Standardizing Spatial Reconstruction Parameters for the Atom Probe Analysis of Common Minerals

Well-defined reconstruction parameters are essential to quantify the size, shape, and distribution of nanoscale features in atom probe tomography (APT) datasets. However, the reconstruction parameters of many minerals are difficult to estimate because intrinsic spatial markers, such as crystallograp...

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Main Authors: Fougerouse, Denis, Saxey, David, Rickard, William, Reddy, Steven, Verberne, R.
Format: Journal Article
Language:English
Published: CAMBRIDGE UNIV PRESS 2022
Subjects:
Online Access:http://purl.org/au-research/grants/arc/DE190101307
http://hdl.handle.net/20.500.11937/91633
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author Fougerouse, Denis
Saxey, David
Rickard, William
Reddy, Steven
Verberne, R.
author_facet Fougerouse, Denis
Saxey, David
Rickard, William
Reddy, Steven
Verberne, R.
author_sort Fougerouse, Denis
building Curtin Institutional Repository
collection Online Access
description Well-defined reconstruction parameters are essential to quantify the size, shape, and distribution of nanoscale features in atom probe tomography (APT) datasets. However, the reconstruction parameters of many minerals are difficult to estimate because intrinsic spatial markers, such as crystallographic planes, are not usually present within the datasets themselves. Using transmission and/or scanning electron microscopy imaging of needle-shaped specimens before and after atom probe analysis, we test various approaches to provide best-fit reconstruction parameters for voltage-based APT reconstructions. The results demonstrate that the length measurement of evaporated material, constrained by overlaying pre-and post-analysis images, yields more consistent reconstruction parameters than the measurement of final tip radius. Using this approach, we provide standardized parameters that may be used in APT reconstructions of 11 minerals. The adoption of standardized reconstruction parameters by the geoscience APT community will alleviate potential problems in the measurement of nanoscale features (e.g., clusters and interfaces) caused by the use of inappropriate parameters.
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spelling curtin-20.500.11937-916332023-05-18T02:36:21Z Standardizing Spatial Reconstruction Parameters for the Atom Probe Analysis of Common Minerals Fougerouse, Denis Saxey, David Rickard, William Reddy, Steven Verberne, R. Science & Technology Technology Materials Science, Multidisciplinary Microscopy Materials Science atom probe microscopy correlative microscopy mineralogy nanoscale U-PB TOMOGRAPHY MONAZITE GOLD APATITE ZIRCON DEPENDENCE XENOTIME TITANITE CALCIUM Well-defined reconstruction parameters are essential to quantify the size, shape, and distribution of nanoscale features in atom probe tomography (APT) datasets. However, the reconstruction parameters of many minerals are difficult to estimate because intrinsic spatial markers, such as crystallographic planes, are not usually present within the datasets themselves. Using transmission and/or scanning electron microscopy imaging of needle-shaped specimens before and after atom probe analysis, we test various approaches to provide best-fit reconstruction parameters for voltage-based APT reconstructions. The results demonstrate that the length measurement of evaporated material, constrained by overlaying pre-and post-analysis images, yields more consistent reconstruction parameters than the measurement of final tip radius. Using this approach, we provide standardized parameters that may be used in APT reconstructions of 11 minerals. The adoption of standardized reconstruction parameters by the geoscience APT community will alleviate potential problems in the measurement of nanoscale features (e.g., clusters and interfaces) caused by the use of inappropriate parameters. 2022 Journal Article http://hdl.handle.net/20.500.11937/91633 10.1017/S1431927621013714 English http://purl.org/au-research/grants/arc/DE190101307 http://purl.org/au-research/grants/arc/DP210102625 http://purl.org/au-research/grants/arc/LE190100176 CAMBRIDGE UNIV PRESS restricted
spellingShingle Science & Technology
Technology
Materials Science, Multidisciplinary
Microscopy
Materials Science
atom probe microscopy
correlative microscopy
mineralogy
nanoscale
U-PB
TOMOGRAPHY
MONAZITE
GOLD
APATITE
ZIRCON
DEPENDENCE
XENOTIME
TITANITE
CALCIUM
Fougerouse, Denis
Saxey, David
Rickard, William
Reddy, Steven
Verberne, R.
Standardizing Spatial Reconstruction Parameters for the Atom Probe Analysis of Common Minerals
title Standardizing Spatial Reconstruction Parameters for the Atom Probe Analysis of Common Minerals
title_full Standardizing Spatial Reconstruction Parameters for the Atom Probe Analysis of Common Minerals
title_fullStr Standardizing Spatial Reconstruction Parameters for the Atom Probe Analysis of Common Minerals
title_full_unstemmed Standardizing Spatial Reconstruction Parameters for the Atom Probe Analysis of Common Minerals
title_short Standardizing Spatial Reconstruction Parameters for the Atom Probe Analysis of Common Minerals
title_sort standardizing spatial reconstruction parameters for the atom probe analysis of common minerals
topic Science & Technology
Technology
Materials Science, Multidisciplinary
Microscopy
Materials Science
atom probe microscopy
correlative microscopy
mineralogy
nanoscale
U-PB
TOMOGRAPHY
MONAZITE
GOLD
APATITE
ZIRCON
DEPENDENCE
XENOTIME
TITANITE
CALCIUM
url http://purl.org/au-research/grants/arc/DE190101307
http://purl.org/au-research/grants/arc/DE190101307
http://purl.org/au-research/grants/arc/DE190101307
http://hdl.handle.net/20.500.11937/91633