A low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries

Solid-state batteries (SSBs) have attracted considerable attention due to their high intrinsic stability and theoretical energy density. As the core part, garnet electrolyte has been extensively investigated due to its high lithium-ion conductivity, wide electrochemical potential window, and easy sy...

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Main Authors: Cao, Chencheng, Zhong, Yijun, Chandula Wasalathilake, Kimal, Tadé, Moses O., Xu, Xiaomin, Rabiee, H., Roknuzzaman, M., Rahman, R., Shao, Zongping
Format: Journal Article
Language:English
Published: ROYAL SOC CHEMISTRY 2022
Subjects:
Online Access:http://purl.org/au-research/grants/arc/DP200103315
http://hdl.handle.net/20.500.11937/90619
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author Cao, Chencheng
Zhong, Yijun
Chandula Wasalathilake, Kimal
Tadé, Moses O.
Xu, Xiaomin
Rabiee, H.
Roknuzzaman, M.
Rahman, R.
Shao, Zongping
author_facet Cao, Chencheng
Zhong, Yijun
Chandula Wasalathilake, Kimal
Tadé, Moses O.
Xu, Xiaomin
Rabiee, H.
Roknuzzaman, M.
Rahman, R.
Shao, Zongping
author_sort Cao, Chencheng
building Curtin Institutional Repository
collection Online Access
description Solid-state batteries (SSBs) have attracted considerable attention due to their high intrinsic stability and theoretical energy density. As the core part, garnet electrolyte has been extensively investigated due to its high lithium-ion conductivity, wide electrochemical potential window, and easy synthesis. However, the poor and electrochemically unstable interfacial contact between the electrolyte and lithium anode greatly impedes the practical use of garnet based SSBs. Here, we report that such an interface challenge can be perfectly tackled by introducing multifunctional Li0.3La0.5TiO3 (LLTO) as an additive into the lithium anode. The limited reaction between the LLTO and lithium effectively changes the physical properties of the lithium anode, making it perfectly compatible with the garnet surface, and consequently significantly decreasing the interfacial resistance from 200 to only 48 Ω cm2 and greatly improving the interface stability and avoiding dendrite formation. Interestingly, LLTO provides additional lithium storage, and the close interface contact and the high lithium-ion conductivity of LLTO ensure high rate performance. Consequently, the symmetrical cell runs stably at 0.1 mA cm-2 for 400 h without obvious degradation. The SSB assembled with the LiFePO4 cathode and Li-LLTO composite anode demonstrates a specific capacity of 147 mA h g-1 and remarkable cycling stability with only 10% capacity decay over 700 cycles at 1C. This journal is
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institution Curtin University Malaysia
institution_category Local University
language English
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publishDate 2022
publisher ROYAL SOC CHEMISTRY
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spelling curtin-20.500.11937-906192023-03-27T02:37:54Z A low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries Cao, Chencheng Zhong, Yijun Chandula Wasalathilake, Kimal Tadé, Moses O. Xu, Xiaomin Rabiee, H. Roknuzzaman, M. Rahman, R. Shao, Zongping Science & Technology Physical Sciences Technology Chemistry, Physical Energy & Fuels Materials Science, Multidisciplinary Chemistry Materials Science NEUTRON-DIFFRACTION CHALLENGES INTERPHASE CONDUCTION MEMBRANE DESIGN Solid-state batteries (SSBs) have attracted considerable attention due to their high intrinsic stability and theoretical energy density. As the core part, garnet electrolyte has been extensively investigated due to its high lithium-ion conductivity, wide electrochemical potential window, and easy synthesis. However, the poor and electrochemically unstable interfacial contact between the electrolyte and lithium anode greatly impedes the practical use of garnet based SSBs. Here, we report that such an interface challenge can be perfectly tackled by introducing multifunctional Li0.3La0.5TiO3 (LLTO) as an additive into the lithium anode. The limited reaction between the LLTO and lithium effectively changes the physical properties of the lithium anode, making it perfectly compatible with the garnet surface, and consequently significantly decreasing the interfacial resistance from 200 to only 48 Ω cm2 and greatly improving the interface stability and avoiding dendrite formation. Interestingly, LLTO provides additional lithium storage, and the close interface contact and the high lithium-ion conductivity of LLTO ensure high rate performance. Consequently, the symmetrical cell runs stably at 0.1 mA cm-2 for 400 h without obvious degradation. The SSB assembled with the LiFePO4 cathode and Li-LLTO composite anode demonstrates a specific capacity of 147 mA h g-1 and remarkable cycling stability with only 10% capacity decay over 700 cycles at 1C. This journal is 2022 Journal Article http://hdl.handle.net/20.500.11937/90619 10.1039/d1ta07804f English http://purl.org/au-research/grants/arc/DP200103315 http://purl.org/au-research/grants/arc/DP200103332 ROYAL SOC CHEMISTRY restricted
spellingShingle Science & Technology
Physical Sciences
Technology
Chemistry, Physical
Energy & Fuels
Materials Science, Multidisciplinary
Chemistry
Materials Science
NEUTRON-DIFFRACTION
CHALLENGES
INTERPHASE
CONDUCTION
MEMBRANE
DESIGN
Cao, Chencheng
Zhong, Yijun
Chandula Wasalathilake, Kimal
Tadé, Moses O.
Xu, Xiaomin
Rabiee, H.
Roknuzzaman, M.
Rahman, R.
Shao, Zongping
A low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries
title A low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries
title_full A low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries
title_fullStr A low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries
title_full_unstemmed A low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries
title_short A low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries
title_sort low resistance and stable lithium-garnet electrolyte interface enabled by a multifunctional anode additive for solid-state lithium batteries
topic Science & Technology
Physical Sciences
Technology
Chemistry, Physical
Energy & Fuels
Materials Science, Multidisciplinary
Chemistry
Materials Science
NEUTRON-DIFFRACTION
CHALLENGES
INTERPHASE
CONDUCTION
MEMBRANE
DESIGN
url http://purl.org/au-research/grants/arc/DP200103315
http://purl.org/au-research/grants/arc/DP200103315
http://hdl.handle.net/20.500.11937/90619