Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves

Tetracera macrophylla is a valuable medicinal plant used traditionally for the treatment of various ailments. The crude ethanol extract was analyzed for its total phenolic and flavonoid contents. 2, 2-diphenyl-1-picrylhydrazyl (DPPH) and 2,2′-azinobis-3-ethylbenzothiazine-6-sulfonic acid (ABTS) were...

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Main Authors: Opeyemi Roheem, Fatimah, Ahmed, Qamar Uddin, Mat So'ad, Siti Zaiton, Ali Shah, Syed Adnan, Latip, Jalifah, Alhassan, Alhassan Muhammad, Syed Mohammad, Sharifah Nurul Akilah
Format: Article
Language:English
English
English
Published: Elsevier GmbH 2020
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Online Access:http://irep.iium.edu.my/80752/
http://irep.iium.edu.my/80752/19/80752_Assessment%20of%20Free%20radical%20scavenging%20and%20digestive_article_new.pdf
http://irep.iium.edu.my/80752/13/80752_Assessment%20of%20Free%20radical%20scavenging%20and%20digestive%20enzyme%20inhibitory_SCOPUS.pdf
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author Opeyemi Roheem, Fatimah
Ahmed, Qamar Uddin
Mat So'ad, Siti Zaiton
Ali Shah, Syed Adnan
Latip, Jalifah
Alhassan, Alhassan Muhammad
Syed Mohammad, Sharifah Nurul Akilah
author_facet Opeyemi Roheem, Fatimah
Ahmed, Qamar Uddin
Mat So'ad, Siti Zaiton
Ali Shah, Syed Adnan
Latip, Jalifah
Alhassan, Alhassan Muhammad
Syed Mohammad, Sharifah Nurul Akilah
author_sort Opeyemi Roheem, Fatimah
building IIUM Repository
collection Online Access
description Tetracera macrophylla is a valuable medicinal plant used traditionally for the treatment of various ailments. The crude ethanol extract was analyzed for its total phenolic and flavonoid contents. 2, 2-diphenyl-1-picrylhydrazyl (DPPH) and 2,2′-azinobis-3-ethylbenzothiazine-6-sulfonic acid (ABTS) were used to examine the free radical scavenging capacity while enzyme inhibitory activity was assessed using α-amylase and α-glucosidase inhibitory methods. The crude extract was found to be rich in both phenolic and flavonoid contents (417.90 and5.86 μg GAE and QUE/mg dry weight, respectively) thus exhibited good radical scavenging activity on DPPH and ABTS radicals (IC50 values of 16.2 and 14.65 μg/mL, respectively). It also showed a promising concentration dependent enzymes inhibitory activity against α-amylase and α-glucosidase with IC50 of 72.17 and 76.16 μg/mL, respectively. Fractionation of active ethanol extract of T. macrophylla leaves through liquid-liquid partitioning yielded fractions Fa, Fb, Fc, and Fd. Among all the fractions, Fb (ethyl acetate fraction) showed the highest phenolic and flavonoid contents (206.34 μg/ GAE and 4.01 μg/ QUE respectively) and was also found to exhibit highest antioxidant and α-glucosidase inhibitory activities. The most active fraction, Fb upon purification yielded five compounds which were characterized and identified through different spectroscopic techniques. FTQ-4 among the compounds exhibited the strongest free radical and enzyme inhibitory activities followed by FTQ-3. All the compounds were isolated from this plant for the first time and found active against free radicals and/or digestive enzymes.These results further suggest the medicinal potential of T. macrophylla leaves as a therapeutic agent against hyperglycemia and free radical associated problems.
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institution International Islamic University Malaysia
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publishDate 2020
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spelling iium-807522021-05-06T03:43:42Z http://irep.iium.edu.my/80752/ Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves Opeyemi Roheem, Fatimah Ahmed, Qamar Uddin Mat So'ad, Siti Zaiton Ali Shah, Syed Adnan Latip, Jalifah Alhassan, Alhassan Muhammad Syed Mohammad, Sharifah Nurul Akilah QD Chemistry Tetracera macrophylla is a valuable medicinal plant used traditionally for the treatment of various ailments. The crude ethanol extract was analyzed for its total phenolic and flavonoid contents. 2, 2-diphenyl-1-picrylhydrazyl (DPPH) and 2,2′-azinobis-3-ethylbenzothiazine-6-sulfonic acid (ABTS) were used to examine the free radical scavenging capacity while enzyme inhibitory activity was assessed using α-amylase and α-glucosidase inhibitory methods. The crude extract was found to be rich in both phenolic and flavonoid contents (417.90 and5.86 μg GAE and QUE/mg dry weight, respectively) thus exhibited good radical scavenging activity on DPPH and ABTS radicals (IC50 values of 16.2 and 14.65 μg/mL, respectively). It also showed a promising concentration dependent enzymes inhibitory activity against α-amylase and α-glucosidase with IC50 of 72.17 and 76.16 μg/mL, respectively. Fractionation of active ethanol extract of T. macrophylla leaves through liquid-liquid partitioning yielded fractions Fa, Fb, Fc, and Fd. Among all the fractions, Fb (ethyl acetate fraction) showed the highest phenolic and flavonoid contents (206.34 μg/ GAE and 4.01 μg/ QUE respectively) and was also found to exhibit highest antioxidant and α-glucosidase inhibitory activities. The most active fraction, Fb upon purification yielded five compounds which were characterized and identified through different spectroscopic techniques. FTQ-4 among the compounds exhibited the strongest free radical and enzyme inhibitory activities followed by FTQ-3. All the compounds were isolated from this plant for the first time and found active against free radicals and/or digestive enzymes.These results further suggest the medicinal potential of T. macrophylla leaves as a therapeutic agent against hyperglycemia and free radical associated problems. Elsevier GmbH 2020-04-06 Article PeerReviewed application/pdf en http://irep.iium.edu.my/80752/19/80752_Assessment%20of%20Free%20radical%20scavenging%20and%20digestive_article_new.pdf application/pdf en http://irep.iium.edu.my/80752/13/80752_Assessment%20of%20Free%20radical%20scavenging%20and%20digestive%20enzyme%20inhibitory_SCOPUS.pdf application/pdf en http://irep.iium.edu.my/80752/20/80752_Assessment%20of%20Free%20radical%20scavenging%20and%20digestive_wos.pdf Opeyemi Roheem, Fatimah and Ahmed, Qamar Uddin and Mat So'ad, Siti Zaiton and Ali Shah, Syed Adnan and Latip, Jalifah and Alhassan, Alhassan Muhammad and Syed Mohammad, Sharifah Nurul Akilah (2020) Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves. Journal of Herbal Medicine, 22. pp. 1-8. ISSN 2210-8033 https://www.sciencedirect.com/science/article/abs/pii/S2210803320300233 10.1016/j.hermed.2020.100351
spellingShingle QD Chemistry
Opeyemi Roheem, Fatimah
Ahmed, Qamar Uddin
Mat So'ad, Siti Zaiton
Ali Shah, Syed Adnan
Latip, Jalifah
Alhassan, Alhassan Muhammad
Syed Mohammad, Sharifah Nurul Akilah
Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves
title Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves
title_full Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves
title_fullStr Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves
title_full_unstemmed Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves
title_short Assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from Tetracera macrophylla leaves
title_sort assessment of free radical scavenging and digestive enzyme inhibitory activities of extract, fractions and isolated compounds from tetracera macrophylla leaves
topic QD Chemistry
url http://irep.iium.edu.my/80752/
http://irep.iium.edu.my/80752/
http://irep.iium.edu.my/80752/
http://irep.iium.edu.my/80752/19/80752_Assessment%20of%20Free%20radical%20scavenging%20and%20digestive_article_new.pdf
http://irep.iium.edu.my/80752/13/80752_Assessment%20of%20Free%20radical%20scavenging%20and%20digestive%20enzyme%20inhibitory_SCOPUS.pdf
http://irep.iium.edu.my/80752/20/80752_Assessment%20of%20Free%20radical%20scavenging%20and%20digestive_wos.pdf