Preparation and toughening mechanism of Al2O3 composite ceramic toughened by B4C@TiB2 core–shell units

In this paper, the concept of incorporating core–shell structured units as secondary phases to toughen Al2O3 ceramics is proposed. Al2O3 composite ceramics toughened by B4C@TiB2 core–shell units are successfully synthesized using a combination of molten salt methodology and spark plasma sintering. T...

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Main Authors: Shi, Yingjie, Li, Weixing, Zhang, Xiaorong, Jin, Jiachao, Wang, Jilin, Dong, Yu, Mu, Jingbo, Wang, Guangsuo, Zhang, Xiaoliang, Zhang, Zhixiao
Format: Journal Article
Language:English
Published: Tsinghua University Press Ltd 2023
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/94122
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author Shi, Yingjie
Li, Weixing
Zhang, Xiaorong
Jin, Jiachao
Wang, Jilin
Dong, Yu
Mu, Jingbo
Wang, Guangsuo
Zhang, Xiaoliang
Zhang, Zhixiao
author_facet Shi, Yingjie
Li, Weixing
Zhang, Xiaorong
Jin, Jiachao
Wang, Jilin
Dong, Yu
Mu, Jingbo
Wang, Guangsuo
Zhang, Xiaoliang
Zhang, Zhixiao
author_sort Shi, Yingjie
building Curtin Institutional Repository
collection Online Access
description In this paper, the concept of incorporating core–shell structured units as secondary phases to toughen Al2O3 ceramics is proposed. Al2O3 composite ceramics toughened by B4C@TiB2 core–shell units are successfully synthesized using a combination of molten salt methodology and spark plasma sintering. The synthesis of B4C@TiB2 core–shell toughening units stems from the prior production of core–shell structural B4C@TiB2 powders, and this core–shell structure is effectively preserved within the Al2O3 matrix after sintering. The B4C@TiB2 core–shell toughening unit consists of a micron-sized B4C core enclosed by a shell approximately 500 nm in thickness, composed of numerous nanosized TiB2 grains. The regions surrounding these core–shell units exhibit distinct geometric structures and encompass multidimensional variations in phase composition, grain dimensions, and thermal expansion coefficients. Consequently, intricate stress distributions emerge, fostering the propagation of cracks in multiple dimensions. This behavior consumes a considerable amount of crack propagation energy, thereby enhancing the fracture toughness of the Al2O3 matrix. The resulting Al2O3 composite ceramics display relative density of 99.7%±0.2%, Vickers hardness of 21.5±0.8 GPa, and fracture toughness 6.92±0.22 MPa·m1/2.
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spelling curtin-20.500.11937-941222024-01-30T07:30:42Z Preparation and toughening mechanism of Al2O3 composite ceramic toughened by B4C@TiB2 core–shell units Shi, Yingjie Li, Weixing Zhang, Xiaorong Jin, Jiachao Wang, Jilin Dong, Yu Mu, Jingbo Wang, Guangsuo Zhang, Xiaoliang Zhang, Zhixiao Al2O3 composite ceramics core–shell structure microstructure design spark plasma sintering toughening mechanism In this paper, the concept of incorporating core–shell structured units as secondary phases to toughen Al2O3 ceramics is proposed. Al2O3 composite ceramics toughened by B4C@TiB2 core–shell units are successfully synthesized using a combination of molten salt methodology and spark plasma sintering. The synthesis of B4C@TiB2 core–shell toughening units stems from the prior production of core–shell structural B4C@TiB2 powders, and this core–shell structure is effectively preserved within the Al2O3 matrix after sintering. The B4C@TiB2 core–shell toughening unit consists of a micron-sized B4C core enclosed by a shell approximately 500 nm in thickness, composed of numerous nanosized TiB2 grains. The regions surrounding these core–shell units exhibit distinct geometric structures and encompass multidimensional variations in phase composition, grain dimensions, and thermal expansion coefficients. Consequently, intricate stress distributions emerge, fostering the propagation of cracks in multiple dimensions. This behavior consumes a considerable amount of crack propagation energy, thereby enhancing the fracture toughness of the Al2O3 matrix. The resulting Al2O3 composite ceramics display relative density of 99.7%±0.2%, Vickers hardness of 21.5±0.8 GPa, and fracture toughness 6.92±0.22 MPa·m1/2. 2023 Journal Article http://hdl.handle.net/20.500.11937/94122 10.26599/JAC.2023.9220826 English http://creativecommons.org/licenses/by/4.0/ Tsinghua University Press Ltd fulltext
spellingShingle Al2O3 composite ceramics
core–shell structure
microstructure design
spark plasma sintering
toughening mechanism
Shi, Yingjie
Li, Weixing
Zhang, Xiaorong
Jin, Jiachao
Wang, Jilin
Dong, Yu
Mu, Jingbo
Wang, Guangsuo
Zhang, Xiaoliang
Zhang, Zhixiao
Preparation and toughening mechanism of Al2O3 composite ceramic toughened by B4C@TiB2 core–shell units
title Preparation and toughening mechanism of Al2O3 composite ceramic toughened by B4C@TiB2 core–shell units
title_full Preparation and toughening mechanism of Al2O3 composite ceramic toughened by B4C@TiB2 core–shell units
title_fullStr Preparation and toughening mechanism of Al2O3 composite ceramic toughened by B4C@TiB2 core–shell units
title_full_unstemmed Preparation and toughening mechanism of Al2O3 composite ceramic toughened by B4C@TiB2 core–shell units
title_short Preparation and toughening mechanism of Al2O3 composite ceramic toughened by B4C@TiB2 core–shell units
title_sort preparation and toughening mechanism of al2o3 composite ceramic toughened by b4c@tib2 core–shell units
topic Al2O3 composite ceramics
core–shell structure
microstructure design
spark plasma sintering
toughening mechanism
url http://hdl.handle.net/20.500.11937/94122