Metal coordination with an amide-functionalized axially chiral resorcinarene

The synthesis and characterization of an amide-functionalized axially chiral resorcinarene, 14,36,56,76-tetra-2-oxo-2-(2-hydroxyethylamino)ethoxy-16,34,54,74-tetramethoxy-2,4,6,8- tetrapropylresorcin[4]arene, is reported. Metal complexation with picrate salts gave crystalline products that could be...

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Main Authors: Vaughan, Jamila, Bertata, Munna Ali Mohamed, Skelton, B.W., Ogden, Mark, Mocerino, Mauro
Format: Journal Article
Language:English
Published: SPRINGER 2019
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/76622
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author Vaughan, Jamila
Bertata, Munna Ali Mohamed
Skelton, B.W.
Ogden, Mark
Mocerino, Mauro
author_facet Vaughan, Jamila
Bertata, Munna Ali Mohamed
Skelton, B.W.
Ogden, Mark
Mocerino, Mauro
author_sort Vaughan, Jamila
building Curtin Institutional Repository
collection Online Access
description The synthesis and characterization of an amide-functionalized axially chiral resorcinarene, 14,36,56,76-tetra-2-oxo-2-(2-hydroxyethylamino)ethoxy-16,34,54,74-tetramethoxy-2,4,6,8- tetrapropylresorcin[4]arene, is reported. Metal complexation with picrate salts gave crystalline products that could be structurally characterised for calcium, lanthanum, praseodymium, and ytterbium. While the details of these structures vary, the metal–ligand interactions are remarkably consistent, with coordination polymers formed through interaction between three of the amide O atoms, each binding to a different metal atom. No other potential donor atom of the macrocycle is bound to the metal atoms, with the coordination spheres completed by solvent or picrate donor O atoms.
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spelling curtin-20.500.11937-766222020-06-02T00:39:54Z Metal coordination with an amide-functionalized axially chiral resorcinarene Vaughan, Jamila Bertata, Munna Ali Mohamed Skelton, B.W. Ogden, Mark Mocerino, Mauro Science & Technology Physical Sciences Chemistry, Multidisciplinary Chemistry Resorcinarene Lanthanide Picrate Crystal structure RARE-EARTH COMPLEXES CRYSTAL-STRUCTURE STRUCTURAL-CHARACTERIZATION SYSTEMATICS The synthesis and characterization of an amide-functionalized axially chiral resorcinarene, 14,36,56,76-tetra-2-oxo-2-(2-hydroxyethylamino)ethoxy-16,34,54,74-tetramethoxy-2,4,6,8- tetrapropylresorcin[4]arene, is reported. Metal complexation with picrate salts gave crystalline products that could be structurally characterised for calcium, lanthanum, praseodymium, and ytterbium. While the details of these structures vary, the metal–ligand interactions are remarkably consistent, with coordination polymers formed through interaction between three of the amide O atoms, each binding to a different metal atom. No other potential donor atom of the macrocycle is bound to the metal atoms, with the coordination spheres completed by solvent or picrate donor O atoms. 2019 Journal Article http://hdl.handle.net/20.500.11937/76622 10.1007/s10847-019-00922-w English SPRINGER fulltext
spellingShingle Science & Technology
Physical Sciences
Chemistry, Multidisciplinary
Chemistry
Resorcinarene
Lanthanide
Picrate
Crystal structure
RARE-EARTH COMPLEXES
CRYSTAL-STRUCTURE
STRUCTURAL-CHARACTERIZATION
SYSTEMATICS
Vaughan, Jamila
Bertata, Munna Ali Mohamed
Skelton, B.W.
Ogden, Mark
Mocerino, Mauro
Metal coordination with an amide-functionalized axially chiral resorcinarene
title Metal coordination with an amide-functionalized axially chiral resorcinarene
title_full Metal coordination with an amide-functionalized axially chiral resorcinarene
title_fullStr Metal coordination with an amide-functionalized axially chiral resorcinarene
title_full_unstemmed Metal coordination with an amide-functionalized axially chiral resorcinarene
title_short Metal coordination with an amide-functionalized axially chiral resorcinarene
title_sort metal coordination with an amide-functionalized axially chiral resorcinarene
topic Science & Technology
Physical Sciences
Chemistry, Multidisciplinary
Chemistry
Resorcinarene
Lanthanide
Picrate
Crystal structure
RARE-EARTH COMPLEXES
CRYSTAL-STRUCTURE
STRUCTURAL-CHARACTERIZATION
SYSTEMATICS
url http://hdl.handle.net/20.500.11937/76622