ A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides Carbone, Giorgio Burnley, James Moses, John E. We report here a new catalytic reaction in which, p-nitro azides are acylated by aldehydes to produce amides and molecular nitrogen in a single step. The transformation is believed to proceed via an electron transfer process mediated by the tert-butoxide ion, and catalysed by a thiazolium salt derived species. Royal Society of Chemistry 2013-02-12 Article PeerReviewed Carbone, Giorgio, Burnley, James and Moses, John E. (2013) A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides. Chemical Communications, 49 (27). pp. 2759-2761. ISSN 1364-548X http://pubs.rsc.org/en/Content/ArticleLanding/2013/CC/c3cc40452h doi:10.1039/c3cc40452h doi:10.1039/c3cc40452h
spellingShingle Carbone, Giorgio
Burnley, James
Moses, John E.
A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides
title A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides
title_full A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides
title_fullStr A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides
title_full_unstemmed A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides
title_short A catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides
title_sort catalytic and tert-butoxide ion-mediated amidation of aldehydes with para-nitro azides
url https://eprints.nottingham.ac.uk/2050/
https://eprints.nottingham.ac.uk/2050/
https://eprints.nottingham.ac.uk/2050/