High-Quality Ruddlesden–Popper Perovskite Film Formation for High-Performance Perovskite Solar Cells
In the last decade, perovskite solar cells (PSCs) have undergone unprecedented rapid development and become a promising candidate for a new-generation solar cell. Among various PSCs, typical 3D halide perovskite-based PSCs deliver the highest efficiency but they suffer from severe instability, which...
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| Format: | Journal Article |
| Language: | English |
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WILEY-V C H VERLAG GMBH
2021
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| Online Access: | https://onlinelibrary.wiley.com/doi/am-pdf/10.1002/adma.202002582 http://hdl.handle.net/20.500.11937/91961 |
| _version_ | 1848765606405341184 |
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| author | Liu, P. Han, N. Wang, Wei Ran, R. Zhou, W. Shao, Zongping |
| author_facet | Liu, P. Han, N. Wang, Wei Ran, R. Zhou, W. Shao, Zongping |
| author_sort | Liu, P. |
| building | Curtin Institutional Repository |
| collection | Online Access |
| description | In the last decade, perovskite solar cells (PSCs) have undergone unprecedented rapid development and become a promising candidate for a new-generation solar cell. Among various PSCs, typical 3D halide perovskite-based PSCs deliver the highest efficiency but they suffer from severe instability, which restricts their practical applications. By contrast, the low-dimensional Ruddlesden–Popper (RP) perovskite-based PSCs have recently raised increasing attention due to their superior stability. Yet, the efficiency of RP perovskite-based PSCs is still far from that of the 3D counterparts owing to the difficulty in fabricating high-quality RP perovskite films. In pursuit of high-efficiency RP perovskite-based PSCs, it is critical to manipulate the film formation process to prepare high-quality RP perovskite films. This review aims to provide comprehensive understanding of the high-quality RP-type perovskite film formation by investigating the influential factors. On this basis, several strategies to improve the RP perovskite film quality are proposed via summarizing the recent progress and efforts on the preparation of high-quality RP perovskite film. This review will provide useful guidelines for a better understanding of the crystallization and phase kinetics during RP perovskite film formation process and the design and development of high-performance RP perovskite-based PSCs, promoting the commercialization of PSC technology. |
| first_indexed | 2025-11-14T11:37:55Z |
| format | Journal Article |
| id | curtin-20.500.11937-91961 |
| institution | Curtin University Malaysia |
| institution_category | Local University |
| language | English |
| last_indexed | 2025-11-14T11:37:55Z |
| publishDate | 2021 |
| publisher | WILEY-V C H VERLAG GMBH |
| recordtype | eprints |
| repository_type | Digital Repository |
| spelling | curtin-20.500.11937-919612023-06-08T06:34:16Z High-Quality Ruddlesden–Popper Perovskite Film Formation for High-Performance Perovskite Solar Cells Liu, P. Han, N. Wang, Wei Ran, R. Zhou, W. Shao, Zongping Science & Technology Physical Sciences Technology Chemistry, Multidisciplinary Chemistry, Physical Nanoscience & Nanotechnology Materials Science, Multidisciplinary Physics, Applied Physics, Condensed Matter Chemistry Science & Technology - Other Topics Materials Science Physics low dimensional perovskite perovskite film quality perovskite solar cells power conversion efficiency Ruddlesden-Popper perovskite LAYERED HYBRID PEROVSKITES METAL HALIDE PEROVSKITES LEAD IODIDE PEROVSKITES QUASI-2-DIMENSIONAL PEROVSKITE 2D PEROVSKITES THIN-FILMS VERTICAL ORIENTATION ENHANCED EFFICIENCY PHASE-TRANSITIONS CARRIER DYNAMICS Ruddlesden-Popper perovskite low dimensional perovskite perovskite film quality perovskite solar cells power conversion efficiency In the last decade, perovskite solar cells (PSCs) have undergone unprecedented rapid development and become a promising candidate for a new-generation solar cell. Among various PSCs, typical 3D halide perovskite-based PSCs deliver the highest efficiency but they suffer from severe instability, which restricts their practical applications. By contrast, the low-dimensional Ruddlesden–Popper (RP) perovskite-based PSCs have recently raised increasing attention due to their superior stability. Yet, the efficiency of RP perovskite-based PSCs is still far from that of the 3D counterparts owing to the difficulty in fabricating high-quality RP perovskite films. In pursuit of high-efficiency RP perovskite-based PSCs, it is critical to manipulate the film formation process to prepare high-quality RP perovskite films. This review aims to provide comprehensive understanding of the high-quality RP-type perovskite film formation by investigating the influential factors. On this basis, several strategies to improve the RP perovskite film quality are proposed via summarizing the recent progress and efforts on the preparation of high-quality RP perovskite film. This review will provide useful guidelines for a better understanding of the crystallization and phase kinetics during RP perovskite film formation process and the design and development of high-performance RP perovskite-based PSCs, promoting the commercialization of PSC technology. 2021 Journal Article http://hdl.handle.net/20.500.11937/91961 10.1002/adma.202002582 English https://onlinelibrary.wiley.com/doi/am-pdf/10.1002/adma.202002582 http://purl.org/au-research/grants/arc/DP150104365 http://purl.org/au-research/grants/arc/DP160104835 WILEY-V C H VERLAG GMBH unknown |
| spellingShingle | Science & Technology Physical Sciences Technology Chemistry, Multidisciplinary Chemistry, Physical Nanoscience & Nanotechnology Materials Science, Multidisciplinary Physics, Applied Physics, Condensed Matter Chemistry Science & Technology - Other Topics Materials Science Physics low dimensional perovskite perovskite film quality perovskite solar cells power conversion efficiency Ruddlesden-Popper perovskite LAYERED HYBRID PEROVSKITES METAL HALIDE PEROVSKITES LEAD IODIDE PEROVSKITES QUASI-2-DIMENSIONAL PEROVSKITE 2D PEROVSKITES THIN-FILMS VERTICAL ORIENTATION ENHANCED EFFICIENCY PHASE-TRANSITIONS CARRIER DYNAMICS Ruddlesden-Popper perovskite low dimensional perovskite perovskite film quality perovskite solar cells power conversion efficiency Liu, P. Han, N. Wang, Wei Ran, R. Zhou, W. Shao, Zongping High-Quality Ruddlesden–Popper Perovskite Film Formation for High-Performance Perovskite Solar Cells |
| title | High-Quality Ruddlesden–Popper Perovskite Film Formation for High-Performance Perovskite Solar Cells |
| title_full | High-Quality Ruddlesden–Popper Perovskite Film Formation for High-Performance Perovskite Solar Cells |
| title_fullStr | High-Quality Ruddlesden–Popper Perovskite Film Formation for High-Performance Perovskite Solar Cells |
| title_full_unstemmed | High-Quality Ruddlesden–Popper Perovskite Film Formation for High-Performance Perovskite Solar Cells |
| title_short | High-Quality Ruddlesden–Popper Perovskite Film Formation for High-Performance Perovskite Solar Cells |
| title_sort | high-quality ruddlesden–popper perovskite film formation for high-performance perovskite solar cells |
| topic | Science & Technology Physical Sciences Technology Chemistry, Multidisciplinary Chemistry, Physical Nanoscience & Nanotechnology Materials Science, Multidisciplinary Physics, Applied Physics, Condensed Matter Chemistry Science & Technology - Other Topics Materials Science Physics low dimensional perovskite perovskite film quality perovskite solar cells power conversion efficiency Ruddlesden-Popper perovskite LAYERED HYBRID PEROVSKITES METAL HALIDE PEROVSKITES LEAD IODIDE PEROVSKITES QUASI-2-DIMENSIONAL PEROVSKITE 2D PEROVSKITES THIN-FILMS VERTICAL ORIENTATION ENHANCED EFFICIENCY PHASE-TRANSITIONS CARRIER DYNAMICS Ruddlesden-Popper perovskite low dimensional perovskite perovskite film quality perovskite solar cells power conversion efficiency |
| url | https://onlinelibrary.wiley.com/doi/am-pdf/10.1002/adma.202002582 https://onlinelibrary.wiley.com/doi/am-pdf/10.1002/adma.202002582 https://onlinelibrary.wiley.com/doi/am-pdf/10.1002/adma.202002582 http://hdl.handle.net/20.500.11937/91961 |