Toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface

Biodiesel is created through the transesterification of fats/oils and its usage is increasing worldwide as global warming concerns increase. Biodiesel fuel properties change depending on the feedstock used to create it. The aim of this study was to assess the different toxicological properties of bi...

Full description

Bibliographic Details
Main Authors: Landwehr, K.R., Hillas, J., Mead-Hunter, Ryan, King, A., O'Leary, R.A., Kicic, Anthony, Mullins, Ben, Larcombe, Alexander
Format: Journal Article
Language:English
Published: ELSEVIER 2022
Subjects:
Online Access:https://www.sciencedirect.com/science/article/am/pii/S004896972202109X
http://hdl.handle.net/20.500.11937/91632
_version_ 1848765564073279488
author Landwehr, K.R.
Hillas, J.
Mead-Hunter, Ryan
King, A.
O'Leary, R.A.
Kicic, Anthony
Mullins, Ben
Larcombe, Alexander
author_facet Landwehr, K.R.
Hillas, J.
Mead-Hunter, Ryan
King, A.
O'Leary, R.A.
Kicic, Anthony
Mullins, Ben
Larcombe, Alexander
author_sort Landwehr, K.R.
building Curtin Institutional Repository
collection Online Access
description Biodiesel is created through the transesterification of fats/oils and its usage is increasing worldwide as global warming concerns increase. Biodiesel fuel properties change depending on the feedstock used to create it. The aim of this study was to assess the different toxicological properties of biodiesel exhausts created from different feedstocks using a complex 3D air-liquid interface (ALI) model that mimics the human airway. Primary human airway epithelial cells were grown at ALI until full differentiation was achieved. Cells were then exposed to 1/20 diluted exhaust from an engine running on Diesel (ULSD), pure or 20% blended Canola biodiesel and pure or 20% blended Tallow biodiesel, or Air for control. Exhaust was analysed for various physio-chemical properties and 24-h after exposure, ALI cultures were assessed for permeability, protein release and mediator response. All measured exhaust components were within industry safety standards. ULSD contained the highest concentrations of various combustion gases. We found no differences in terms of particle characteristics for any of the tested exhausts, likely due to the high dilution used. Exposure to Tallow B100 and B20 induced increased permeability in the ALI culture and the greatest increase in mediator response in both the apical and basal compartments. In contrast, Canola B100 and B20 did not impact permeability and induced the smallest mediator response. All exhausts but Canola B20 induced increased protein release, indicating epithelial damage. Despite the concentrations of all exhausts used in this study meeting industry safety regulations, we found significant toxic effects. Tallow biodiesel was found to be the most toxic of the tested fuels and Canola the least, both for blended and pure biodiesel fuels. This suggests that the feedstock biodiesel is made from is crucial for the resulting health effects of exhaust exposure, even when not comprising the majority of fuel composition.
first_indexed 2025-11-14T11:37:15Z
format Journal Article
id curtin-20.500.11937-91632
institution Curtin University Malaysia
institution_category Local University
language English
last_indexed 2025-11-14T11:37:15Z
publishDate 2022
publisher ELSEVIER
recordtype eprints
repository_type Digital Repository
spelling curtin-20.500.11937-916322024-02-06T04:54:59Z Toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface Landwehr, K.R. Hillas, J. Mead-Hunter, Ryan King, A. O'Leary, R.A. Kicic, Anthony Mullins, Ben Larcombe, Alexander Science & Technology Life Sciences & Biomedicine Environmental Sciences Environmental Sciences & Ecology Exhaust toxicology Biodiesel health effects Air-liquid Interface Exhaust exposure Biodiesel exhaust Primary human cell culture 28-DAY INHALATION EXPOSURE DIESEL-ENGINE EXHAUST OXIDATIVE STRESS PARTICULATE MATTER 2ND-GENERATION BIODIESEL IN-VITRO SYSTEMIC INFLAMMATION BARRIER INTEGRITY TREATMENT DEVICES PETRODIESEL FUEL Air-liquid Interface Biodiesel exhaust Biodiesel health effects Exhaust exposure Exhaust toxicology Primary human cell culture Air Pollutants Biofuels Epithelial Cells Gasoline Humans Particulate Matter Vehicle Emissions WAERP Epithelial Cells Humans Air Pollutants Gasoline Vehicle Emissions Particulate Matter Biofuels Biodiesel is created through the transesterification of fats/oils and its usage is increasing worldwide as global warming concerns increase. Biodiesel fuel properties change depending on the feedstock used to create it. The aim of this study was to assess the different toxicological properties of biodiesel exhausts created from different feedstocks using a complex 3D air-liquid interface (ALI) model that mimics the human airway. Primary human airway epithelial cells were grown at ALI until full differentiation was achieved. Cells were then exposed to 1/20 diluted exhaust from an engine running on Diesel (ULSD), pure or 20% blended Canola biodiesel and pure or 20% blended Tallow biodiesel, or Air for control. Exhaust was analysed for various physio-chemical properties and 24-h after exposure, ALI cultures were assessed for permeability, protein release and mediator response. All measured exhaust components were within industry safety standards. ULSD contained the highest concentrations of various combustion gases. We found no differences in terms of particle characteristics for any of the tested exhausts, likely due to the high dilution used. Exposure to Tallow B100 and B20 induced increased permeability in the ALI culture and the greatest increase in mediator response in both the apical and basal compartments. In contrast, Canola B100 and B20 did not impact permeability and induced the smallest mediator response. All exhausts but Canola B20 induced increased protein release, indicating epithelial damage. Despite the concentrations of all exhausts used in this study meeting industry safety regulations, we found significant toxic effects. Tallow biodiesel was found to be the most toxic of the tested fuels and Canola the least, both for blended and pure biodiesel fuels. This suggests that the feedstock biodiesel is made from is crucial for the resulting health effects of exhaust exposure, even when not comprising the majority of fuel composition. 2022 Journal Article http://hdl.handle.net/20.500.11937/91632 10.1016/j.scitotenv.2022.155016 English https://www.sciencedirect.com/science/article/am/pii/S004896972202109X http://purl.org/au-research/grants/arc/DP170104346 ELSEVIER fulltext
spellingShingle Science & Technology
Life Sciences & Biomedicine
Environmental Sciences
Environmental Sciences & Ecology
Exhaust toxicology
Biodiesel health effects
Air-liquid Interface
Exhaust exposure
Biodiesel exhaust
Primary human cell culture
28-DAY INHALATION EXPOSURE
DIESEL-ENGINE EXHAUST
OXIDATIVE STRESS
PARTICULATE MATTER
2ND-GENERATION BIODIESEL
IN-VITRO
SYSTEMIC INFLAMMATION
BARRIER INTEGRITY
TREATMENT DEVICES
PETRODIESEL FUEL
Air-liquid Interface
Biodiesel exhaust
Biodiesel health effects
Exhaust exposure
Exhaust toxicology
Primary human cell culture
Air Pollutants
Biofuels
Epithelial Cells
Gasoline
Humans
Particulate Matter
Vehicle Emissions
WAERP
Epithelial Cells
Humans
Air Pollutants
Gasoline
Vehicle Emissions
Particulate Matter
Biofuels
Landwehr, K.R.
Hillas, J.
Mead-Hunter, Ryan
King, A.
O'Leary, R.A.
Kicic, Anthony
Mullins, Ben
Larcombe, Alexander
Toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface
title Toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface
title_full Toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface
title_fullStr Toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface
title_full_unstemmed Toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface
title_short Toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface
title_sort toxicity of different biodiesel exhausts in primary human airway epithelial cells grown at air-liquid interface
topic Science & Technology
Life Sciences & Biomedicine
Environmental Sciences
Environmental Sciences & Ecology
Exhaust toxicology
Biodiesel health effects
Air-liquid Interface
Exhaust exposure
Biodiesel exhaust
Primary human cell culture
28-DAY INHALATION EXPOSURE
DIESEL-ENGINE EXHAUST
OXIDATIVE STRESS
PARTICULATE MATTER
2ND-GENERATION BIODIESEL
IN-VITRO
SYSTEMIC INFLAMMATION
BARRIER INTEGRITY
TREATMENT DEVICES
PETRODIESEL FUEL
Air-liquid Interface
Biodiesel exhaust
Biodiesel health effects
Exhaust exposure
Exhaust toxicology
Primary human cell culture
Air Pollutants
Biofuels
Epithelial Cells
Gasoline
Humans
Particulate Matter
Vehicle Emissions
WAERP
Epithelial Cells
Humans
Air Pollutants
Gasoline
Vehicle Emissions
Particulate Matter
Biofuels
url https://www.sciencedirect.com/science/article/am/pii/S004896972202109X
https://www.sciencedirect.com/science/article/am/pii/S004896972202109X
http://hdl.handle.net/20.500.11937/91632