Nanoscale distribution of Ge in Cu-rich sphalerite

A large proportion of the critical elements resources Ge, Ga, and In are associated with sphalerite in Pb-Zn ore deposits. Germanium in sphalerite has been proposed to be structurally bound in the crystal lattice. Using a combination of microstructural, geochemical and nanoscale observations, we sho...

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Main Authors: Fougerouse, Denis, Cugerone, A., Reddy, Steven, Luo, K., Motto-Ros, V.
Format: Journal Article
Published: 2023
Online Access:text
http://hdl.handle.net/20.500.11937/94712
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author Fougerouse, Denis
Cugerone, A.
Reddy, Steven
Luo, K.
Motto-Ros, V.
author_facet Fougerouse, Denis
Cugerone, A.
Reddy, Steven
Luo, K.
Motto-Ros, V.
author_sort Fougerouse, Denis
building Curtin Institutional Repository
collection Online Access
description A large proportion of the critical elements resources Ge, Ga, and In are associated with sphalerite in Pb-Zn ore deposits. Germanium in sphalerite has been proposed to be structurally bound in the crystal lattice. Using a combination of microstructural, geochemical and nanoscale observations, we show that Ge can be hosted in sphalerite crystal structure as well as nanoparticles of briartite (Cu2(Zn,Fe)GeS4). The structurally-bound Ge was preserved in undeformed sphalerite grains from the Saint-Salvy Pb-Zn vein deposit (France), whereas the briartite nanoparticles were observed in metamorphosed sphalerite from Arre. The briartite nanoparticles likely exsolved from sphalerite during the Pyrenean-Alpine metamorphism and deformation. The presence of nanoparticles may harden the sphalerite during crystal-plastic deformation and help to preserve the critical elements resources of Pb-Zn deposits during metamorphism.
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spelling curtin-20.500.11937-947122024-04-16T06:05:12Z Nanoscale distribution of Ge in Cu-rich sphalerite Fougerouse, Denis Cugerone, A. Reddy, Steven Luo, K. Motto-Ros, V. A large proportion of the critical elements resources Ge, Ga, and In are associated with sphalerite in Pb-Zn ore deposits. Germanium in sphalerite has been proposed to be structurally bound in the crystal lattice. Using a combination of microstructural, geochemical and nanoscale observations, we show that Ge can be hosted in sphalerite crystal structure as well as nanoparticles of briartite (Cu2(Zn,Fe)GeS4). The structurally-bound Ge was preserved in undeformed sphalerite grains from the Saint-Salvy Pb-Zn vein deposit (France), whereas the briartite nanoparticles were observed in metamorphosed sphalerite from Arre. The briartite nanoparticles likely exsolved from sphalerite during the Pyrenean-Alpine metamorphism and deformation. The presence of nanoparticles may harden the sphalerite during crystal-plastic deformation and help to preserve the critical elements resources of Pb-Zn deposits during metamorphism. 2023 Journal Article http://hdl.handle.net/20.500.11937/94712 10.1016/j.gca.2023.02.011 text http://purl.org/au-research/grants/arc/DE190101307 http://creativecommons.org/licenses/by-nc-nd/4.0/ fulltext
spellingShingle Fougerouse, Denis
Cugerone, A.
Reddy, Steven
Luo, K.
Motto-Ros, V.
Nanoscale distribution of Ge in Cu-rich sphalerite
title Nanoscale distribution of Ge in Cu-rich sphalerite
title_full Nanoscale distribution of Ge in Cu-rich sphalerite
title_fullStr Nanoscale distribution of Ge in Cu-rich sphalerite
title_full_unstemmed Nanoscale distribution of Ge in Cu-rich sphalerite
title_short Nanoscale distribution of Ge in Cu-rich sphalerite
title_sort nanoscale distribution of ge in cu-rich sphalerite
url text
text
http://hdl.handle.net/20.500.11937/94712