Exceptional preservation of palaeozoic steroids in a diagenetic continuum

The occurrence of intact sterols has been restricted to immature Cretaceous (~125 Ma) sediments with one report from the Late Jurassic (~165 Ma). Here we report the oldest occurrence of intact sterols in a Crustacean fossil preserved for ca. 380 Ma within a Devonian concretion. The exceptional prese...

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Main Authors: Melendez, Ines, Grice, Kliti, Schwark, Lorenz
Format: Journal Article
Published: Nature Publishing Group 2013
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Online Access:http://hdl.handle.net/20.500.11937/8544
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author Melendez, Ines
Grice, Kliti
Schwark, Lorenz
author_facet Melendez, Ines
Grice, Kliti
Schwark, Lorenz
author_sort Melendez, Ines
building Curtin Institutional Repository
collection Online Access
description The occurrence of intact sterols has been restricted to immature Cretaceous (~125 Ma) sediments with one report from the Late Jurassic (~165 Ma). Here we report the oldest occurrence of intact sterols in a Crustacean fossil preserved for ca. 380 Ma within a Devonian concretion. The exceptional preservation of the biomass is attributed to microbially induced carbonate encapsulation, preventing full decomposition and transformation thus extending sterol occurrences in the geosphere by 250 Ma. A suite of diagenetic transformation products of sterols was also identified in the concretion, demonstrating the remarkable coexistence of biomolecules and geomolecules in the same sample. Most importantly the original biolipids were found to be the most abundant steroids in the sample. We attribute the coexistence of steroids in a diagenetic continuum-ranging from stenols to triaromatic steroids-to microbially mediated eogenetic processes.
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spelling curtin-20.500.11937-85442017-09-13T14:52:45Z Exceptional preservation of palaeozoic steroids in a diagenetic continuum Melendez, Ines Grice, Kliti Schwark, Lorenz palaeoclimate biogeochemistry sterols geochemistry The occurrence of intact sterols has been restricted to immature Cretaceous (~125 Ma) sediments with one report from the Late Jurassic (~165 Ma). Here we report the oldest occurrence of intact sterols in a Crustacean fossil preserved for ca. 380 Ma within a Devonian concretion. The exceptional preservation of the biomass is attributed to microbially induced carbonate encapsulation, preventing full decomposition and transformation thus extending sterol occurrences in the geosphere by 250 Ma. A suite of diagenetic transformation products of sterols was also identified in the concretion, demonstrating the remarkable coexistence of biomolecules and geomolecules in the same sample. Most importantly the original biolipids were found to be the most abundant steroids in the sample. We attribute the coexistence of steroids in a diagenetic continuum-ranging from stenols to triaromatic steroids-to microbially mediated eogenetic processes. 2013 Journal Article http://hdl.handle.net/20.500.11937/8544 10.1038/srep02768 Nature Publishing Group fulltext
spellingShingle palaeoclimate
biogeochemistry
sterols
geochemistry
Melendez, Ines
Grice, Kliti
Schwark, Lorenz
Exceptional preservation of palaeozoic steroids in a diagenetic continuum
title Exceptional preservation of palaeozoic steroids in a diagenetic continuum
title_full Exceptional preservation of palaeozoic steroids in a diagenetic continuum
title_fullStr Exceptional preservation of palaeozoic steroids in a diagenetic continuum
title_full_unstemmed Exceptional preservation of palaeozoic steroids in a diagenetic continuum
title_short Exceptional preservation of palaeozoic steroids in a diagenetic continuum
title_sort exceptional preservation of palaeozoic steroids in a diagenetic continuum
topic palaeoclimate
biogeochemistry
sterols
geochemistry
url http://hdl.handle.net/20.500.11937/8544