Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol

The effect of metals on support material fluorine-doped tin oxide (FTO), were studied. A series of metals such as ruthenium (Ru), osmium (Os), palladium (Pd), and copper (Cu) on FTO support were prepared by a simple wet mixture method, and attempted as a heterogeneous catalyst to enhance the hydroge...

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Main Authors: Samad, Wan Zurina, Wan Isahak, Wan Nor Roslam, Hamzah, Noraini, Yarmo, Mohd Ambar, Yusop, Muhammad Rahimi
Format: Proceeding Paper
Language:English
English
Published: Trans Tech. Publications 2017
Subjects:
Online Access:http://irep.iium.edu.my/56699/
http://irep.iium.edu.my/56699/13/56699_Effect%20of%20metals%20compatibility%20on%20fluorine-doped.pdf
http://irep.iium.edu.my/56699/24/56699-Effect%20of%20metals%20compatibility%20on%20fluorine-doped%20tin-SCOPUS.pdf
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author Samad, Wan Zurina
Wan Isahak, Wan Nor Roslam
Hamzah, Noraini
Yarmo, Mohd Ambar
Yusop, Muhammad Rahimi
author_facet Samad, Wan Zurina
Wan Isahak, Wan Nor Roslam
Hamzah, Noraini
Yarmo, Mohd Ambar
Yusop, Muhammad Rahimi
author_sort Samad, Wan Zurina
building IIUM Repository
collection Online Access
description The effect of metals on support material fluorine-doped tin oxide (FTO), were studied. A series of metals such as ruthenium (Ru), osmium (Os), palladium (Pd), and copper (Cu) on FTO support were prepared by a simple wet mixture method, and attempted as a heterogeneous catalyst to enhance the hydrogenolysis of glycerol converted to 1,2-propanediol (1,2-PDO). The physicochemical properties of the catalysts were characterized by XRD, XPS, BET, FESEM, TEM, TPR, and TPD techniques. In particular, the catalyst of Ru-FTO was recorded as a good catalyst with an optimum glycerol conversion of 100% and 1,2-PDO selectivity of 94% respectively. It was suggesting that the acid an basic properties of the catalyst could achieved the C-O and C-H bond dissociation by formation of different intermediates of acetol and acetaldehyde to become 1,2-PDO. Despite that, some reaction parameters were evaluated and optimized reaction condition were established
first_indexed 2025-11-14T16:42:52Z
format Proceeding Paper
id iium-56699
institution International Islamic University Malaysia
institution_category Local University
language English
English
last_indexed 2025-11-14T16:42:52Z
publishDate 2017
publisher Trans Tech. Publications
recordtype eprints
repository_type Digital Repository
spelling iium-566992018-03-15T09:33:24Z http://irep.iium.edu.my/56699/ Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol Samad, Wan Zurina Wan Isahak, Wan Nor Roslam Hamzah, Noraini Yarmo, Mohd Ambar Yusop, Muhammad Rahimi Q Science (General) The effect of metals on support material fluorine-doped tin oxide (FTO), were studied. A series of metals such as ruthenium (Ru), osmium (Os), palladium (Pd), and copper (Cu) on FTO support were prepared by a simple wet mixture method, and attempted as a heterogeneous catalyst to enhance the hydrogenolysis of glycerol converted to 1,2-propanediol (1,2-PDO). The physicochemical properties of the catalysts were characterized by XRD, XPS, BET, FESEM, TEM, TPR, and TPD techniques. In particular, the catalyst of Ru-FTO was recorded as a good catalyst with an optimum glycerol conversion of 100% and 1,2-PDO selectivity of 94% respectively. It was suggesting that the acid an basic properties of the catalyst could achieved the C-O and C-H bond dissociation by formation of different intermediates of acetol and acetaldehyde to become 1,2-PDO. Despite that, some reaction parameters were evaluated and optimized reaction condition were established Trans Tech. Publications 2017-03 Proceeding Paper PeerReviewed application/pdf en http://irep.iium.edu.my/56699/13/56699_Effect%20of%20metals%20compatibility%20on%20fluorine-doped.pdf application/pdf en http://irep.iium.edu.my/56699/24/56699-Effect%20of%20metals%20compatibility%20on%20fluorine-doped%20tin-SCOPUS.pdf Samad, Wan Zurina and Wan Isahak, Wan Nor Roslam and Hamzah, Noraini and Yarmo, Mohd Ambar and Yusop, Muhammad Rahimi (2017) Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol. In: International Conference on X-Rays and Related Techniques in Research and Industry, ICXRI 2016, 17th-18th August, 2016, Dorsett Hotel, Putrajaya. https://www.scientific.net/MSF.888.496 10.4028/www.scientific.net/MSF.888.496
spellingShingle Q Science (General)
Samad, Wan Zurina
Wan Isahak, Wan Nor Roslam
Hamzah, Noraini
Yarmo, Mohd Ambar
Yusop, Muhammad Rahimi
Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol
title Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol
title_full Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol
title_fullStr Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol
title_full_unstemmed Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol
title_short Effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-Propanediol
title_sort effect of metals compatibility on fluorine-doped tin oxide catalyst for glycerol conversion to 1,2-propanediol
topic Q Science (General)
url http://irep.iium.edu.my/56699/
http://irep.iium.edu.my/56699/
http://irep.iium.edu.my/56699/
http://irep.iium.edu.my/56699/13/56699_Effect%20of%20metals%20compatibility%20on%20fluorine-doped.pdf
http://irep.iium.edu.my/56699/24/56699-Effect%20of%20metals%20compatibility%20on%20fluorine-doped%20tin-SCOPUS.pdf